Large‐Scale, Mechanically Robust, Solvent‐Resistant, and Antioxidant MXene‐Based Composites for Reliable Long‐Term Infrared Stealth

MXene‐based thermal camouflage materials have gained increasing attention due to their low emissivity, however, the poor anti‐oxidation restricts their potential applications under complex environments. Various modification methods and strategies, e.g., the addition of antioxidant molecules and fill...

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Published inAdvanced science Vol. 11; no. 17; pp. e2309392 - n/a
Main Authors Guo, Bi‐Fan, Wang, Ye‐Jun, Cao, Cheng‐Fei, Qu, Zhang‐Hao, Song, Jiang, Li, Shi‐Neng, Gao, Jie‐Feng, Song, Pingan, Zhang, Guo‐Dong, Shi, Yong‐Qian, Tang, Long‐Cheng
Format Journal Article
LanguageEnglish
Published Germany John Wiley & Sons, Inc 01.05.2024
John Wiley and Sons Inc
Wiley
Subjects
Aging
Antioxidants
Aqueous solutions
Composite materials
Cotton
infrared stealth
long‐term anti‐oxidation
micro‐/nanoarchitecture
Molecular weight
MXene
Nanoparticles
Oxidation
Radiation
Temperature
Textiles
weather resistance
micro‐/nanoarchitecture
long‐term anti‐oxidation
infrared stealth
MXene
weather resistance
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Abstract MXene‐based thermal camouflage materials have gained increasing attention due to their low emissivity, however, the poor anti‐oxidation restricts their potential applications under complex environments. Various modification methods and strategies, e.g., the addition of antioxidant molecules and fillers have been developed to overcome this, but the realization of long‐term, reliable thermal camouflage using MXene network (coating) with excellent comprehensive performance remains a great challenge. Here, a MXene‐based hybrid network comodified with hyaluronic acid (HA) and hyperbranched polysiloxane (HSi) molecules is designed and fabricated. Notably, the presence of appreciated HA molecules restricts the oxidation of MXene sheets without altering infrared stealth performance, superior to other water‐soluble polymers; while the HSi molecules can act as efficient cross‐linking agents to generate strong interactions between MXene sheets and HA molecules. The optimized MXene/HA/HSi composites exhibit excellent mechanical flexibility (folded into crane structure), good water/solvent resistance, and long‐term stable thermal camouflage capability (with low infrared emissivity of ≈0.29). The long‐term thermal camouflage reliability (≈8 months) under various outdoor weathers and the scalable coating capability of the MXene‐coated textile enable them to disguise the IR signal of various targets in complex environments, indicating the great promise of achieved material for thermal camouflage, IR stealth, and counter surveillance. A high‐performance thermal camouflage material is designed and successfully fabricated by decorating MXene network with hyaluronic acid (HA) and hyperbranched polysiloxane (HSi). Besides excellent mid‐infrared (IR) thermal camouflage, such material also integrates multiple advantages into itself, including being large‐scale, mechanically flexible, weather‐resistant, and thus showing great potential for stealth applications.
AbstractList MXene‐based thermal camouflage materials have gained increasing attention due to their low emissivity, however, the poor anti‐oxidation restricts their potential applications under complex environments. Various modification methods and strategies, e.g., the addition of antioxidant molecules and fillers have been developed to overcome this, but the realization of long‐term, reliable thermal camouflage using MXene network (coating) with excellent comprehensive performance remains a great challenge. Here, a MXene‐based hybrid network comodified with hyaluronic acid (HA) and hyperbranched polysiloxane (HSi) molecules is designed and fabricated. Notably, the presence of appreciated HA molecules restricts the oxidation of MXene sheets without altering infrared stealth performance, superior to other water‐soluble polymers; while the HSi molecules can act as efficient cross‐linking agents to generate strong interactions between MXene sheets and HA molecules. The optimized MXene/HA/HSi composites exhibit excellent mechanical flexibility (folded into crane structure), good water/solvent resistance, and long‐term stable thermal camouflage capability (with low infrared emissivity of ≈0.29). The long‐term thermal camouflage reliability (≈8 months) under various outdoor weathers and the scalable coating capability of the MXene‐coated textile enable them to disguise the IR signal of various targets in complex environments, indicating the great promise of achieved material for thermal camouflage, IR stealth, and counter surveillance.
MXene-based thermal camouflage materials have gained increasing attention due to their low emissivity, however, the poor anti-oxidation restricts their potential applications under complex environments. Various modification methods and strategies, e.g., the addition of antioxidant molecules and fillers have been developed to overcome this, but the realization of long-term, reliable thermal camouflage using MXene network (coating) with excellent comprehensive performance remains a great challenge. Here, a MXene-based hybrid network comodified with hyaluronic acid (HA) and hyperbranched polysiloxane (HSi) molecules is designed and fabricated. Notably, the presence of appreciated HA molecules restricts the oxidation of MXene sheets without altering infrared stealth performance, superior to other water-soluble polymers; while the HSi molecules can act as efficient cross-linking agents to generate strong interactions between MXene sheets and HA molecules. The optimized MXene/HA/HSi composites exhibit excellent mechanical flexibility (folded into crane structure), good water/solvent resistance, and long-term stable thermal camouflage capability (with low infrared emissivity of ≈0.29). The long-term thermal camouflage reliability (≈8 months) under various outdoor weathers and the scalable coating capability of the MXene-coated textile enable them to disguise the IR signal of various targets in complex environments, indicating the great promise of achieved material for thermal camouflage, IR stealth, and counter surveillance.MXene-based thermal camouflage materials have gained increasing attention due to their low emissivity, however, the poor anti-oxidation restricts their potential applications under complex environments. Various modification methods and strategies, e.g., the addition of antioxidant molecules and fillers have been developed to overcome this, but the realization of long-term, reliable thermal camouflage using MXene network (coating) with excellent comprehensive performance remains a great challenge. Here, a MXene-based hybrid network comodified with hyaluronic acid (HA) and hyperbranched polysiloxane (HSi) molecules is designed and fabricated. Notably, the presence of appreciated HA molecules restricts the oxidation of MXene sheets without altering infrared stealth performance, superior to other water-soluble polymers; while the HSi molecules can act as efficient cross-linking agents to generate strong interactions between MXene sheets and HA molecules. The optimized MXene/HA/HSi composites exhibit excellent mechanical flexibility (folded into crane structure), good water/solvent resistance, and long-term stable thermal camouflage capability (with low infrared emissivity of ≈0.29). The long-term thermal camouflage reliability (≈8 months) under various outdoor weathers and the scalable coating capability of the MXene-coated textile enable them to disguise the IR signal of various targets in complex environments, indicating the great promise of achieved material for thermal camouflage, IR stealth, and counter surveillance.
Abstract MXene‐based thermal camouflage materials have gained increasing attention due to their low emissivity, however, the poor anti‐oxidation restricts their potential applications under complex environments. Various modification methods and strategies, e.g., the addition of antioxidant molecules and fillers have been developed to overcome this, but the realization of long‐term, reliable thermal camouflage using MXene network (coating) with excellent comprehensive performance remains a great challenge. Here, a MXene‐based hybrid network comodified with hyaluronic acid (HA) and hyperbranched polysiloxane (HSi) molecules is designed and fabricated. Notably, the presence of appreciated HA molecules restricts the oxidation of MXene sheets without altering infrared stealth performance, superior to other water‐soluble polymers; while the HSi molecules can act as efficient cross‐linking agents to generate strong interactions between MXene sheets and HA molecules. The optimized MXene/HA/HSi composites exhibit excellent mechanical flexibility (folded into crane structure), good water/solvent resistance, and long‐term stable thermal camouflage capability (with low infrared emissivity of ≈0.29). The long‐term thermal camouflage reliability (≈8 months) under various outdoor weathers and the scalable coating capability of the MXene‐coated textile enable them to disguise the IR signal of various targets in complex environments, indicating the great promise of achieved material for thermal camouflage, IR stealth, and counter surveillance.
MXene‐based thermal camouflage materials have gained increasing attention due to their low emissivity, however, the poor anti‐oxidation restricts their potential applications under complex environments. Various modification methods and strategies, e.g., the addition of antioxidant molecules and fillers have been developed to overcome this, but the realization of long‐term, reliable thermal camouflage using MXene network (coating) with excellent comprehensive performance remains a great challenge. Here, a MXene‐based hybrid network comodified with hyaluronic acid (HA) and hyperbranched polysiloxane (HSi) molecules is designed and fabricated. Notably, the presence of appreciated HA molecules restricts the oxidation of MXene sheets without altering infrared stealth performance, superior to other water‐soluble polymers; while the HSi molecules can act as efficient cross‐linking agents to generate strong interactions between MXene sheets and HA molecules. The optimized MXene/HA/HSi composites exhibit excellent mechanical flexibility (folded into crane structure), good water/solvent resistance, and long‐term stable thermal camouflage capability (with low infrared emissivity of ≈0.29). The long‐term thermal camouflage reliability (≈8 months) under various outdoor weathers and the scalable coating capability of the MXene‐coated textile enable them to disguise the IR signal of various targets in complex environments, indicating the great promise of achieved material for thermal camouflage, IR stealth, and counter surveillance. A high‐performance thermal camouflage material is designed and successfully fabricated by decorating MXene network with hyaluronic acid (HA) and hyperbranched polysiloxane (HSi). Besides excellent mid‐infrared (IR) thermal camouflage, such material also integrates multiple advantages into itself, including being large‐scale, mechanically flexible, weather‐resistant, and thus showing great potential for stealth applications.
Author Song, Jiang
Zhang, Guo‐Dong
Gao, Jie‐Feng
Qu, Zhang‐Hao
Li, Shi‐Neng
Wang, Ye‐Jun
Song, Pingan
Cao, Cheng‐Fei
Shi, Yong‐Qian
Tang, Long‐Cheng
Guo, Bi‐Fan
AuthorAffiliation 1 College of Material, Chemistry and Chemical Engineering Key Laboratory of Organosilicon Chemistry and Material Technology of MoE Key Laboratory of Silicone Materials Technology of Zhejiang Province Hangzhou Normal University Hangzhou 311121 China
2 Centre for Future Materials University of Southern Queensland Springfield 4300 Australia
5 School of Agriculture and Environmental Science University of Southern Queensland Springfield 4300 Australia
6 College of Environment and Safety Engineering Fuzhou University Fuzhou 350116 China
3 College of Chemistry and Materials Engineering Zhejiang A&F University Hangzhou 311300 China
4 College of Chemistry and Chemical Engineering Yangzhou University Yangzhou Jiangsu 225002 China
AuthorAffiliation_xml – name: 5 School of Agriculture and Environmental Science University of Southern Queensland Springfield 4300 Australia
– name: 2 Centre for Future Materials University of Southern Queensland Springfield 4300 Australia
– name: 1 College of Material, Chemistry and Chemical Engineering Key Laboratory of Organosilicon Chemistry and Material Technology of MoE Key Laboratory of Silicone Materials Technology of Zhejiang Province Hangzhou Normal University Hangzhou 311121 China
– name: 3 College of Chemistry and Materials Engineering Zhejiang A&F University Hangzhou 311300 China
– name: 6 College of Environment and Safety Engineering Fuzhou University Fuzhou 350116 China
– name: 4 College of Chemistry and Chemical Engineering Yangzhou University Yangzhou Jiangsu 225002 China
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  fullname: Song, Jiang
  organization: Hangzhou Normal University
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  surname: Zhang
  fullname: Zhang, Guo‐Dong
  organization: Hangzhou Normal University
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  surname: Tang
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  email: lctang@hznu.edu.cn
  organization: Hangzhou Normal University
BackLink https://www.ncbi.nlm.nih.gov/pubmed/38403451$$D View this record in MEDLINE/PubMed
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Issue 17
Keywords micro‐/nanoarchitecture
long‐term anti‐oxidation
infrared stealth
MXene
weather resistance
Language English
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SSID ssj0001537418
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Snippet MXene‐based thermal camouflage materials have gained increasing attention due to their low emissivity, however, the poor anti‐oxidation restricts their...
MXene-based thermal camouflage materials have gained increasing attention due to their low emissivity, however, the poor anti-oxidation restricts their...
Abstract MXene‐based thermal camouflage materials have gained increasing attention due to their low emissivity, however, the poor anti‐oxidation restricts...
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StartPage e2309392
SubjectTerms Aging
Antioxidants
Aqueous solutions
Composite materials
Cotton
infrared stealth
long‐term anti‐oxidation
micro‐/nanoarchitecture
Molecular weight
MXene
Nanoparticles
Oxidation
Radiation
Temperature
Textiles
weather resistance
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Title Large‐Scale, Mechanically Robust, Solvent‐Resistant, and Antioxidant MXene‐Based Composites for Reliable Long‐Term Infrared Stealth
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fadvs.202309392
https://www.ncbi.nlm.nih.gov/pubmed/38403451
https://www.proquest.com/docview/3051837978
https://www.proquest.com/docview/2932017428
https://pubmed.ncbi.nlm.nih.gov/PMC11077694
https://doaj.org/article/9112c63a0f7a4261aa9685b286b89fbf
Volume 11
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