Spectroscopy of light-molecule endofullerenes

Molecular endofullerenes are supramolecular systems consisting of fullerene cages encapsulating small molecules. Although most early examples consist of encapsulated metal clusters, recently developed synthetic routes have provided endofullerenes with non-metallic guest molecules in high purity and...

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Published inPhilosophical transactions of the Royal Society of London. Series A: Mathematical, physical, and engineering sciences Vol. 371; no. 1998; p. 20120429
Main Author Levitt, Malcolm H.
Format Journal Article
LanguageEnglish
Published England The Royal Society Publishing 13.09.2013
Subjects
Endofullerenes
Infrared Spectroscopy
Neutron Scattering
Nuclear Magnetic Resonance
Parahydrogen
Spin Isomers
neutron scattering
endofullerenes
spin isomers
nuclear magnetic resonance
parahydrogen
infrared spectroscopy
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Abstract Molecular endofullerenes are supramolecular systems consisting of fullerene cages encapsulating small molecules. Although most early examples consist of encapsulated metal clusters, recently developed synthetic routes have provided endofullerenes with non-metallic guest molecules in high purity and macroscopic quantities. The encapsulated light molecule behaves as a confined quantum rotor, displaying rotational quantization as well as translational quantization, and a rich coupling between the translational and rotational degrees of freedom. Furthermore, many encapsulated molecules display spin isomerism. Spectroscopies such as inelastic neutron scattering, nuclear magnetic resonance and infrared spectroscopy may be used to obtain information on the quantized energy level structure and spin isomerism of the guest molecules. It is also possible to study the influence of the guest molecules on the cages, and to explore the communication between the guest molecules and the molecular environment outside the cage.
AbstractList Molecular endofullerenes are supramolecular systems consisting of fullerene cages encapsulating small molecules. Although most early examples consist of encapsulated metal clusters, recently developed synthetic routes have provided endofullerenes with non-metallic guest molecules in high purity and macroscopic quantities. The encapsulated light molecule behaves as a confined quantum rotor, displaying rotational quantization as well as translational quantization, and a rich coupling between the translational and rotational degrees of freedom. Furthermore, many encapsulated molecules display spin isomerism. Spectroscopies such as inelastic neutron scattering, nuclear magnetic resonance and infrared spectroscopy may be used to obtain information on the quantized energy level structure and spin isomerism of the guest molecules. It is also possible to study the influence of the guest molecules on the cages, and to explore the communication between the guest molecules and the molecular environment outside the cage.
Author Levitt, Malcolm H.
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Issue 1998
Keywords neutron scattering
endofullerenes
spin isomers
nuclear magnetic resonance
parahydrogen
infrared spectroscopy
Language English
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One contribution of 13 to a Theo Murphy Meeting Issue Nanolaboratories: physics and chemistry of small-molecule endofullerenes.
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Theo Murphy Meeting Issue 'Nanolaboratories: physics and chemistry of small-molecule endofullerenes' organized and edited by Malcolm H. Levitt and Anthony J. Horsewill
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Snippet Molecular endofullerenes are supramolecular systems consisting of fullerene cages encapsulating small molecules. Although most early examples consist of...
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SubjectTerms Endofullerenes
Infrared Spectroscopy
Neutron Scattering
Nuclear Magnetic Resonance
Parahydrogen
Spin Isomers
Title Spectroscopy of light-molecule endofullerenes
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https://royalsocietypublishing.org/doi/full/10.1098/rsta.2012.0429
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Volume 371
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