Magnesium-doped Zinc Oxide as Electron Selective Contact Layers for Efficient Perovskite Solar Cells

The electron‐selective contact layer (ESL) in organometal halide‐based perovskite solar cells (PSCs) determines not only the power conversion efficiency (PCE) but also the thermostability of PSCs. To improve the thermostability of ZnO‐based PSCs, we developed Mg‐doped ZnO [Zn1−xMgxO (ZMO)] as a high...

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Published in	ChemSusChem Vol. 9; no. 18; pp. 2640 - 2647
Main Authors	Song, Jiaxing, Zheng, Enqiang, Liu, Leijing, Wang, Xiao-Feng, Chen, Gang, Tian, Wenjing, Miyasaka, Tsutomu
Format	Journal Article
Language	English
Published	Germany Blackwell Publishing Ltd 22.09.2016 Wiley Subscription Services, Inc
Subjects	Calcium Compounds - chemistry Contact Drug Stability Electric Power Supplies electron-selective contact Energy conversion efficiency Magnesium Magnesium - chemistry Oxides - chemistry perovskite Perovskites Photovoltaic cells Solar cells Solar Energy Stability Temperature Thermal stability thermostability Titanium - chemistry Zinc oxide Zinc Oxide - chemistry Zinc oxides electron-selective contact perovskite solar cells thermostability zinc oxide
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Abstract	The electron‐selective contact layer (ESL) in organometal halide‐based perovskite solar cells (PSCs) determines not only the power conversion efficiency (PCE) but also the thermostability of PSCs. To improve the thermostability of ZnO‐based PSCs, we developed Mg‐doped ZnO [Zn1−xMgxO (ZMO)] as a high optical transmittance ESL for the methylammonium lead trihalide perovskite absorber [CH3NH3PbI3]. We further investigated the optical and electrical properties of the ESL films with Mg contents of 0–30 mol % and the corresponding devices. We achieved a maximum PCE of 16.5 % with improved thermal stability of CH3NH3PbI3 on ESL with the optimal ZMO (0.4 m) containing 10 mol % Mg. Moreover, this optimized ZMO PSC exhibited significantly improved durability and photostability owing to the improved chemical/photochemical stability of the wider optical bandgap ZMO. Mg+ZnO=improved stability: To improve the power conversion efficiency and the thermostability in ZnO/CH3NH3PbI3‐based perovskite solar cells (PSCs), magnesium‐doped ZnO is developed as the electron‐selective contact layer. The optimized ZMO PSCs exhibit significantly improved durability and photo‐stability.
AbstractList	The electron-selective contact layer (ESL) in organometal halide-based perovskite solar cells (PSCs) determines not only the power conversion efficiency (PCE) but also the thermostability of PSCs. To improve the thermostability of ZnO-based PSCs, we developed Mg-doped ZnO [Zn sub(1-x)Mg sub(x)O (ZMO)] as a high optical transmittance ESL for the methylammonium lead trihalide perovskite absorber [CH sub(3)NH sub(3)PbI sub( 3)]. We further investigated the optical and electrical properties of the ESL films with Mg contents of 0-30mol% and the corresponding devices. We achieved a maximum PCE of 16.5% with improved thermal stability of CH sub(3)NH sub(3)PbI sub(3 ) on ESL with the optimal ZMO (0.4m) containing 10mol% Mg. Moreover, this optimized ZMO PSC exhibited significantly improved durability and photostability owing to the improved chemical/photochemical stability of the wider optical bandgap ZMO. Mg+ZnO=improved stability: To improve the power conversion efficiency and the thermostability in ZnO/CH sub(3)NH sub(3)PbI sub(3)-based perovskite solar cells (PSCs), magnesium-doped ZnO is developed as the electron-selective contact layer. The optimized ZMO PSCs exhibit significantly improved durability and photo-stability. The electron-selective contact layer (ESL) in organometal halide-based perovskite solar cells (PSCs) determines not only the power conversion efficiency (PCE) but also the thermostability of PSCs. To improve the thermostability of ZnO-based PSCs, we developed Mg-doped ZnO [Zn Mg O (ZMO)] as a high optical transmittance ESL for the methylammonium lead trihalide perovskite absorber [CH NH PbI ]. We further investigated the optical and electrical properties of the ESL films with Mg contents of 0-30 mol % and the corresponding devices. We achieved a maximum PCE of 16.5 % with improved thermal stability of CH NH PbI on ESL with the optimal ZMO (0.4 m) containing 10 mol % Mg. Moreover, this optimized ZMO PSC exhibited significantly improved durability and photostability owing to the improved chemical/photochemical stability of the wider optical bandgap ZMO. The electron-selective contact layer (ESL) in organometal halide-based perovskite solar cells (PSCs) determines not only the power conversion efficiency (PCE) but also the thermostability of PSCs. To improve the thermostability of ZnO-based PSCs, we developed Mg-doped ZnO [Zn1-xMgxO (ZMO)] as a high optical transmittance ESL for the methylammonium lead trihalide perovskite absorber [CH3NH3PbI3]. We further investigated the optical and electrical properties of the ESL films with Mg contents of 0-30mol% and the corresponding devices. We achieved a maximum PCE of 16.5% with improved thermal stability of CH3NH3PbI3 on ESL with the optimal ZMO (0.4m) containing 10mol% Mg. Moreover, this optimized ZMO PSC exhibited significantly improved durability and photostability owing to the improved chemical/photochemical stability of the wider optical bandgap ZMO. The electron‐selective contact layer (ESL) in organometal halide‐based perovskite solar cells (PSCs) determines not only the power conversion efficiency (PCE) but also the thermostability of PSCs. To improve the thermostability of ZnO‐based PSCs, we developed Mg‐doped ZnO [Zn 1− x Mg x O (ZMO)] as a high optical transmittance ESL for the methylammonium lead trihalide perovskite absorber [CH 3 NH 3 PbI 3 ]. We further investigated the optical and electrical properties of the ESL films with Mg contents of 0–30 mol % and the corresponding devices. We achieved a maximum PCE of 16.5 % with improved thermal stability of CH 3 NH 3 PbI 3 on ESL with the optimal ZMO (0.4 m ) containing 10 mol % Mg. Moreover, this optimized ZMO PSC exhibited significantly improved durability and photostability owing to the improved chemical/photochemical stability of the wider optical bandgap ZMO. The electron-selective contact layer (ESL) in organometal halide-based perovskite solar cells (PSCs) determines not only the power conversion efficiency (PCE) but also the thermostability of PSCs. To improve the thermostability of ZnO-based PSCs, we developed Mg-doped ZnO [Zn1-x Mgx O (ZMO)] as a high optical transmittance ESL for the methylammonium lead trihalide perovskite absorber [CH3 NH3 PbI3 ]. We further investigated the optical and electrical properties of the ESL films with Mg contents of 0-30 mol % and the corresponding devices. We achieved a maximum PCE of 16.5 % with improved thermal stability of CH3 NH3 PbI3 on ESL with the optimal ZMO (0.4 m) containing 10 mol % Mg. Moreover, this optimized ZMO PSC exhibited significantly improved durability and photostability owing to the improved chemical/photochemical stability of the wider optical bandgap ZMO.The electron-selective contact layer (ESL) in organometal halide-based perovskite solar cells (PSCs) determines not only the power conversion efficiency (PCE) but also the thermostability of PSCs. To improve the thermostability of ZnO-based PSCs, we developed Mg-doped ZnO [Zn1-x Mgx O (ZMO)] as a high optical transmittance ESL for the methylammonium lead trihalide perovskite absorber [CH3 NH3 PbI3 ]. We further investigated the optical and electrical properties of the ESL films with Mg contents of 0-30 mol % and the corresponding devices. We achieved a maximum PCE of 16.5 % with improved thermal stability of CH3 NH3 PbI3 on ESL with the optimal ZMO (0.4 m) containing 10 mol % Mg. Moreover, this optimized ZMO PSC exhibited significantly improved durability and photostability owing to the improved chemical/photochemical stability of the wider optical bandgap ZMO. The electron‐selective contact layer (ESL) in organometal halide‐based perovskite solar cells (PSCs) determines not only the power conversion efficiency (PCE) but also the thermostability of PSCs. To improve the thermostability of ZnO‐based PSCs, we developed Mg‐doped ZnO [Zn1−xMgxO (ZMO)] as a high optical transmittance ESL for the methylammonium lead trihalide perovskite absorber [CH3NH3PbI3]. We further investigated the optical and electrical properties of the ESL films with Mg contents of 0–30 mol % and the corresponding devices. We achieved a maximum PCE of 16.5 % with improved thermal stability of CH3NH3PbI3 on ESL with the optimal ZMO (0.4 m) containing 10 mol % Mg. Moreover, this optimized ZMO PSC exhibited significantly improved durability and photostability owing to the improved chemical/photochemical stability of the wider optical bandgap ZMO. Mg+ZnO=improved stability: To improve the power conversion efficiency and the thermostability in ZnO/CH3NH3PbI3‐based perovskite solar cells (PSCs), magnesium‐doped ZnO is developed as the electron‐selective contact layer. The optimized ZMO PSCs exhibit significantly improved durability and photo‐stability.
Author	Tian, Wenjing Miyasaka, Tsutomu Zheng, Enqiang Chen, Gang Song, Jiaxing Liu, Leijing Wang, Xiao-Feng
Author_xml	– sequence: 1 givenname: Jiaxing surname: Song fullname: Song, Jiaxing organization: State Key Laboratory of Supramolecular Structure and Materials, Jilin University, 130012, Changchun, PR China – sequence: 2 givenname: Enqiang surname: Zheng fullname: Zheng, Enqiang organization: Key Laboratory of Physics and Technology for Advanced Batteries, Ministry of Education, College of Physics, Jilin University, 130012, Changchun, PR China – sequence: 3 givenname: Leijing surname: Liu fullname: Liu, Leijing organization: State Key Laboratory of Supramolecular Structure and Materials, Jilin University, 130012, Changchun, PR China – sequence: 4 givenname: Xiao-Feng surname: Wang fullname: Wang, Xiao-Feng email: xf_wang@jlu.edu.cn organization: Key Laboratory of Physics and Technology for Advanced Batteries, Ministry of Education, College of Physics, Jilin University, 130012, Changchun, PR China – sequence: 5 givenname: Gang surname: Chen fullname: Chen, Gang organization: Key Laboratory of Physics and Technology for Advanced Batteries, Ministry of Education, College of Physics, Jilin University, 130012, Changchun, PR China – sequence: 6 givenname: Wenjing surname: Tian fullname: Tian, Wenjing email: wjtian@jlu.edu.cn organization: State Key Laboratory of Supramolecular Structure and Materials, Jilin University, 130012, Changchun, PR China – sequence: 7 givenname: Tsutomu surname: Miyasaka fullname: Miyasaka, Tsutomu organization: Graduate School of Engineering, Toin University of Yokohama, 1614 Kurogane-cho, Aoba, Kanagawa, 225-8503, Yokohama, Japan
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Keywords	electron-selective contact perovskite solar cells thermostability zinc oxide
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Snippet	The electron‐selective contact layer (ESL) in organometal halide‐based perovskite solar cells (PSCs) determines not only the power conversion efficiency (PCE)... The electron-selective contact layer (ESL) in organometal halide-based perovskite solar cells (PSCs) determines not only the power conversion efficiency (PCE)...
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SubjectTerms	Calcium Compounds - chemistry Contact Drug Stability Electric Power Supplies electron-selective contact Energy conversion efficiency Magnesium Magnesium - chemistry Oxides - chemistry perovskite Perovskites Photovoltaic cells Solar cells Solar Energy Stability Temperature Thermal stability thermostability Titanium - chemistry Zinc oxide Zinc Oxide - chemistry Zinc oxides
Title	Magnesium-doped Zinc Oxide as Electron Selective Contact Layers for Efficient Perovskite Solar Cells
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