Highly Flexible, Tough, and Self-Healing Supramolecular Polymeric Materials Using Host-Guest Interaction

Flexible, tough, and self‐healable polymeric materials are promising to be a solution to the energy problem by substituting for conventional heavy materials. A fusion of supramolecular chemistry and polymer chemistry is a powerful method to create such intelligent materials. Here, a supramolecular p...

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Published in	Macromolecular rapid communications. Vol. 37; no. 1; pp. 86 - 92
Main Authors	Nakahata, Masaki, Takashima, Yoshinori, Harada, Akira
Format	Journal Article
Language	English
Published	Germany Blackwell Publishing Ltd 01.01.2016 Wiley Subscription Services, Inc
Subjects	Chains (polymeric) Cyclodextrins Drying host-guest interactions Hydrogels Polymer chemistry Polymers Recognition reversible bond formation scratch-curable coatings self-healing Smart materials tough polymers Utilities tough polymers scratch-curable coatings self-healing reversible bond formation host-guest interactions
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Abstract	Flexible, tough, and self‐healable polymeric materials are promising to be a solution to the energy problem by substituting for conventional heavy materials. A fusion of supramolecular chemistry and polymer chemistry is a powerful method to create such intelligent materials. Here, a supramolecular polymeric material using multipoint molecular recognition between cyclodextrin (CD) and hydrophobic guest molecules at polymer side chain is reported. A transparent, flexible, and tough hydrogel (host–guest gel) is formed by a simple preparation procedure. The host–guest gel shows self‐healing property in both wet state and dry state due to reversible nature of host–guest interaction. The practical utility of the host–guest gel as a scratch curable coating is demonstrated. Flexible, tough, and self‐healable polymeric materials are promising to be a substitute for conventional heavy materials. Here, a supramolecular polymeric material using multipoint host–guest interaction between cyclodextrin (CD) and hydrophobic guest molecules at polymer side chain is reported. The obtained host–guest gel shows a self‐healing property in both wet and dry states due to the reversible nature of the host–guest interaction.
AbstractList	Flexible, tough, and self‐healable polymeric materials are promising to be a solution to the energy problem by substituting for conventional heavy materials. A fusion of supramolecular chemistry and polymer chemistry is a powerful method to create such intelligent materials. Here, a supramolecular polymeric material using multipoint molecular recognition between cyclodextrin (CD) and hydrophobic guest molecules at polymer side chain is reported. A transparent, flexible, and tough hydrogel (host–guest gel) is formed by a simple preparation procedure. The host–guest gel shows self‐healing property in both wet state and dry state due to reversible nature of host–guest interaction. The practical utility of the host–guest gel as a scratch curable coating is demonstrated. Flexible, tough, and self‐healable polymeric materials are promising to be a substitute for conventional heavy materials. Here, a supramolecular polymeric material using multipoint host–guest interaction between cyclodextrin (CD) and hydrophobic guest molecules at polymer side chain is reported. The obtained host–guest gel shows a self‐healing property in both wet and dry states due to the reversible nature of the host–guest interaction. Flexible, tough, and self-healable polymeric materials are promising to be a solution to the energy problem by substituting for conventional heavy materials. A fusion of supramolecular chemistry and polymer chemistry is a powerful method to create such intelligent materials. Here, a supramolecular polymeric material using multipoint molecular recognition between cyclodextrin (CD) and hydrophobic guest molecules at polymer side chain is reported. A transparent, flexible, and tough hydrogel (host-guest gel) is formed by a simple preparation procedure. The host-guest gel shows self-healing property in both wet state and dry state due to reversible nature of host-guest interaction. The practical utility of the host-guest gel as a scratch curable coating is demonstrated. Flexible, tough, and self-healable polymeric materials are promising to be a substitute for conventional heavy materials. Here, a supramolecular polymeric material using multipoint host-guest interaction between cyclodextrin (CD) and hydrophobic guest molecules at polymer side chain is reported. The obtained host-guest gel shows a self-healing property in both wet and dry states due to the reversible nature of the host-guest interaction. Flexible, tough, and self-healable polymeric materials are promising to be a solution to the energy problem by substituting for conventional heavy materials. A fusion of supramolecular chemistry and polymer chemistry is a powerful method to create such intelligent materials. Here, a supramolecular polymeric material using multipoint molecular recognition between cyclodextrin (CD) and hydrophobic guest molecules at polymer side chain is reported. A transparent, flexible, and tough hydrogel (host-guest gel) is formed by a simple preparation procedure. The host-guest gel shows self-healing property in both wet state and dry state due to reversible nature of host-guest interaction. The practical utility of the host-guest gel as a scratch curable coating is demonstrated.Flexible, tough, and self-healable polymeric materials are promising to be a solution to the energy problem by substituting for conventional heavy materials. A fusion of supramolecular chemistry and polymer chemistry is a powerful method to create such intelligent materials. Here, a supramolecular polymeric material using multipoint molecular recognition between cyclodextrin (CD) and hydrophobic guest molecules at polymer side chain is reported. A transparent, flexible, and tough hydrogel (host-guest gel) is formed by a simple preparation procedure. The host-guest gel shows self-healing property in both wet state and dry state due to reversible nature of host-guest interaction. The practical utility of the host-guest gel as a scratch curable coating is demonstrated. Flexible, tough, and self-healable polymeric materials are promising to be a solution to the energy problem by substituting for conventional heavy materials. A fusion of supramolecular chemistry and polymer chemistry is a powerful method to create such intelligent materials. Here, a supramolecular polymeric material using multipoint molecular recognition between cyclodextrin (CD) and hydrophobic guest molecules at polymer side chain is reported. A transparent, flexible, and tough hydrogel (host-guest gel) is formed by a simple preparation procedure. The host-guest gel shows self-healing property in both wet state and dry state due to reversible nature of host-guest interaction. The practical utility of the host-guest gel as a scratch curable coating is demonstrated. Flexible, tough, and self‐healable polymeric materials are promising to be a solution to the energy problem by substituting for conventional heavy materials. A fusion of supramolecular chemistry and polymer chemistry is a powerful method to create such intelligent materials. Here, a supramolecular polymeric material using multipoint molecular recognition between cyclodextrin (CD) and hydrophobic guest molecules at polymer side chain is reported. A transparent, flexible, and tough hydrogel (host–guest gel) is formed by a simple preparation procedure. The host–guest gel shows self‐healing property in both wet state and dry state due to reversible nature of host–guest interaction. The practical utility of the host–guest gel as a scratch curable coating is demonstrated. image
Author	Harada, Akira Nakahata, Masaki Takashima, Yoshinori
Author_xml	– sequence: 1 givenname: Masaki surname: Nakahata fullname: Nakahata, Masaki organization: Department of Macromolecular Science, Graduate School of Science, Osaka University, 560-0043, Toyonaka, Osaka, Japan – sequence: 2 givenname: Yoshinori surname: Takashima fullname: Takashima, Yoshinori organization: Department of Macromolecular Science, Graduate School of Science, Osaka University, 560-0043, Toyonaka, Osaka, Japan – sequence: 3 givenname: Akira surname: Harada fullname: Harada, Akira email: harada@chem.sci.osaka-u.ac.jp organization: Department of Macromolecular Science, Graduate School of Science, Osaka University, 560-0043, Toyonaka, Osaka, Japan
BackLink	https://www.ncbi.nlm.nih.gov/pubmed/26398922$$D View this record in MEDLINE/PubMed
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PublicationDateYYYYMMDD	2016-01-01
PublicationDate_xml	– month: 01 year: 2016 text: January 2016
PublicationDecade	2010
PublicationPlace	Germany
PublicationPlace_xml	– name: Germany – name: Weinheim
PublicationTitle	Macromolecular rapid communications.
PublicationTitleAlternate	Macromol. Rapid Commun
PublicationYear	2016
Publisher	Blackwell Publishing Ltd Wiley Subscription Services, Inc
Publisher_xml	– name: Blackwell Publishing Ltd – name: Wiley Subscription Services, Inc
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Snippet	Flexible, tough, and self‐healable polymeric materials are promising to be a solution to the energy problem by substituting for conventional heavy materials. A... Flexible, tough, and self-healable polymeric materials are promising to be a solution to the energy problem by substituting for conventional heavy materials. A...
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SubjectTerms	Chains (polymeric) Cyclodextrins Drying host-guest interactions Hydrogels Polymer chemistry Polymers Recognition reversible bond formation scratch-curable coatings self-healing Smart materials tough polymers Utilities
Title	Highly Flexible, Tough, and Self-Healing Supramolecular Polymeric Materials Using Host-Guest Interaction
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