Scaling of Memories and Crossover in Glassy Magnets
Glassiness is ubiquitous and diverse in characteristics in nature. Understanding their differences and classification remains a major scientific challenge. Here, we show that scaling of magnetic memories with time can be used to classify magnetic glassy materials into two distinct classes. The syste...
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Published in | Scientific reports Vol. 7; no. 1; pp. 12053 - 8 |
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Main Authors | , , , , , , , , , , , , , , |
Format | Journal Article |
Language | English |
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London
Nature Publishing Group UK
21.09.2017
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Abstract | Glassiness is ubiquitous and diverse in characteristics in nature. Understanding their differences and classification remains a major scientific challenge. Here, we show that scaling of magnetic memories with time can be used to classify magnetic glassy materials into two distinct classes. The systems studied are high temperature superconductor-related materials, spin-orbit Mott insulators, frustrated magnets, and dilute magnetic alloys. Our bulk magnetization measurements reveal that most densely populated magnets exhibit similar memory behavior characterized by a relaxation exponent of
1
−
n
≈
0.6
(
1
)
. This exponent is different from
1
−
n
≈
1
/
3
of dilute magnetic alloys that was ascribed to their hierarchical and fractal energy landscape, and is also different from
1
−
n
=
1
of the conventional Debye relaxation expected for a spin solid, a state with long range order. Furthermore, our systematic study on dilute magnetic alloys with varying magnetic concentration exhibits crossovers among the two glassy states and spin solid. |
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AbstractList | Glassiness is ubiquitous and diverse in characteristics in nature. Understanding their differences and classification remains a major scientific challenge. Here, we show that scaling of magnetic memories with time can be used to classify magnetic glassy materials into two distinct classes. The systems studied are high temperature superconductor-related materials, spin-orbit Mott insulators, frustrated magnets, and dilute magnetic alloys. Our bulk magnetization measurements reveal that most densely populated magnets exhibit similar memory behavior characterized by a relaxation exponent of \[1-n\approx 0.6(1)\]. This exponent is different from \[1-{\boldsymbol{n}}\approx 1/3\] of dilute magnetic alloys that was ascribed to their hierarchical and fractal energy landscape, and is also different from \[1-{\boldsymbol{n}}=1\] of the conventional Debye relaxation expected for a spin solid, a state with long range order. Furthermore, our systematic study on dilute magnetic alloys with varying magnetic concentration exhibits crossovers among the two glassy states and spin solid. Glassiness is ubiquitous and diverse in characteristics in nature. Understanding their differences and classification remains a major scientific challenge. Here, we show that scaling of magnetic memories with time can be used to classify magnetic glassy materials into two distinct classes. The systems studied are high temperature superconductor-related materials, spin-orbit Mott insulators, frustrated magnets, and dilute magnetic alloys. Our bulk magnetization measurements reveal that most densely populated magnets exhibit similar memory behavior characterized by a relaxation exponent of [Formula: see text]. This exponent is different from [Formula: see text] of dilute magnetic alloys that was ascribed to their hierarchical and fractal energy landscape, and is also different from [Formula: see text] of the conventional Debye relaxation expected for a spin solid, a state with long range order. Furthermore, our systematic study on dilute magnetic alloys with varying magnetic concentration exhibits crossovers among the two glassy states and spin solid. Glassiness is ubiquitous and diverse in characteristics in nature. Understanding their differences and classification remains a major scientific challenge. Here, we show that scaling of magnetic memories with time can be used to classify magnetic glassy materials into two distinct classes. The systems studied are high temperature superconductor-related materials, spin-orbit Mott insulators, frustrated magnets, and dilute magnetic alloys. Our bulk magnetization measurements reveal that most densely populated magnets exhibit similar memory behavior characterized by a relaxation exponent of 1 − n ≈ 0.6 ( 1 ) . This exponent is different from 1 − n ≈ 1 / 3 of dilute magnetic alloys that was ascribed to their hierarchical and fractal energy landscape, and is also different from 1 − n = 1 of the conventional Debye relaxation expected for a spin solid, a state with long range order. Furthermore, our systematic study on dilute magnetic alloys with varying magnetic concentration exhibits crossovers among the two glassy states and spin solid. Glassiness is ubiquitous and diverse in characteristics in nature. Understanding their differences and classification remains a major scientific challenge. Here, we show that scaling of magnetic memories with time can be used to classify magnetic glassy materials into two distinct classes. The systems studied are high temperature superconductor-related materials, spin-orbit Mott insulators, frustrated magnets, and dilute magnetic alloys. Our bulk magnetization measurements reveal that most densely populated magnets exhibit similar memory behavior characterized by a relaxation exponent of \documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$$1-n\approx 0.6(1)$$\end{document} 1 − n ≈ 0.6 ( 1 ) . This exponent is different from \documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$$1-{\boldsymbol{n}}\approx 1/3$$\end{document} 1 − n ≈ 1 / 3 of dilute magnetic alloys that was ascribed to their hierarchical and fractal energy landscape, and is also different from \documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$$1-{\boldsymbol{n}}=1$$\end{document} 1 − n = 1 of the conventional Debye relaxation expected for a spin solid, a state with long range order. Furthermore, our systematic study on dilute magnetic alloys with varying magnetic concentration exhibits crossovers among the two glassy states and spin solid. Abstract Glassiness is ubiquitous and diverse in characteristics in nature. Understanding their differences and classification remains a major scientific challenge. Here, we show that scaling of magnetic memories with time can be used to classify magnetic glassy materials into two distinct classes. The systems studied are high temperature superconductor-related materials, spin-orbit Mott insulators, frustrated magnets, and dilute magnetic alloys. Our bulk magnetization measurements reveal that most densely populated magnets exhibit similar memory behavior characterized by a relaxation exponent of $$1-n\approx 0.6(1)$$ 1 − n ≈ 0.6 ( 1 ) . This exponent is different from $$1-{\boldsymbol{n}}\approx 1/3$$ 1 − n ≈ 1 / 3 of dilute magnetic alloys that was ascribed to their hierarchical and fractal energy landscape, and is also different from $$1-{\boldsymbol{n}}=1$$ 1 − n = 1 of the conventional Debye relaxation expected for a spin solid, a state with long range order. Furthermore, our systematic study on dilute magnetic alloys with varying magnetic concentration exhibits crossovers among the two glassy states and spin solid. |
ArticleNumber | 12053 |
Author | Lee, S.-H. Yang, J. Samarakoon, A. M. Ehlers, G. Katayama, N. Sato, T. J. Tennant, D. A. Zhang, D. Chern, G-W. Yamada, K. Takahashi, M. Wakimoto, S. Sinclair, R. Zhou, H. D. Diallo, S. O. |
Author_xml | – sequence: 1 givenname: A. M. orcidid: 0000-0001-5361-1815 surname: Samarakoon fullname: Samarakoon, A. M. organization: Department of Physics, University of Virginia, Oak Ridge National Laboratory – sequence: 2 givenname: M. surname: Takahashi fullname: Takahashi, M. organization: Institute of Multidisciplinary Research for Advanced Materials, Tohoku University, Katahira – sequence: 3 givenname: D. surname: Zhang fullname: Zhang, D. organization: Department of Physics, University of Virginia – sequence: 4 givenname: J. surname: Yang fullname: Yang, J. organization: Department of Physics, University of Virginia – sequence: 5 givenname: N. surname: Katayama fullname: Katayama, N. organization: Department of Physics, University of Virginia, Department of Applied Physics, Nagoya University – sequence: 6 givenname: R. surname: Sinclair fullname: Sinclair, R. organization: Department of Physics and Astronomy, University of Tennessee – sequence: 7 givenname: H. D. surname: Zhou fullname: Zhou, H. D. organization: Department of Physics and Astronomy, University of Tennessee – sequence: 8 givenname: S. O. surname: Diallo fullname: Diallo, S. O. organization: Oak Ridge National Laboratory – sequence: 9 givenname: G. orcidid: 0000-0003-3513-508X surname: Ehlers fullname: Ehlers, G. organization: Oak Ridge National Laboratory – sequence: 10 givenname: D. A. orcidid: 0000-0002-9575-3368 surname: Tennant fullname: Tennant, D. A. organization: Oak Ridge National Laboratory – sequence: 11 givenname: S. surname: Wakimoto fullname: Wakimoto, S. organization: Materials Sciences Research Center, Japan Atomic Energy Agency, 2-4 Shirakata Shirane, Tokai, Naka – sequence: 12 givenname: K. surname: Yamada fullname: Yamada, K. organization: Institute of Materials Structure Science, High Energy Accelerator Research Organization, Oho – sequence: 13 givenname: G-W. surname: Chern fullname: Chern, G-W. organization: Department of Physics, University of Virginia – sequence: 14 givenname: T. J. surname: Sato fullname: Sato, T. J. email: taku@tagen.tohoku.ac.jp organization: Institute of Multidisciplinary Research for Advanced Materials, Tohoku University, Katahira – sequence: 15 givenname: S.-H. surname: Lee fullname: Lee, S.-H. email: shlee@virginia.edu organization: Department of Physics, University of Virginia |
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Snippet | Glassiness is ubiquitous and diverse in characteristics in nature. Understanding their differences and classification remains a major scientific challenge.... Abstract Glassiness is ubiquitous and diverse in characteristics in nature. Understanding their differences and classification remains a major scientific... |
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SubjectTerms | 639/301 639/766 Alloys High temperature High temperature superconductors Humanities and Social Sciences Magnetism multidisciplinary Population density Scaling Science Science (multidisciplinary) |
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Title | Scaling of Memories and Crossover in Glassy Magnets |
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