Long range electrostatic forces in ionic liquids
Ionic liquids are pure salts that are liquid under ambient conditions. As liquids composed solely of ions, the scientific consensus has been that ionic liquids have exceedingly high ionic strengths and thus very short Debye screening lengths. However, several recent experiments from laboratories aro...
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| Published in | Chemical communications (Cambridge, England) Vol. 53; no. 7; pp. 1214 - 1224 |
|---|---|
| Main Authors | , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
England
2017
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| Subjects | |
| Online Access | Get full text |
| ISSN | 1359-7345 1364-548X 1364-548X |
| DOI | 10.1039/c6cc08820a |
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| Abstract | Ionic liquids are pure salts that are liquid under ambient conditions. As liquids composed solely of ions, the scientific consensus has been that ionic liquids have exceedingly high ionic strengths and thus very short Debye screening lengths. However, several recent experiments from laboratories around the world have reported data for the approach of two surfaces separated by ionic liquids which revealed remarkable long range forces that appear to be electrostatic in origin. Evidence has accumulated demonstrating long range surface forces for several different combinations of ionic liquids and electrically charged surfaces, as well as for concentrated mixtures of inorganic salts in solvent. The original interpretation of these forces, that ionic liquids could be envisioned as "dilute electrolytes," was controversial, and the origin of long range forces in ionic liquids remains the subject of discussion. Here we seek to collate and examine the evidence for long range surface forces in ionic liquids, identify key outstanding questions, and explore possible mechanisms underlying the origin of these long range forces. Long range surface forces in ionic liquids and other highly concentrated electrolytes hold diverse implications from designing ionic liquids for energy storage applications to rationalizing electrostatic correlations in biological self-assembly.
Experimental evidence for long range surface forces in ionic liquids is collated and examined, key outstanding questions are identified, and possible mechanisms underpinning these long range forces are explored. |
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| AbstractList | Ionic liquids are pure salts that are liquid under ambient conditions. As liquids composed solely of ions, the scientific consensus has been that ionic liquids have exceedingly high ionic strengths and thus very short Debye screening lengths. However, several recent experiments from laboratories around the world have reported data for the approach of two surfaces separated by ionic liquids which revealed remarkable long range forces that appear to be electrostatic in origin. Evidence has accumulated demonstrating long range surface forces for several different combinations of ionic liquids and electrically charged surfaces, as well as for concentrated mixtures of inorganic salts in solvent. The original interpretation of these forces, that ionic liquids could be envisioned as "dilute electrolytes," was controversial, and the origin of long range forces in ionic liquids remains the subject of discussion. Here we seek to collate and examine the evidence for long range surface forces in ionic liquids, identify key outstanding questions, and explore possible mechanisms underlying the origin of these long range forces. Long range surface forces in ionic liquids and other highly concentrated electrolytes hold diverse implications from designing ionic liquids for energy storage applications to rationalizing electrostatic correlations in biological self-assembly.
Experimental evidence for long range surface forces in ionic liquids is collated and examined, key outstanding questions are identified, and possible mechanisms underpinning these long range forces are explored. Ionic liquids are pure salts that are liquid under ambient conditions. As liquids composed solely of ions, the scientific consensus has been that ionic liquids have exceedingly high ionic strengths and thus very short Debye screening lengths. However, several recent experiments from laboratories around the world have reported data for the approach of two surfaces separated by ionic liquids which revealed remarkable long range forces that appear to be electrostatic in origin. Evidence has accumulated demonstrating long range surface forces for several different combinations of ionic liquids and electrically charged surfaces, as well as for concentrated mixtures of inorganic salts in solvent. The original interpretation of these forces, that ionic liquids could be envisioned as "dilute electrolytes," was controversial, and the origin of long range forces in ionic liquids remains the subject of discussion. Here we seek to collate and examine the evidence for long range surface forces in ionic liquids, identify key outstanding questions, and explore possible mechanisms underlying the origin of these long range forces. Long range surface forces in ionic liquids and other highly concentrated electrolytes hold diverse implications from designing ionic liquids for energy storage applications to rationalizing electrostatic correlations in biological self-assembly. |
| Author | Rutland, Mark W Valtiner, Markus Atkin, Rob Smith, Alexander M Warr, Gregory G Lee, Alpha A Israelachvili, Jacob N Dobbs, Howard A Banquy, Xavier Gebbie, Matthew A Perkin, Susan |
| AuthorAffiliation | The University of Sydney Priority Research Centre for Advanced Fluid Interfaces Stanford University Newcastle Institute for Energy and Resources Surface and Corrosion Science F11 SP Chemistry Materials and Surfaces Physical & Theoretical Chemistry Laboratory University of California School of Engineering and Applied Sciences Faculty of Pharmacy KTH Royal Institute of Technology Harvard University Geballe Laboratory for Advanced Materials School of Chemistry Department of Chemistry The University of Newcastle Interface Chemistry and Surface Engineering Department of Chemical Engineering University of Oxford Max Planck Institut fur Eisenforschung GmbH Universite de Montreal |
| AuthorAffiliation_xml | – name: Department of Chemical Engineering – name: Surface and Corrosion Science – name: Department of Chemistry – name: Interface Chemistry and Surface Engineering – name: Geballe Laboratory for Advanced Materials – name: The University of Newcastle – name: School of Engineering and Applied Sciences – name: Newcastle Institute for Energy and Resources – name: Max Planck Institut fur Eisenforschung GmbH – name: Physical & Theoretical Chemistry Laboratory – name: The University of Sydney – name: Faculty of Pharmacy – name: Stanford University – name: University of Oxford – name: F11 – name: University of California – name: KTH Royal Institute of Technology – name: SP Chemistry Materials and Surfaces – name: Priority Research Centre for Advanced Fluid Interfaces – name: Harvard University – name: School of Chemistry – name: Universite de Montreal |
| Author_xml | – sequence: 1 givenname: Matthew A surname: Gebbie fullname: Gebbie, Matthew A – sequence: 2 givenname: Alexander M surname: Smith fullname: Smith, Alexander M – sequence: 3 givenname: Howard A surname: Dobbs fullname: Dobbs, Howard A – sequence: 4 givenname: Alpha A surname: Lee fullname: Lee, Alpha A – sequence: 5 givenname: Gregory G surname: Warr fullname: Warr, Gregory G – sequence: 6 givenname: Xavier surname: Banquy fullname: Banquy, Xavier – sequence: 7 givenname: Markus surname: Valtiner fullname: Valtiner, Markus – sequence: 8 givenname: Mark W surname: Rutland fullname: Rutland, Mark W – sequence: 9 givenname: Jacob N surname: Israelachvili fullname: Israelachvili, Jacob N – sequence: 10 givenname: Susan surname: Perkin fullname: Perkin, Susan – sequence: 11 givenname: Rob surname: Atkin fullname: Atkin, Rob |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/28000809$$D View this record in MEDLINE/PubMed https://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-204710$$DView record from Swedish Publication Index https://urn.kb.se/resolve?urn=urn:nbn:se:ri:diva-30985$$DView record from Swedish Publication Index |
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| Snippet | Ionic liquids are pure salts that are liquid under ambient conditions. As liquids composed solely of ions, the scientific consensus has been that ionic liquids... |
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| SubjectTerms | chemical reactions dielectric constant Electrolytes electrostatic interactions Electrostatics energy force Inorganic salts ion ionic liquid Ionic liquids ionic strength ions Liquids nanomaterial Origins physics screening Self assembly Solvents static electricity surface property |
| Title | Long range electrostatic forces in ionic liquids |
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