Nickel@Siloxene catalytic nanosheets for high-performance CO2 methanation
Two-dimensional (2D) materials are of considerable interest for catalyzing the heterogeneous conversion of CO 2 to synthetic fuels. In this regard, 2D siloxene nanosheets, have escaped thorough exploration, despite being composed of earth-abundant elements. Herein we demonstrate the remarkable catal...
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| Published in | Nature communications Vol. 10; no. 1; pp. 2608 - 11 |
|---|---|
| Main Authors | , , , , , , , , , , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
13.06.2019
Nature Publishing Group Nature Portfolio |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Two-dimensional (2D) materials are of considerable interest for catalyzing the heterogeneous conversion of CO
2
to synthetic fuels. In this regard, 2D siloxene nanosheets, have escaped thorough exploration, despite being composed of earth-abundant elements. Herein we demonstrate the remarkable catalytic activity, selectivity, and stability of a nickel@siloxene nanocomposite; it is found that this promising catalytic performance is highly sensitive to the location of the nickel component, being on either the interior or the exterior of adjacent siloxene nanosheets. Control over the location of nickel is achieved by employing the terminal groups of siloxene and varying the solvent used during its nucleation and growth, which ultimately determines the distinct reaction intermediates and pathways for the catalytic CO
2
methanation. Significantly, a CO
2
methanation rate of 100 mmol g
Ni
−1
h
−1
is achieved with over 90% selectivity when nickel resides specifically between the sheets of siloxene.
There is a strong push to develop new catalysts and supports to convert low-value CO
2
into high-value CH
4
. Here, authors found that the internal or external confinement of Ni on multi-layered siloxene supports determined the reaction pathway, activity, selectivity, and stability in CO
2
methanation. |
|---|---|
| AbstractList | Abstract Two-dimensional (2D) materials are of considerable interest for catalyzing the heterogeneous conversion of CO2 to synthetic fuels. In this regard, 2D siloxene nanosheets, have escaped thorough exploration, despite being composed of earth-abundant elements. Herein we demonstrate the remarkable catalytic activity, selectivity, and stability of a nickel@siloxene nanocomposite; it is found that this promising catalytic performance is highly sensitive to the location of the nickel component, being on either the interior or the exterior of adjacent siloxene nanosheets. Control over the location of nickel is achieved by employing the terminal groups of siloxene and varying the solvent used during its nucleation and growth, which ultimately determines the distinct reaction intermediates and pathways for the catalytic CO2 methanation. Significantly, a CO2 methanation rate of 100 mmol gNi−1 h−1 is achieved with over 90% selectivity when nickel resides specifically between the sheets of siloxene. Two-dimensional (2D) materials are of considerable interest for catalyzing the heterogeneous conversion of CO2 to synthetic fuels. In this regard, 2D siloxene nanosheets, have escaped thorough exploration, despite being composed of earth-abundant elements. Herein we demonstrate the remarkable catalytic activity, selectivity, and stability of a nickel@siloxene nanocomposite; it is found that this promising catalytic performance is highly sensitive to the location of the nickel component, being on either the interior or the exterior of adjacent siloxene nanosheets. Control over the location of nickel is achieved by employing the terminal groups of siloxene and varying the solvent used during its nucleation and growth, which ultimately determines the distinct reaction intermediates and pathways for the catalytic CO2 methanation. Significantly, a CO2 methanation rate of 100 mmol gNi−1 h−1 is achieved with over 90% selectivity when nickel resides specifically between the sheets of siloxene.There is a strong push to develop new catalysts and supports to convert low-value CO2 into high-value CH4. Here, authors found that the internal or external confinement of Ni on multi-layered siloxene supports determined the reaction pathway, activity, selectivity, and stability in CO2 methanation. Two-dimensional (2D) materials are of considerable interest for catalyzing the heterogeneous conversion of CO 2 to synthetic fuels. In this regard, 2D siloxene nanosheets, have escaped thorough exploration, despite being composed of earth-abundant elements. Herein we demonstrate the remarkable catalytic activity, selectivity, and stability of a nickel@siloxene nanocomposite; it is found that this promising catalytic performance is highly sensitive to the location of the nickel component, being on either the interior or the exterior of adjacent siloxene nanosheets. Control over the location of nickel is achieved by employing the terminal groups of siloxene and varying the solvent used during its nucleation and growth, which ultimately determines the distinct reaction intermediates and pathways for the catalytic CO 2 methanation. Significantly, a CO 2 methanation rate of 100 mmol g Ni −1 h −1 is achieved with over 90% selectivity when nickel resides specifically between the sheets of siloxene. There is a strong push to develop new catalysts and supports to convert low-value CO 2 into high-value CH 4 . Here, authors found that the internal or external confinement of Ni on multi-layered siloxene supports determined the reaction pathway, activity, selectivity, and stability in CO 2 methanation. Two-dimensional (2D) materials are of considerable interest for catalyzing the heterogeneous conversion of CO2 to synthetic fuels. In this regard, 2D siloxene nanosheets, have escaped thorough exploration, despite being composed of earth-abundant elements. Herein we demonstrate the remarkable catalytic activity, selectivity, and stability of a nickel@siloxene nanocomposite; it is found that this promising catalytic performance is highly sensitive to the location of the nickel component, being on either the interior or the exterior of adjacent siloxene nanosheets. Control over the location of nickel is achieved by employing the terminal groups of siloxene and varying the solvent used during its nucleation and growth, which ultimately determines the distinct reaction intermediates and pathways for the catalytic CO2 methanation. Significantly, a CO2 methanation rate of 100 mmol gNi−1 h−1 is achieved with over 90% selectivity when nickel resides specifically between the sheets of siloxene. Two-dimensional (2D) materials are of considerable interest for catalyzing the heterogeneous conversion of CO2 to synthetic fuels. In this regard, 2D siloxene nanosheets, have escaped thorough exploration, despite being composed of earth-abundant elements. Herein we demonstrate the remarkable catalytic activity, selectivity, and stability of a nickel@siloxene nanocomposite; it is found that this promising catalytic performance is highly sensitive to the location of the nickel component, being on either the interior or the exterior of adjacent siloxene nanosheets. Control over the location of nickel is achieved by employing the terminal groups of siloxene and varying the solvent used during its nucleation and growth, which ultimately determines the distinct reaction intermediates and pathways for the catalytic CO2 methanation. Significantly, a CO2 methanation rate of 100 mmol gNi–1 h–1 is achieved with over 90% selectivity when nickel resides specifically between the sheets of siloxene. Abstract Two-dimensional (2D) materials are of considerable interest for catalyzing the heterogeneous conversion of CO 2 to synthetic fuels. In this regard, 2D siloxene nanosheets, have escaped thorough exploration, despite being composed of earth-abundant elements. Herein we demonstrate the remarkable catalytic activity, selectivity, and stability of a nickel@siloxene nanocomposite; it is found that this promising catalytic performance is highly sensitive to the location of the nickel component, being on either the interior or the exterior of adjacent siloxene nanosheets. Control over the location of nickel is achieved by employing the terminal groups of siloxene and varying the solvent used during its nucleation and growth, which ultimately determines the distinct reaction intermediates and pathways for the catalytic CO 2 methanation. Significantly, a CO 2 methanation rate of 100 mmol g Ni −1 h −1 is achieved with over 90% selectivity when nickel resides specifically between the sheets of siloxene. |
| ArticleNumber | 2608 |
| Author | Hung, Darius L. H. Wang, Wu Tavasoli, Alexandra Song, Rui Kumar, Sai Govind Hari Guo, Jiuli Li, Ruifeng Wang, Di Kübel, Christian Wan, Lili Sun, Wei Fan, Liming Li, Young Feng Duchesne, Paul N. Wang, Lu Gourevich, Ilya Lu, Jingjun Yan, Xiaoliang Hatton, Benjamin D. Ali, Feysal M. Ozin, Geoffrey A. Wood, Thomas E. |
| Author_xml | – sequence: 1 givenname: Xiaoliang surname: Yan fullname: Yan, Xiaoliang email: yanxiaoliang@tyut.edu.cn organization: College of Chemistry and Chemical Engineering, Taiyuan University of Technology, Materials Chemistry and Nanochemistry Research Group, Solar Fuels Cluster, Department of Chemistry, University of Toronto – sequence: 2 givenname: Wei surname: Sun fullname: Sun, Wei organization: Materials Chemistry and Nanochemistry Research Group, Solar Fuels Cluster, Department of Chemistry, University of Toronto, State Key Laboratory of Silicon Materials and School of Materials Science and Engineering, Zhejiang University – sequence: 3 givenname: Liming surname: Fan fullname: Fan, Liming organization: College of Chemistry and Chemical Engineering, Taiyuan University of Technology – sequence: 4 givenname: Paul N. surname: Duchesne fullname: Duchesne, Paul N. organization: Materials Chemistry and Nanochemistry Research Group, Solar Fuels Cluster, Department of Chemistry, University of Toronto – sequence: 5 givenname: Wu surname: Wang fullname: Wang, Wu organization: Karlsruhe Institute of Technology (KIT), Institute of Nanotechnology (INT) – sequence: 6 givenname: Christian orcidid: 0000-0001-5701-4006 surname: Kübel fullname: Kübel, Christian organization: Karlsruhe Institute of Technology (KIT), Institute of Nanotechnology (INT) – sequence: 7 givenname: Di surname: Wang fullname: Wang, Di organization: Karlsruhe Institute of Technology (KIT), Institute of Nanotechnology (INT) – sequence: 8 givenname: Sai Govind Hari surname: Kumar fullname: Kumar, Sai Govind Hari organization: Materials Chemistry and Nanochemistry Research Group, Solar Fuels Cluster, Department of Chemistry, University of Toronto – sequence: 9 givenname: Young Feng surname: Li fullname: Li, Young Feng organization: Materials Chemistry and Nanochemistry Research Group, Solar Fuels Cluster, Department of Chemistry, University of Toronto – sequence: 10 givenname: Alexandra surname: Tavasoli fullname: Tavasoli, Alexandra organization: Materials Chemistry and Nanochemistry Research Group, Solar Fuels Cluster, Department of Chemistry, University of Toronto, Department of Materials Science and Engineering, University of Toronto – sequence: 11 givenname: Thomas E. surname: Wood fullname: Wood, Thomas E. organization: Materials Chemistry and Nanochemistry Research Group, Solar Fuels Cluster, Department of Chemistry, University of Toronto – sequence: 12 givenname: Darius L. H. orcidid: 0000-0002-3819-7078 surname: Hung fullname: Hung, Darius L. H. organization: Materials Chemistry and Nanochemistry Research Group, Solar Fuels Cluster, Department of Chemistry, University of Toronto – sequence: 13 givenname: Lili surname: Wan fullname: Wan, Lili organization: Materials Chemistry and Nanochemistry Research Group, Solar Fuels Cluster, Department of Chemistry, University of Toronto – sequence: 14 givenname: Lu orcidid: 0000-0002-4165-4022 surname: Wang fullname: Wang, Lu organization: Materials Chemistry and Nanochemistry Research Group, Solar Fuels Cluster, Department of Chemistry, University of Toronto – sequence: 15 givenname: Rui surname: Song fullname: Song, Rui organization: Materials Chemistry and Nanochemistry Research Group, Solar Fuels Cluster, Department of Chemistry, University of Toronto – sequence: 16 givenname: Jiuli surname: Guo fullname: Guo, Jiuli organization: Materials Chemistry and Nanochemistry Research Group, Solar Fuels Cluster, Department of Chemistry, University of Toronto – sequence: 17 givenname: Ilya orcidid: 0000-0003-3726-9233 surname: Gourevich fullname: Gourevich, Ilya organization: Materials Chemistry and Nanochemistry Research Group, Solar Fuels Cluster, Department of Chemistry, University of Toronto – sequence: 18 givenname: Feysal M. surname: Ali fullname: Ali, Feysal M. organization: Materials Chemistry and Nanochemistry Research Group, Solar Fuels Cluster, Department of Chemistry, University of Toronto – sequence: 19 givenname: Jingjun surname: Lu fullname: Lu, Jingjun organization: College of Chemistry and Chemical Engineering, Taiyuan University of Technology – sequence: 20 givenname: Ruifeng surname: Li fullname: Li, Ruifeng organization: College of Chemistry and Chemical Engineering, Taiyuan University of Technology – sequence: 21 givenname: Benjamin D. orcidid: 0000-0002-8181-1344 surname: Hatton fullname: Hatton, Benjamin D. organization: Department of Materials Science and Engineering, University of Toronto – sequence: 22 givenname: Geoffrey A. orcidid: 0000-0002-6315-0925 surname: Ozin fullname: Ozin, Geoffrey A. email: gozin@chem.utoronto.ca organization: Materials Chemistry and Nanochemistry Research Group, Solar Fuels Cluster, Department of Chemistry, University of Toronto |
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| Copyright | The Author(s) 2019 2019. This work is published under http://creativecommons.org/licenses/by/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License. The Author(s) 2019. This work is published under http://creativecommons.org/licenses/by/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License. |
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| CorporateAuthor | Argonne National Laboratory (ANL), Argonne, IL (United States). Advanced Photon Source (APS) |
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| DOI | 10.1038/s41467-019-10464-x |
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to synthetic fuels. In this regard, 2D siloxene... Abstract Two-dimensional (2D) materials are of considerable interest for catalyzing the heterogeneous conversion of CO 2 to synthetic fuels. In this regard, 2D... Two-dimensional (2D) materials are of considerable interest for catalyzing the heterogeneous conversion of CO2 to synthetic fuels. In this regard, 2D siloxene... Abstract Two-dimensional (2D) materials are of considerable interest for catalyzing the heterogeneous conversion of CO2 to synthetic fuels. In this regard, 2D... |
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| Title | Nickel@Siloxene catalytic nanosheets for high-performance CO2 methanation |
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