Facile Synthesis of Single Crystal Vanadium Disulfide Nanosheets by Chemical Vapor Deposition for Efficient Hydrogen Evolution Reaction

A facile chemical vapor deposition method to prepare single‐crystalline VS2 nanosheets for the hydrogen evolution reaction is reported. The electrocatalytic hydrogen evolution reaction (HER) activities of VS2 show an extremely low overpotential of −68 mV at 10 mA cm−2, small Tafel slopes of ≈34 mV d...

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Published in	Advanced materials (Weinheim) Vol. 27; no. 37; pp. 5605 - 5609
Main Authors	Yuan, Jiangtan, Wu, Jingjie, Hardy, Will J., Loya, Philip, Lou, Minhan, Yang, Yingchao, Najmaei, Sina, Jiang, Menglei, Qin, Fan, Keyshar, Kunttal, Ji, Heng, Gao, Weilu, Bao, Jiming, Kono, Junichiro, Natelson, Douglas, Ajayan, Pulickel M., Lou, Jun
Format	Journal Article
Language	English
Published	Germany Blackwell Publishing Ltd 07.10.2015
Subjects	Chemical vapor deposition Disulfides Hydrogen evolution hydrogen evolution reactions metals Nanostructure Single crystals Stability Synthesis (chemistry) Tafel slopes transition metal dichalcogenides vanadium disulfide metals vanadium disulfide hydrogen evolution reactions transition metal dichalcogenides chemical vapor deposition
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Abstract	A facile chemical vapor deposition method to prepare single‐crystalline VS2 nanosheets for the hydrogen evolution reaction is reported. The electrocatalytic hydrogen evolution reaction (HER) activities of VS2 show an extremely low overpotential of −68 mV at 10 mA cm−2, small Tafel slopes of ≈34 mV decade−1, as well as high stability, demonstrating its potential as a candidate non‐noble‐metal catalyst for the HER.
AbstractList	A facile chemical vapor deposition method to prepare single-crystalline VS sub(2) nanosheets for the hydrogen evolution reaction is reported. The electrocatalytic hydrogen evolution reaction (HER) activities of VS sub(2) show an extremely low overpotential of -68 mV at 10 mA cm super(-2), small Tafel slopes of approximately 34 mV decade super(-1), as well as high stability, demonstrating its potential as a candidate non-noble-metal catalyst for the HER. A facile chemical vapor deposition method to prepare single-crystalline VS2 nanosheets for the hydrogen evolution reaction is reported. The electrocatalytic hydrogen evolution reaction (HER) activities of VS2 show an extremely low overpotential of -68 mV at 10 mA cm(-2), small Tafel slopes of ≈34 mV decade(-1), as well as high stability, demonstrating its potential as a candidate non-noble-metal catalyst for the HER.A facile chemical vapor deposition method to prepare single-crystalline VS2 nanosheets for the hydrogen evolution reaction is reported. The electrocatalytic hydrogen evolution reaction (HER) activities of VS2 show an extremely low overpotential of -68 mV at 10 mA cm(-2), small Tafel slopes of ≈34 mV decade(-1), as well as high stability, demonstrating its potential as a candidate non-noble-metal catalyst for the HER. A facile chemical vapor deposition method to prepare single-crystalline VS2 nanosheets for the hydrogen evolution reaction is reported. The electrocatalytic hydrogen evolution reaction (HER) activities of VS2 show an extremely low overpotential of -68 mV at 10 mA cm(-2), small Tafel slopes of ≈34 mV decade(-1), as well as high stability, demonstrating its potential as a candidate non-noble-metal catalyst for the HER. A facile chemical vapor deposition method to prepare single‐crystalline VS2 nanosheets for the hydrogen evolution reaction is reported. The electrocatalytic hydrogen evolution reaction (HER) activities of VS2 show an extremely low overpotential of −68 mV at 10 mA cm−2, small Tafel slopes of ≈34 mV decade−1, as well as high stability, demonstrating its potential as a candidate non‐noble‐metal catalyst for the HER.
Author	Ajayan, Pulickel M. Najmaei, Sina Bao, Jiming Yuan, Jiangtan Jiang, Menglei Gao, Weilu Kono, Junichiro Lou, Jun Hardy, Will J. Loya, Philip Wu, Jingjie Lou, Minhan Ji, Heng Qin, Fan Natelson, Douglas Keyshar, Kunttal Yang, Yingchao
Author_xml	– sequence: 1 givenname: Jiangtan surname: Yuan fullname: Yuan, Jiangtan organization: Department of Materials Science and NanoEngineering, Rice University, TX, 77005, Houston, USA – sequence: 2 givenname: Jingjie surname: Wu fullname: Wu, Jingjie organization: Department of Materials Science and NanoEngineering, Rice University, TX, 77005, Houston, USA – sequence: 3 givenname: Will J. surname: Hardy fullname: Hardy, Will J. organization: Department of Physics and Astronomy, Rice University, TX, 77005, Houston, USA – sequence: 4 givenname: Philip surname: Loya fullname: Loya, Philip organization: Department of Materials Science and NanoEngineering, Rice University, TX, 77005, Houston, USA – sequence: 5 givenname: Minhan surname: Lou fullname: Lou, Minhan organization: Department of Electrical and Computer Engineering, Rice University, TX, 77005, Houston, USA – sequence: 6 givenname: Yingchao surname: Yang fullname: Yang, Yingchao organization: Department of Materials Science and NanoEngineering, Rice University, TX, 77005, Houston, USA – sequence: 7 givenname: Sina surname: Najmaei fullname: Najmaei, Sina organization: Department of Materials Science and NanoEngineering, Rice University, TX, 77005, Houston, USA – sequence: 8 givenname: Menglei surname: Jiang fullname: Jiang, Menglei organization: Department of Materials Science and NanoEngineering, Rice University, TX, 77005, Houston, USA – sequence: 9 givenname: Fan surname: Qin fullname: Qin, Fan organization: Department of Electrical and Computer Engineering, University of Houston, TX, 77204, Houston, USA – sequence: 10 givenname: Kunttal surname: Keyshar fullname: Keyshar, Kunttal organization: Department of Materials Science and NanoEngineering, Rice University, TX, 77005, Houston, USA – sequence: 11 givenname: Heng surname: Ji fullname: Ji, Heng organization: Department of Physics and Astronomy, Rice University, TX, 77005, Houston, USA – sequence: 12 givenname: Weilu surname: Gao fullname: Gao, Weilu organization: Department of Electrical and Computer Engineering, Rice University, TX, 77005, Houston, USA – sequence: 13 givenname: Jiming surname: Bao fullname: Bao, Jiming organization: Department of Electrical and Computer Engineering, University of Houston, 77204, Houston, TX, USA – sequence: 14 givenname: Junichiro surname: Kono fullname: Kono, Junichiro organization: Department of Electrical and Computer Engineering, Rice University, TX, 77005, Houston, USA – sequence: 15 givenname: Douglas surname: Natelson fullname: Natelson, Douglas organization: Department of Physics and Astronomy, Rice University, TX, 77005, Houston, USA – sequence: 16 givenname: Pulickel M. surname: Ajayan fullname: Ajayan, Pulickel M. organization: Department of Materials Science and NanoEngineering, Rice University, TX, 77005, Houston, USA – sequence: 17 givenname: Jun surname: Lou fullname: Lou, Jun email: jlou@rice.edu organization: Department of Materials Science and NanoEngineering, Rice University, TX, 77005, Houston, USA
BackLink	https://www.ncbi.nlm.nih.gov/pubmed/26293810$$D View this record in MEDLINE/PubMed
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Keywords	metals vanadium disulfide hydrogen evolution reactions transition metal dichalcogenides chemical vapor deposition
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Snippet	A facile chemical vapor deposition method to prepare single‐crystalline VS2 nanosheets for the hydrogen evolution reaction is reported. The electrocatalytic... A facile chemical vapor deposition method to prepare single-crystalline VS2 nanosheets for the hydrogen evolution reaction is reported. The electrocatalytic... A facile chemical vapor deposition method to prepare single-crystalline VS sub(2) nanosheets for the hydrogen evolution reaction is reported. The...
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SubjectTerms	Chemical vapor deposition Disulfides Hydrogen evolution hydrogen evolution reactions metals Nanostructure Single crystals Stability Synthesis (chemistry) Tafel slopes transition metal dichalcogenides vanadium disulfide
Title	Facile Synthesis of Single Crystal Vanadium Disulfide Nanosheets by Chemical Vapor Deposition for Efficient Hydrogen Evolution Reaction
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