Hydrogenated Cs2AgBiBr6 for significantly improved efficiency of lead-free inorganic double perovskite solar cell

Development of lead-free inorganic perovskite material, such as Cs 2 AgBiBr 6 , is of great importance to solve the toxicity and stability issues of traditional lead halide perovskite solar cells. However, due to a wide bandgap of Cs 2 AgBiBr 6 film, its light absorption ability is largely limited a...

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Published inNature communications Vol. 13; no. 1; pp. 3397 - 12
Main Authors Zhang, Zeyu, Sun, Qingde, Lu, Yue, Lu, Feng, Mu, Xulin, Wei, Su-Huai, Sui, Manling
Format Journal Article
LanguageEnglish
Published London Nature Publishing Group UK 13.06.2022
Nature Publishing Group
Nature Portfolio
Subjects
140/146
147/135
147/143
639/301/299/946
639/4077/909/4101/4096/946
Carrier lifetime
Carrier mobility
Conduction bands
Efficiency
Electromagnetic absorption
Energy conversion efficiency
Energy gap
Energy levels
Humanities and Social Sciences
Hydrogenation
Lead compounds
Lead free
Metal halides
multidisciplinary
Perovskites
Photoelectricity
Photovoltaic cells
Science
Science (multidisciplinary)
Solar cells
Stability
Toxicity
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Abstract Development of lead-free inorganic perovskite material, such as Cs 2 AgBiBr 6 , is of great importance to solve the toxicity and stability issues of traditional lead halide perovskite solar cells. However, due to a wide bandgap of Cs 2 AgBiBr 6 film, its light absorption ability is largely limited and the photoelectronic conversion efficiency is normally lower than 4.23%. In this text, by using a hydrogenation method, the bandgap of Cs 2 AgBiBr 6 films could be tunable from 2.18 eV to 1.64 eV. At the same time, the highest photoelectric conversion efficiency of hydrogenated Cs 2 AgBiBr 6 perovskite solar cell has been improved up to 6.37% with good environmental stability. Further investigations confirmed that the interstitial doping of atomic hydrogen in Cs 2 AgBiBr 6 lattice could not only adjust its valence and conduction band energy levels, but also optimize the carrier mobility and carrier lifetime. All these works provide an insightful strategy to fabricate high performance lead-free inorganic perovskite solar cells. Though inorganic perovskites are an attractive, non-toxic and stable alternative to organic-inorganic halide perovskite solar cells, realizing efficient devices remains a challenge. Here, the authors report hydrogenated lead-free inorganic perovskite solar cells with enhanced power conversion efficiency.
AbstractList Development of lead-free inorganic perovskite material, such as Cs2AgBiBr6, is of great importance to solve the toxicity and stability issues of traditional lead halide perovskite solar cells. However, due to a wide bandgap of Cs2AgBiBr6 film, its light absorption ability is largely limited and the photoelectronic conversion efficiency is normally lower than 4.23%. In this text, by using a hydrogenation method, the bandgap of Cs2AgBiBr6 films could be tunable from 2.18 eV to 1.64 eV. At the same time, the highest photoelectric conversion efficiency of hydrogenated Cs2AgBiBr6 perovskite solar cell has been improved up to 6.37% with good environmental stability. Further investigations confirmed that the interstitial doping of atomic hydrogen in Cs2AgBiBr6 lattice could not only adjust its valence and conduction band energy levels, but also optimize the carrier mobility and carrier lifetime. All these works provide an insightful strategy to fabricate high performance lead-free inorganic perovskite solar cells.Development of lead-free inorganic perovskite material, such as Cs2AgBiBr6, is of great importance to solve the toxicity and stability issues of traditional lead halide perovskite solar cells. However, due to a wide bandgap of Cs2AgBiBr6 film, its light absorption ability is largely limited and the photoelectronic conversion efficiency is normally lower than 4.23%. In this text, by using a hydrogenation method, the bandgap of Cs2AgBiBr6 films could be tunable from 2.18 eV to 1.64 eV. At the same time, the highest photoelectric conversion efficiency of hydrogenated Cs2AgBiBr6 perovskite solar cell has been improved up to 6.37% with good environmental stability. Further investigations confirmed that the interstitial doping of atomic hydrogen in Cs2AgBiBr6 lattice could not only adjust its valence and conduction band energy levels, but also optimize the carrier mobility and carrier lifetime. All these works provide an insightful strategy to fabricate high performance lead-free inorganic perovskite solar cells.
Development of lead-free inorganic perovskite material, such as Cs 2 AgBiBr 6 , is of great importance to solve the toxicity and stability issues of traditional lead halide perovskite solar cells. However, due to a wide bandgap of Cs 2 AgBiBr 6 film, its light absorption ability is largely limited and the photoelectronic conversion efficiency is normally lower than 4.23%. In this text, by using a hydrogenation method, the bandgap of Cs 2 AgBiBr 6 films could be tunable from 2.18 eV to 1.64 eV. At the same time, the highest photoelectric conversion efficiency of hydrogenated Cs 2 AgBiBr 6 perovskite solar cell has been improved up to 6.37% with good environmental stability. Further investigations confirmed that the interstitial doping of atomic hydrogen in Cs 2 AgBiBr 6 lattice could not only adjust its valence and conduction band energy levels, but also optimize the carrier mobility and carrier lifetime. All these works provide an insightful strategy to fabricate high performance lead-free inorganic perovskite solar cells. Though inorganic perovskites are an attractive, non-toxic and stable alternative to organic-inorganic halide perovskite solar cells, realizing efficient devices remains a challenge. Here, the authors report hydrogenated lead-free inorganic perovskite solar cells with enhanced power conversion efficiency.
Though inorganic perovskites are an attractive, non-toxic and stable alternative to organic-inorganic halide perovskite solar cells, realizing efficient devices remains a challenge. Here, the authors report hydrogenated lead-free inorganic perovskite solar cells with enhanced power conversion efficiency.
Development of lead-free inorganic perovskite material, such as Cs 2 AgBiBr 6 , is of great importance to solve the toxicity and stability issues of traditional lead halide perovskite solar cells. However, due to a wide bandgap of Cs 2 AgBiBr 6 film, its light absorption ability is largely limited and the photoelectronic conversion efficiency is normally lower than 4.23%. In this text, by using a hydrogenation method, the bandgap of Cs 2 AgBiBr 6 films could be tunable from 2.18 eV to 1.64 eV. At the same time, the highest photoelectric conversion efficiency of hydrogenated Cs 2 AgBiBr 6 perovskite solar cell has been improved up to 6.37% with good environmental stability. Further investigations confirmed that the interstitial doping of atomic hydrogen in Cs 2 AgBiBr 6 lattice could not only adjust its valence and conduction band energy levels, but also optimize the carrier mobility and carrier lifetime. All these works provide an insightful strategy to fabricate high performance lead-free inorganic perovskite solar cells.
Development of lead-free inorganic perovskite material, such as Cs2AgBiBr6, is of great importance to solve the toxicity and stability issues of traditional lead halide perovskite solar cells. However, due to a wide bandgap of Cs2AgBiBr6 film, its light absorption ability is largely limited and the photoelectronic conversion efficiency is normally lower than 4.23%. In this text, by using a hydrogenation method, the bandgap of Cs2AgBiBr6 films could be tunable from 2.18 eV to 1.64 eV. At the same time, the highest photoelectric conversion efficiency of hydrogenated Cs2AgBiBr6 perovskite solar cell has been improved up to 6.37% with good environmental stability. Further investigations confirmed that the interstitial doping of atomic hydrogen in Cs2AgBiBr6 lattice could not only adjust its valence and conduction band energy levels, but also optimize the carrier mobility and carrier lifetime. All these works provide an insightful strategy to fabricate high performance lead-free inorganic perovskite solar cells.Though inorganic perovskites are an attractive, non-toxic and stable alternative to organic-inorganic halide perovskite solar cells, realizing efficient devices remains a challenge. Here, the authors report hydrogenated lead-free inorganic perovskite solar cells with enhanced power conversion efficiency.
ArticleNumber 3397
Author Lu, Yue
Mu, Xulin
Zhang, Zeyu
Sui, Manling
Wei, Su-Huai
Lu, Feng
Sun, Qingde
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  organization: Beijing Key Laboratory of Microstructure and Properties of Solids, Faculty of Materials and Manufacturing, Beijing University of Technology
– sequence: 2
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  surname: Sun
  fullname: Sun, Qingde
  organization: Beijing Computational Science Research Center
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  givenname: Yue
  orcidid: 0000-0001-9800-3792
  surname: Lu
  fullname: Lu, Yue
  email: luyue@bjut.edu.cn
  organization: Beijing Key Laboratory of Microstructure and Properties of Solids, Faculty of Materials and Manufacturing, Beijing University of Technology
– sequence: 4
  givenname: Feng
  surname: Lu
  fullname: Lu, Feng
  organization: Department of Electronic Science and Engineering, and Tianjin Key Laboratory of Photo-Electronic Thin Film Device and Technology, Nankai University
– sequence: 5
  givenname: Xulin
  surname: Mu
  fullname: Mu, Xulin
  organization: Beijing Key Laboratory of Microstructure and Properties of Solids, Faculty of Materials and Manufacturing, Beijing University of Technology
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  givenname: Su-Huai
  orcidid: 0000-0003-1563-4738
  surname: Wei
  fullname: Wei, Su-Huai
  email: suhuaiwei@csrc.ac.cn
  organization: Beijing Computational Science Research Center
– sequence: 7
  givenname: Manling
  orcidid: 0000-0002-0415-5881
  surname: Sui
  fullname: Sui, Manling
  email: mlsui@bjut.edu.cn
  organization: Beijing Key Laboratory of Microstructure and Properties of Solids, Faculty of Materials and Manufacturing, Beijing University of Technology
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Snippet Development of lead-free inorganic perovskite material, such as Cs 2 AgBiBr 6 , is of great importance to solve the toxicity and stability issues of...
Development of lead-free inorganic perovskite material, such as Cs2AgBiBr6, is of great importance to solve the toxicity and stability issues of traditional...
Though inorganic perovskites are an attractive, non-toxic and stable alternative to organic-inorganic halide perovskite solar cells, realizing efficient...
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639/4077/909/4101/4096/946
Carrier lifetime
Carrier mobility
Conduction bands
Efficiency
Electromagnetic absorption
Energy conversion efficiency
Energy gap
Energy levels
Humanities and Social Sciences
Hydrogenation
Lead compounds
Lead free
Metal halides
multidisciplinary
Perovskites
Photoelectricity
Photovoltaic cells
Science
Science (multidisciplinary)
Solar cells
Stability
Toxicity
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Title Hydrogenated Cs2AgBiBr6 for significantly improved efficiency of lead-free inorganic double perovskite solar cell
URI https://link.springer.com/article/10.1038/s41467-022-31016-w
https://www.proquest.com/docview/2675830336
https://www.proquest.com/docview/2676553340
https://pubmed.ncbi.nlm.nih.gov/PMC9192601
https://doaj.org/article/31040615be224672b42468b1b6563a4e
Volume 13
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