Metal 3D printing technology for functional integration of catalytic system
Mechanical properties and geometries of printed products have been extensively studied in metal 3D printing. However, chemical properties and catalytic functions, introduced by metal 3D printing itself, are rarely mentioned. Here we show that metal 3D printing products themselves can simultaneously...
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| Published in | Nature communications Vol. 11; no. 1; p. 4098 |
|---|---|
| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
14.08.2020
Nature Publishing Group Nature Portfolio |
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| Abstract | Mechanical properties and geometries of printed products have been extensively studied in metal 3D printing. However, chemical properties and catalytic functions, introduced by metal 3D printing itself, are rarely mentioned. Here we show that metal 3D printing products themselves can simultaneously serve as chemical reactors and catalysts (denoted as self-catalytic reactor or SCR) for direct conversion of C1 molecules (including CO, CO
2
and CH
4
) into high value-added chemicals. The Fe-SCR and Co-SCR successfully catalyze synthesis of liquid fuel from Fischer-Tropsch synthesis and CO
2
hydrogenation; the Ni-SCR efficiently produces syngas (CO/H
2
) by CO
2
reforming of CH
4
. Further, the Co-SCR geometrical studies indicate that metal 3D printing itself can establish multiple control functions to tune the catalytic product distribution. The present work provides a simple and low-cost manufacturing method to realize functional integration of catalyst and reactor, and will facilitate the developments of chemical synthesis and 3D printing technology.
Metal 3D printing is a very promising technology to revolutionize catalytic systems. Here the authors show that metal 3D printing products themselves can simultaneously serve as chemical reactors and catalysts for conversion of C1 molecules into high value-added chemicals. |
|---|---|
| AbstractList | Mechanical properties and geometries of printed products have been extensively studied in metal 3D printing. However, chemical properties and catalytic functions, introduced by metal 3D printing itself, are rarely mentioned. Here we show that metal 3D printing products themselves can simultaneously serve as chemical reactors and catalysts (denoted as self-catalytic reactor or SCR) for direct conversion of C1 molecules (including CO, CO
2
and CH
4
) into high value-added chemicals. The Fe-SCR and Co-SCR successfully catalyze synthesis of liquid fuel from Fischer-Tropsch synthesis and CO
2
hydrogenation; the Ni-SCR efficiently produces syngas (CO/H
2
) by CO
2
reforming of CH
4
. Further, the Co-SCR geometrical studies indicate that metal 3D printing itself can establish multiple control functions to tune the catalytic product distribution. The present work provides a simple and low-cost manufacturing method to realize functional integration of catalyst and reactor, and will facilitate the developments of chemical synthesis and 3D printing technology. Metal 3D printing is a very promising technology to revolutionize catalytic systems. Here the authors show that metal 3D printing products themselves can simultaneously serve as chemical reactors and catalysts for conversion of C1 molecules into high value-added chemicals. Mechanical properties and geometries of printed products have been extensively studied in metal 3D printing. However, chemical properties and catalytic functions, introduced by metal 3D printing itself, are rarely mentioned. Here we show that metal 3D printing products themselves can simultaneously serve as chemical reactors and catalysts (denoted as self-catalytic reactor or SCR) for direct conversion of C1 molecules (including CO, CO 2 and CH 4 ) into high value-added chemicals. The Fe-SCR and Co-SCR successfully catalyze synthesis of liquid fuel from Fischer-Tropsch synthesis and CO 2 hydrogenation; the Ni-SCR efficiently produces syngas (CO/H 2 ) by CO 2 reforming of CH 4 . Further, the Co-SCR geometrical studies indicate that metal 3D printing itself can establish multiple control functions to tune the catalytic product distribution. The present work provides a simple and low-cost manufacturing method to realize functional integration of catalyst and reactor, and will facilitate the developments of chemical synthesis and 3D printing technology. Metal 3D printing is a very promising technology to revolutionize catalytic systems. Here the authors show that metal 3D printing products themselves can simultaneously serve as chemical reactors and catalysts for conversion of C1 molecules into high value-added chemicals. Mechanical properties and geometries of printed products have been extensively studied in metal 3D printing. However, chemical properties and catalytic functions, introduced by metal 3D printing itself, are rarely mentioned. Here we show that metal 3D printing products themselves can simultaneously serve as chemical reactors and catalysts (denoted as self-catalytic reactor or SCR) for direct conversion of C1 molecules (including CO, CO2 and CH4) into high value-added chemicals. The Fe-SCR and Co-SCR successfully catalyze synthesis of liquid fuel from Fischer-Tropsch synthesis and CO2 hydrogenation; the Ni-SCR efficiently produces syngas (CO/H2) by CO2 reforming of CH4. Further, the Co-SCR geometrical studies indicate that metal 3D printing itself can establish multiple control functions to tune the catalytic product distribution. The present work provides a simple and low-cost manufacturing method to realize functional integration of catalyst and reactor, and will facilitate the developments of chemical synthesis and 3D printing technology.Metal 3D printing is a very promising technology to revolutionize catalytic systems. Here the authors show that metal 3D printing products themselves can simultaneously serve as chemical reactors and catalysts for conversion of C1 molecules into high value-added chemicals. |
| ArticleNumber | 4098 |
| Author | Wang, Yang Wei, Qinhong Li, Hangjie Tan, Yen Ee He, Yingluo Tsubaki, Noritatsu Yang, Guohui Wang, Ding Peng, Xiaobo Liu, Guoguo |
| Author_xml | – sequence: 1 givenname: Qinhong surname: Wei fullname: Wei, Qinhong organization: Department of Applied Chemistry, School of Engineering, University of Toyama, Department of Chemical Engineering, School of Petrochemical Technology and Energy Engineering, Zhejiang Ocean University – sequence: 2 givenname: Hangjie surname: Li fullname: Li, Hangjie organization: Department of Applied Chemistry, School of Engineering, University of Toyama – sequence: 3 givenname: Guoguo surname: Liu fullname: Liu, Guoguo organization: Department of Applied Chemistry, School of Engineering, University of Toyama – sequence: 4 givenname: Yingluo surname: He fullname: He, Yingluo organization: Department of Applied Chemistry, School of Engineering, University of Toyama – sequence: 5 givenname: Yang surname: Wang fullname: Wang, Yang organization: Department of Applied Chemistry, School of Engineering, University of Toyama – sequence: 6 givenname: Yen Ee surname: Tan fullname: Tan, Yen Ee organization: Department of Applied Chemistry, School of Engineering, University of Toyama – sequence: 7 givenname: Ding surname: Wang fullname: Wang, Ding organization: School of Material Science & Engineering, University of Shanghai for Science and Technology – sequence: 8 givenname: Xiaobo orcidid: 0000-0002-4437-1546 surname: Peng fullname: Peng, Xiaobo email: PENG.Xiaobo@nims.go.jp organization: National Institute for Materials Science, Key Laboratory of the Ministry of Education for Advanced Catalysis Materials, Institute of Physical Chemistry, Zhejiang Normal University – sequence: 9 givenname: Guohui orcidid: 0000-0001-9799-0984 surname: Yang fullname: Yang, Guohui email: thomas@eng.u-toyama.ac.jp organization: Department of Applied Chemistry, School of Engineering, University of Toyama, State Key Laboratory of Coal Conversion, Institute of Coal Chemistry, Chinese Academy of Sciences – sequence: 10 givenname: Noritatsu orcidid: 0000-0001-6786-5058 surname: Tsubaki fullname: Tsubaki, Noritatsu email: tsubaki@eng.u-toyama.ac.jp organization: Department of Applied Chemistry, School of Engineering, University of Toyama |
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| Snippet | Mechanical properties and geometries of printed products have been extensively studied in metal 3D printing. However, chemical properties and catalytic... Metal 3D printing is a very promising technology to revolutionize catalytic systems. Here the authors show that metal 3D printing products themselves can... |
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| StartPage | 4098 |
| SubjectTerms | 3-D printers 639/301/930/1032 639/638/675 639/638/77/887 639/638/898 Carbon dioxide Catalysts Catalytic converters Chemical properties Chemical reactors Chemicals Direct conversion Fischer-Tropsch process Functional integration Humanities and Social Sciences Integration Liquid fuels Mechanical properties Metals Methane multidisciplinary Nuclear fuels Printing Production methods Reactors Reforming Science Science (multidisciplinary) Selective catalytic reduction Synthesis gas Technology Three dimensional printing |
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| Title | Metal 3D printing technology for functional integration of catalytic system |
| URI | https://link.springer.com/article/10.1038/s41467-020-17941-8 https://www.proquest.com/docview/2434146934 https://search.proquest.com/docview/2434476478 https://pubmed.ncbi.nlm.nih.gov/PMC7428005 https://doaj.org/article/488efdfc9a634a8395f1457a89cef02b |
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