A versatile functionalized ionic liquid to boost the solution-mediated performances of lithium-oxygen batteries
Due to the high theoretical specific energy, the lithium–oxygen battery has been heralded as a promising energy storage system for applications such as electric vehicles. However, its large over-potentials during discharge–charge cycling lead to the formation of side-products, and short cycle life....
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| Published in | Nature communications Vol. 10; no. 1; pp. 602 - 10 |
|---|---|
| Main Authors | , , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
05.02.2019
Nature Publishing Group Nature Portfolio |
| Subjects | |
| Online Access | Get full text |
| ISSN | 2041-1723 2041-1723 |
| DOI | 10.1038/s41467-019-08422-8 |
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| Abstract | Due to the high theoretical specific energy, the lithium–oxygen battery has been heralded as a promising energy storage system for applications such as electric vehicles. However, its large over-potentials during discharge–charge cycling lead to the formation of side-products, and short cycle life. Herein, we report an ionic liquid bearing the redox active 2,2,6,6-tetramethyl-1-piperidinyloxy moiety, which serves multiple functions as redox mediator, oxygen shuttle, lithium anode protector, as well as electrolyte solvent. The additive contributes a 33-fold increase of the discharge capacity in comparison to a pure ether-based electrolyte and lowers the over-potential to an exceptionally low value of 0.9 V. Meanwhile, its molecule facilitates smooth lithium plating/stripping, and promotes the formation of a stable solid electrolyte interface to suppress side-reactions. Moreover, the proportion of ionic liquid in the electrolyte influences the reaction mechanism, and a high proportion leads to the formation of amorphous lithium peroxide and a long cycling life (> 200 cycles). In particular, it enables an outstanding electrochemical performance when operated in air.
Li-O
2
batteries are promising candidates for the next generation of rechargeable batteries, but the side reactions and poor cycling stability limit their applications. Here, the authors show a versatile ionic liquid with functional groups that can address both issues for cells operated in oxygen and air. |
|---|---|
| AbstractList | Due to the high theoretical specific energy, the lithium–oxygen battery has been heralded as a promising energy storage system for applications such as electric vehicles. However, its large over-potentials during discharge–charge cycling lead to the formation of side-products, and short cycle life. Herein, we report an ionic liquid bearing the redox active 2,2,6,6-tetramethyl-1-piperidinyloxy moiety, which serves multiple functions as redox mediator, oxygen shuttle, lithium anode protector, as well as electrolyte solvent. The additive contributes a 33-fold increase of the discharge capacity in comparison to a pure ether-based electrolyte and lowers the over-potential to an exceptionally low value of 0.9 V. Meanwhile, its molecule facilitates smooth lithium plating/stripping, and promotes the formation of a stable solid electrolyte interface to suppress side-reactions. Moreover, the proportion of ionic liquid in the electrolyte influences the reaction mechanism, and a high proportion leads to the formation of amorphous lithium peroxide and a long cycling life (> 200 cycles). In particular, it enables an outstanding electrochemical performance when operated in air.Li-O2 batteries are promising candidates for the next generation of rechargeable batteries, but the side reactions and poor cycling stability limit their applications. Here, the authors show a versatile ionic liquid with functional groups that can address both issues for cells operated in oxygen and air. Due to the high theoretical specific energy, the lithium–oxygen battery has been heralded as a promising energy storage system for applications such as electric vehicles. However, its large over-potentials during discharge–charge cycling lead to the formation of side-products, and short cycle life. Herein, we report an ionic liquid bearing the redox active 2,2,6,6-tetramethyl-1-piperidinyloxy moiety, which serves multiple functions as redox mediator, oxygen shuttle, lithium anode protector, as well as electrolyte solvent. The additive contributes a 33-fold increase of the discharge capacity in comparison to a pure ether-based electrolyte and lowers the over-potential to an exceptionally low value of 0.9 V. Meanwhile, its molecule facilitates smooth lithium plating/stripping, and promotes the formation of a stable solid electrolyte interface to suppress side-reactions. Moreover, the proportion of ionic liquid in the electrolyte influences the reaction mechanism, and a high proportion leads to the formation of amorphous lithium peroxide and a long cycling life (> 200 cycles). In particular, it enables an outstanding electrochemical performance when operated in air. Due to the high theoretical specific energy, the lithium–oxygen battery has been heralded as a promising energy storage system for applications such as electric vehicles. However, its large over-potentials during discharge–charge cycling lead to the formation of side-products, and short cycle life. Herein, we report an ionic liquid bearing the redox active 2,2,6,6-tetramethyl-1-piperidinyloxy moiety, which serves multiple functions as redox mediator, oxygen shuttle, lithium anode protector, as well as electrolyte solvent. The additive contributes a 33-fold increase of the discharge capacity in comparison to a pure ether-based electrolyte and lowers the over-potential to an exceptionally low value of 0.9 V. Meanwhile, its molecule facilitates smooth lithium plating/stripping, and promotes the formation of a stable solid electrolyte interface to suppress side-reactions. Moreover, the proportion of ionic liquid in the electrolyte influences the reaction mechanism, and a high proportion leads to the formation of amorphous lithium peroxide and a long cycling life (> 200 cycles). In particular, it enables an outstanding electrochemical performance when operated in air. Li-O 2 batteries are promising candidates for the next generation of rechargeable batteries, but the side reactions and poor cycling stability limit their applications. Here, the authors show a versatile ionic liquid with functional groups that can address both issues for cells operated in oxygen and air. Li-O2 batteries are promising candidates for the next generation of rechargeable batteries, but the side reactions and poor cycling stability limit their applications. Here, the authors show a versatile ionic liquid with functional groups that can address both issues for cells operated in oxygen and air. Due to the high theoretical specific energy, the lithium-oxygen battery has been heralded as a promising energy storage system for applications such as electric vehicles. However, its large over-potentials during discharge-charge cycling lead to the formation of side-products, and short cycle life. Herein, we report an ionic liquid bearing the redox active 2,2,6,6-tetramethyl-1-piperidinyloxy moiety, which serves multiple functions as redox mediator, oxygen shuttle, lithium anode protector, as well as electrolyte solvent. The additive contributes a 33-fold increase of the discharge capacity in comparison to a pure ether-based electrolyte and lowers the over-potential to an exceptionally low value of 0.9 V. Meanwhile, its molecule facilitates smooth lithium plating/stripping, and promotes the formation of a stable solid electrolyte interface to suppress side-reactions. Moreover, the proportion of ionic liquid in the electrolyte influences the reaction mechanism, and a high proportion leads to the formation of amorphous lithium peroxide and a long cycling life (> 200 cycles). In particular, it enables an outstanding electrochemical performance when operated in air.Due to the high theoretical specific energy, the lithium-oxygen battery has been heralded as a promising energy storage system for applications such as electric vehicles. However, its large over-potentials during discharge-charge cycling lead to the formation of side-products, and short cycle life. Herein, we report an ionic liquid bearing the redox active 2,2,6,6-tetramethyl-1-piperidinyloxy moiety, which serves multiple functions as redox mediator, oxygen shuttle, lithium anode protector, as well as electrolyte solvent. The additive contributes a 33-fold increase of the discharge capacity in comparison to a pure ether-based electrolyte and lowers the over-potential to an exceptionally low value of 0.9 V. Meanwhile, its molecule facilitates smooth lithium plating/stripping, and promotes the formation of a stable solid electrolyte interface to suppress side-reactions. Moreover, the proportion of ionic liquid in the electrolyte influences the reaction mechanism, and a high proportion leads to the formation of amorphous lithium peroxide and a long cycling life (> 200 cycles). In particular, it enables an outstanding electrochemical performance when operated in air. |
| ArticleNumber | 602 |
| Author | Tkacheva, Anastasia Armand, Michel Wang, Chengyin Zhao, Yufei Peng, Zhangquan Liu, Zhenjie Yan, Kang Rojo, Teofilo Shanmukaraj, Devaraj Guo, Xin McDonagh, Andrew M. Wang, Guoxiu Sun, Bing Zhang, Jinqiang |
| Author_xml | – sequence: 1 givenname: Jinqiang orcidid: 0000-0001-5476-0134 surname: Zhang fullname: Zhang, Jinqiang organization: Centre for Clean Energy Technology, University of Technology Sydney, Broadway – sequence: 2 givenname: Bing surname: Sun fullname: Sun, Bing organization: Centre for Clean Energy Technology, University of Technology Sydney, Broadway – sequence: 3 givenname: Yufei surname: Zhao fullname: Zhao, Yufei organization: Centre for Clean Energy Technology, University of Technology Sydney, Broadway, Department of Materials Science and Engineering, Dongguan University of Technology – sequence: 4 givenname: Anastasia surname: Tkacheva fullname: Tkacheva, Anastasia organization: Centre for Clean Energy Technology, University of Technology Sydney, Broadway – sequence: 5 givenname: Zhenjie surname: Liu fullname: Liu, Zhenjie organization: State Key Laboratory of Electroanalytical Chemistry, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences – sequence: 6 givenname: Kang surname: Yan fullname: Yan, Kang organization: Centre for Clean Energy Technology, University of Technology Sydney, Broadway – sequence: 7 givenname: Xin surname: Guo fullname: Guo, Xin organization: Centre for Clean Energy Technology, University of Technology Sydney, Broadway – sequence: 8 givenname: Andrew M. surname: McDonagh fullname: McDonagh, Andrew M. organization: Centre for Clean Energy Technology, University of Technology Sydney, Broadway – sequence: 9 givenname: Devaraj surname: Shanmukaraj fullname: Shanmukaraj, Devaraj organization: CIC EnergiGUNE – sequence: 10 givenname: Chengyin surname: Wang fullname: Wang, Chengyin organization: College of Chemistry and Chemical Engineering, Yangzhou University – sequence: 11 givenname: Teofilo surname: Rojo fullname: Rojo, Teofilo organization: CIC EnergiGUNE – sequence: 12 givenname: Michel surname: Armand fullname: Armand, Michel email: marmand@cicenergigune.com organization: CIC EnergiGUNE – sequence: 13 givenname: Zhangquan surname: Peng fullname: Peng, Zhangquan email: zqpeng@ciac.ac.cn organization: State Key Laboratory of Electroanalytical Chemistry, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences – sequence: 14 givenname: Guoxiu orcidid: 0000-0003-4295-8578 surname: Wang fullname: Wang, Guoxiu email: Guoxiu.Wang@uts.edu.au organization: Centre for Clean Energy Technology, University of Technology Sydney, Broadway |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/30723193$$D View this record in MEDLINE/PubMed |
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| Snippet | Due to the high theoretical specific energy, the lithium–oxygen battery has been heralded as a promising energy storage system for applications such as... Due to the high theoretical specific energy, the lithium-oxygen battery has been heralded as a promising energy storage system for applications such as... Li-O2 batteries are promising candidates for the next generation of rechargeable batteries, but the side reactions and poor cycling stability limit their... |
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| Title | A versatile functionalized ionic liquid to boost the solution-mediated performances of lithium-oxygen batteries |
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