Strong intrinsic room-temperature ferromagnetism in freestanding non-van der Waals ultrathin 2D crystals
Control of ferromagnetism is of critical importance for a variety of proposed spintronic and topological quantum technologies. Inducing long-range ferromagnetic order in ultrathin 2D crystals will provide more functional possibility to combine their unique electronic, optical and mechanical properti...
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| Published in | Nature communications Vol. 12; no. 1; pp. 5688 - 8 |
|---|---|
| Main Authors | , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
28.09.2021
Nature Publishing Group Nature Portfolio |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Control of ferromagnetism is of critical importance for a variety of proposed spintronic and topological quantum technologies. Inducing long-range ferromagnetic order in ultrathin 2D crystals will provide more functional possibility to combine their unique electronic, optical and mechanical properties to develop new multifunctional coupled applications. Recently discovered intrinsic 2D ferromagnetic crystals such as Cr
2
Ge
2
Te
6
, CrI
3
and Fe
3
GeTe
2
are intrinsically ferromagnetic only below room temperature, mostly far below room temperature (Curie temperature, ~20–207 K). Here we develop a scalable method to prepare freestanding non-van der Waals ultrathin 2D crystals down to mono- and few unit cells (UC) and report unexpected strong, intrinsic, ambient-air-robust, room-temperature ferromagnetism with
T
C
up to ~367 K in freestanding non-van der Waals 2D CrTe crystals. Freestanding 2D CrTe crystals show comparable or better ferromagnetic properties to widely-used Fe, Co, Ni and BaFe
12
O
19
, promising as new platforms for room-temperature intrinsically-ferromagnetic 2D crystals and integrated 2D devices.
Van der Waals crystals have recently been shown to exhibit ferromagnetism, however the Curie temperature is typically quite low. Herein, Wu et al succeed in producing mono and few layer crystals of CrTe, a non-van der Waals crystal, and demonstrate strong intrinsic room temperature ferromagnetism. |
|---|---|
| AbstractList | Control of ferromagnetism is of critical importance for a variety of proposed spintronic and topological quantum technologies. Inducing long-range ferromagnetic order in ultrathin 2D crystals will provide more functional possibility to combine their unique electronic, optical and mechanical properties to develop new multifunctional coupled applications. Recently discovered intrinsic 2D ferromagnetic crystals such as Cr
2
Ge
2
Te
6
, CrI
3
and Fe
3
GeTe
2
are intrinsically ferromagnetic only below room temperature, mostly far below room temperature (Curie temperature, ~20–207 K). Here we develop a scalable method to prepare freestanding non-van der Waals ultrathin 2D crystals down to mono- and few unit cells (UC) and report unexpected strong, intrinsic, ambient-air-robust, room-temperature ferromagnetism with
T
C
up to ~367 K in freestanding non-van der Waals 2D CrTe crystals. Freestanding 2D CrTe crystals show comparable or better ferromagnetic properties to widely-used Fe, Co, Ni and BaFe
12
O
19
, promising as new platforms for room-temperature intrinsically-ferromagnetic 2D crystals and integrated 2D devices.
Van der Waals crystals have recently been shown to exhibit ferromagnetism, however the Curie temperature is typically quite low. Herein, Wu et al succeed in producing mono and few layer crystals of CrTe, a non-van der Waals crystal, and demonstrate strong intrinsic room temperature ferromagnetism. Van der Waals crystals have recently been shown to exhibit ferromagnetism, however the Curie temperature is typically quite low. Herein, Wu et al succeed in producing mono and few layer crystals of CrTe, a non-van der Waals crystal, and demonstrate strong intrinsic room temperature ferromagnetism. Control of ferromagnetism is of critical importance for a variety of proposed spintronic and topological quantum technologies. Inducing long-range ferromagnetic order in ultrathin 2D crystals will provide more functional possibility to combine their unique electronic, optical and mechanical properties to develop new multifunctional coupled applications. Recently discovered intrinsic 2D ferromagnetic crystals such as Cr 2 Ge 2 Te 6 , CrI 3 and Fe 3 GeTe 2 are intrinsically ferromagnetic only below room temperature, mostly far below room temperature (Curie temperature, ~20–207 K). Here we develop a scalable method to prepare freestanding non-van der Waals ultrathin 2D crystals down to mono- and few unit cells (UC) and report unexpected strong, intrinsic, ambient-air-robust, room-temperature ferromagnetism with T C up to ~367 K in freestanding non-van der Waals 2D CrTe crystals. Freestanding 2D CrTe crystals show comparable or better ferromagnetic properties to widely-used Fe, Co, Ni and BaFe 12 O 19 , promising as new platforms for room-temperature intrinsically-ferromagnetic 2D crystals and integrated 2D devices. Control of ferromagnetism is of critical importance for a variety of proposed spintronic and topological quantum technologies. Inducing long-range ferromagnetic order in ultrathin 2D crystals will provide more functional possibility to combine their unique electronic, optical and mechanical properties to develop new multifunctional coupled applications. Recently discovered intrinsic 2D ferromagnetic crystals such as Cr2Ge2Te6, CrI3 and Fe3GeTe2 are intrinsically ferromagnetic only below room temperature, mostly far below room temperature (Curie temperature, ~20–207 K). Here we develop a scalable method to prepare freestanding non-van der Waals ultrathin 2D crystals down to mono- and few unit cells (UC) and report unexpected strong, intrinsic, ambient-air-robust, room-temperature ferromagnetism with TC up to ~367 K in freestanding non-van der Waals 2D CrTe crystals. Freestanding 2D CrTe crystals show comparable or better ferromagnetic properties to widely-used Fe, Co, Ni and BaFe12O19, promising as new platforms for room-temperature intrinsically-ferromagnetic 2D crystals and integrated 2D devices.Van der Waals crystals have recently been shown to exhibit ferromagnetism, however the Curie temperature is typically quite low. Herein, Wu et al succeed in producing mono and few layer crystals of CrTe, a non-van der Waals crystal, and demonstrate strong intrinsic room temperature ferromagnetism. Control of ferromagnetism is of critical importance for a variety of proposed spintronic and topological quantum technologies. Inducing long-range ferromagnetic order in ultrathin 2D crystals will provide more functional possibility to combine their unique electronic, optical and mechanical properties to develop new multifunctional coupled applications. Recently discovered intrinsic 2D ferromagnetic crystals such as Cr2Ge2Te6, CrI3 and Fe3GeTe2 are intrinsically ferromagnetic only below room temperature, mostly far below room temperature (Curie temperature, ~20-207 K). Here we develop a scalable method to prepare freestanding non-van der Waals ultrathin 2D crystals down to mono- and few unit cells (UC) and report unexpected strong, intrinsic, ambient-air-robust, room-temperature ferromagnetism with TC up to ~367 K in freestanding non-van der Waals 2D CrTe crystals. Freestanding 2D CrTe crystals show comparable or better ferromagnetic properties to widely-used Fe, Co, Ni and BaFe12O19, promising as new platforms for room-temperature intrinsically-ferromagnetic 2D crystals and integrated 2D devices.Control of ferromagnetism is of critical importance for a variety of proposed spintronic and topological quantum technologies. Inducing long-range ferromagnetic order in ultrathin 2D crystals will provide more functional possibility to combine their unique electronic, optical and mechanical properties to develop new multifunctional coupled applications. Recently discovered intrinsic 2D ferromagnetic crystals such as Cr2Ge2Te6, CrI3 and Fe3GeTe2 are intrinsically ferromagnetic only below room temperature, mostly far below room temperature (Curie temperature, ~20-207 K). Here we develop a scalable method to prepare freestanding non-van der Waals ultrathin 2D crystals down to mono- and few unit cells (UC) and report unexpected strong, intrinsic, ambient-air-robust, room-temperature ferromagnetism with TC up to ~367 K in freestanding non-van der Waals 2D CrTe crystals. Freestanding 2D CrTe crystals show comparable or better ferromagnetic properties to widely-used Fe, Co, Ni and BaFe12O19, promising as new platforms for room-temperature intrinsically-ferromagnetic 2D crystals and integrated 2D devices. |
| ArticleNumber | 5688 |
| Author | Li, Luying Zhang, Liang Chang, Haixin Wu, Hao Li, Jie Yang, Li Gao, Yihua Du, Juan Zhang, Wenfeng Wang, Jun Shu, Haibo |
| Author_xml | – sequence: 1 givenname: Hao surname: Wu fullname: Wu, Hao organization: Center for Joining and Electronic Packaging, State Key Laboratory of Material Processing and Die & Mold Technology, School of Materials Science and Engineering, Huazhong University of Science and Technology (HUST) – sequence: 2 givenname: Wenfeng surname: Zhang fullname: Zhang, Wenfeng organization: Center for Joining and Electronic Packaging, State Key Laboratory of Material Processing and Die & Mold Technology, School of Materials Science and Engineering, Huazhong University of Science and Technology (HUST) – sequence: 3 givenname: Li surname: Yang fullname: Yang, Li organization: Center for Joining and Electronic Packaging, State Key Laboratory of Material Processing and Die & Mold Technology, School of Materials Science and Engineering, Huazhong University of Science and Technology (HUST) – sequence: 4 givenname: Jun surname: Wang fullname: Wang, Jun organization: College of Optical and Electronic Technology, China Jiliang University – sequence: 5 givenname: Jie surname: Li fullname: Li, Jie organization: Center for Joining and Electronic Packaging, State Key Laboratory of Material Processing and Die & Mold Technology, School of Materials Science and Engineering, Huazhong University of Science and Technology (HUST) – sequence: 6 givenname: Luying surname: Li fullname: Li, Luying organization: Center for Nanoscale Characterization and Devices, Wuhan National Laboratory for Optoelectronics, Huazhong University of Science and Technology – sequence: 7 givenname: Yihua orcidid: 0000-0003-1905-9531 surname: Gao fullname: Gao, Yihua organization: Center for Nanoscale Characterization and Devices, Wuhan National Laboratory for Optoelectronics, Huazhong University of Science and Technology, School of Physics, Huazhong University of Science and Technology – sequence: 8 givenname: Liang surname: Zhang fullname: Zhang, Liang organization: School of Science and Center for Materials Science and Engineering, School of Microelectronics and Materials Engineering, Guangxi University of Science and Technology – sequence: 9 givenname: Juan surname: Du fullname: Du, Juan organization: Ningbo Institute of Material Technology & Engineering, Chinese Academy of Sciences, Institute of Materials, Shanghai University – sequence: 10 givenname: Haibo surname: Shu fullname: Shu, Haibo organization: College of Optical and Electronic Technology, China Jiliang University – sequence: 11 givenname: Haixin orcidid: 0000-0001-9621-4457 surname: Chang fullname: Chang, Haixin email: hxchang@hust.edu.cn organization: Center for Joining and Electronic Packaging, State Key Laboratory of Material Processing and Die & Mold Technology, School of Materials Science and Engineering, Huazhong University of Science and Technology (HUST), School of Science and Center for Materials Science and Engineering, School of Microelectronics and Materials Engineering, Guangxi University of Science and Technology, Institute for Quantum Science and Engineering, Huazhong University of Science and Technology |
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| Copyright | The Author(s) 2021 The Author(s) 2021. This work is published under http://creativecommons.org/licenses/by/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License. 2021. The Author(s). |
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| DOI | 10.1038/s41467-021-26009-0 |
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| Snippet | Control of ferromagnetism is of critical importance for a variety of proposed spintronic and topological quantum technologies. Inducing long-range... Van der Waals crystals have recently been shown to exhibit ferromagnetism, however the Curie temperature is typically quite low. Herein, Wu et al succeed in... |
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| SubjectTerms | 639/301 639/925 Air temperature Barium hexaferrite Crystals Curie temperature Ferromagnetism Humanities and Social Sciences Magnetism Mechanical properties multidisciplinary Nickel Optical properties Room temperature Science Science (multidisciplinary) |
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| Title | Strong intrinsic room-temperature ferromagnetism in freestanding non-van der Waals ultrathin 2D crystals |
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