The Facile Modification of Polyacrylate Emulsion via Hexadecane to Enhance Controlled-release Profiles of Coated Urea
Development of controlled-release urea (CRU) has attracted research attention because of food scarcity problems and environmental concerns. To slow down the nutrient release of CRU coated with waterborne polyacrylate, conventional emulsion polymerization (CEP), conventional emulsion polymerization c...
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| Published in | Scientific reports Vol. 8; no. 1; pp. 12279 - 10 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
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London
Nature Publishing Group UK
16.08.2018
Nature Publishing Group Nature Portfolio |
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| Abstract | Development of controlled-release urea (CRU) has attracted research attention because of food scarcity problems and environmental concerns. To slow down the nutrient release of CRU coated with waterborne polyacrylate, conventional emulsion polymerization (CEP), conventional emulsion polymerization containing hexadecane (CEP + HD), and miniemulsion polymerization (MP) were carried out to discern the influence of polymerization technique and hexadecane on the properties of emulsions, films, and on the resultant nutrient release profiles of controlled-release urea. The addition of hexadecane improved water resistance, decreased the glass-transition temperature, and slowed down the nutrient release. CEP + HD was superior to MP in retarding nutrient release since the majority of HD was distributed in the exteriors of the particles of the former and interiors of the particles of the latter. Exterior HD improved water resistance more effectively, while interior HD reduced glass-transition temperature more significantly. Overall, our findings showed that incorporation of HD into polyacrylate emulsion produces excellent coatings that delay the release of urea. It has great potential application in controlled-release fertilizers coated with waterborne polymers. |
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| AbstractList | Development of controlled-release urea (CRU) has attracted research attention because of food scarcity problems and environmental concerns. To slow down the nutrient release of CRU coated with waterborne polyacrylate, conventional emulsion polymerization (CEP), conventional emulsion polymerization containing hexadecane (CEP + HD), and miniemulsion polymerization (MP) were carried out to discern the influence of polymerization technique and hexadecane on the properties of emulsions, films, and on the resultant nutrient release profiles of controlled-release urea. The addition of hexadecane improved water resistance, decreased the glass-transition temperature, and slowed down the nutrient release. CEP + HD was superior to MP in retarding nutrient release since the majority of HD was distributed in the exteriors of the particles of the former and interiors of the particles of the latter. Exterior HD improved water resistance more effectively, while interior HD reduced glass-transition temperature more significantly. Overall, our findings showed that incorporation of HD into polyacrylate emulsion produces excellent coatings that delay the release of urea. It has great potential application in controlled-release fertilizers coated with waterborne polymers. Development of controlled-release urea (CRU) has attracted research attention because of food scarcity problems and environmental concerns. To slow down the nutrient release of CRU coated with waterborne polyacrylate, conventional emulsion polymerization (CEP), conventional emulsion polymerization containing hexadecane (CEP + HD), and miniemulsion polymerization (MP) were carried out to discern the influence of polymerization technique and hexadecane on the properties of emulsions, films, and on the resultant nutrient release profiles of controlled-release urea. The addition of hexadecane improved water resistance, decreased the glass-transition temperature, and slowed down the nutrient release. CEP + HD was superior to MP in retarding nutrient release since the majority of HD was distributed in the exteriors of the particles of the former and interiors of the particles of the latter. Exterior HD improved water resistance more effectively, while interior HD reduced glass-transition temperature more significantly. Overall, our findings showed that incorporation of HD into polyacrylate emulsion produces excellent coatings that delay the release of urea. It has great potential application in controlled-release fertilizers coated with waterborne polymers.Development of controlled-release urea (CRU) has attracted research attention because of food scarcity problems and environmental concerns. To slow down the nutrient release of CRU coated with waterborne polyacrylate, conventional emulsion polymerization (CEP), conventional emulsion polymerization containing hexadecane (CEP + HD), and miniemulsion polymerization (MP) were carried out to discern the influence of polymerization technique and hexadecane on the properties of emulsions, films, and on the resultant nutrient release profiles of controlled-release urea. The addition of hexadecane improved water resistance, decreased the glass-transition temperature, and slowed down the nutrient release. CEP + HD was superior to MP in retarding nutrient release since the majority of HD was distributed in the exteriors of the particles of the former and interiors of the particles of the latter. Exterior HD improved water resistance more effectively, while interior HD reduced glass-transition temperature more significantly. Overall, our findings showed that incorporation of HD into polyacrylate emulsion produces excellent coatings that delay the release of urea. It has great potential application in controlled-release fertilizers coated with waterborne polymers. Abstract Development of controlled-release urea (CRU) has attracted research attention because of food scarcity problems and environmental concerns. To slow down the nutrient release of CRU coated with waterborne polyacrylate, conventional emulsion polymerization (CEP), conventional emulsion polymerization containing hexadecane (CEP + HD), and miniemulsion polymerization (MP) were carried out to discern the influence of polymerization technique and hexadecane on the properties of emulsions, films, and on the resultant nutrient release profiles of controlled-release urea. The addition of hexadecane improved water resistance, decreased the glass-transition temperature, and slowed down the nutrient release. CEP + HD was superior to MP in retarding nutrient release since the majority of HD was distributed in the exteriors of the particles of the former and interiors of the particles of the latter. Exterior HD improved water resistance more effectively, while interior HD reduced glass-transition temperature more significantly. Overall, our findings showed that incorporation of HD into polyacrylate emulsion produces excellent coatings that delay the release of urea. It has great potential application in controlled-release fertilizers coated with waterborne polymers. |
| ArticleNumber | 12279 |
| Author | Ma, Fei Zhou, Jianmin Shen, Yazhen Du, Changwen |
| Author_xml | – sequence: 1 givenname: Yazhen surname: Shen fullname: Shen, Yazhen organization: State Key Laboratory of Soil and Sustainable Agriculture, Institute of Soil Science, Chinese Academy of Sciences – sequence: 2 givenname: Changwen orcidid: 0000-0002-9064-3581 surname: Du fullname: Du, Changwen email: chwdu@issas.ac.cn organization: State Key Laboratory of Soil and Sustainable Agriculture, Institute of Soil Science, Chinese Academy of Sciences – sequence: 3 givenname: Jianmin surname: Zhou fullname: Zhou, Jianmin organization: State Key Laboratory of Soil and Sustainable Agriculture, Institute of Soil Science, Chinese Academy of Sciences – sequence: 4 givenname: Fei surname: Ma fullname: Ma, Fei organization: State Key Laboratory of Soil and Sustainable Agriculture, Institute of Soil Science, Chinese Academy of Sciences |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/30116004$$D View this record in MEDLINE/PubMed |
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| CitedBy_id | crossref_primary_10_1021_acs_langmuir_3c03713 crossref_primary_10_1016_j_eurpolymj_2020_110114 crossref_primary_10_1039_D3MA00378G crossref_primary_10_1590_0104_1428_04620 crossref_primary_10_3390_gels7040262 crossref_primary_10_1016_j_porgcoat_2020_105759 crossref_primary_10_1002_mren_202000049 crossref_primary_10_1039_C9RA06939A crossref_primary_10_1016_j_porgcoat_2020_105964 crossref_primary_10_1002_app_54846 crossref_primary_10_1016_j_partic_2023_06_019 crossref_primary_10_3390_polym10121296 |
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| Snippet | Development of controlled-release urea (CRU) has attracted research attention because of food scarcity problems and environmental concerns. To slow down the... Abstract Development of controlled-release urea (CRU) has attracted research attention because of food scarcity problems and environmental concerns. To slow... |
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| SubjectTerms | 704/172/4081 704/4111 Coatings Controlled release Emulsion polymerization Emulsions Fertilizers Hexadecane Humanities and Social Sciences multidisciplinary Nutrient release Polyacrylate Polymerization Polymers Science Science (multidisciplinary) Transition temperatures Urea |
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| Title | The Facile Modification of Polyacrylate Emulsion via Hexadecane to Enhance Controlled-release Profiles of Coated Urea |
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