Core–Shell Crystals of Porous Organic Cages
The first examples of core–shell porous molecular crystals are described. The physical properties of the core–shell crystals, such as surface hydrophobicity, CO2 /CH4 selectivity, are controlled by the chemical composition of the shell. This shows that porous core–shell molecular crystals can exhibi...
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| Published in | Angewandte Chemie International Edition Vol. 57; no. 35; pp. 11228 - 11232 |
|---|---|
| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
27.08.2018
John Wiley and Sons Inc |
| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | The first examples of core–shell porous molecular crystals are described. The physical properties of the core–shell crystals, such as surface hydrophobicity, CO2 /CH4 selectivity, are controlled by the chemical composition of the shell. This shows that porous core–shell molecular crystals can exhibit synergistic properties that out‐perform materials built from the individual, constituent molecules.
Synergistic properties: A defect‐free core–shell molecular cocrystal was constructed. It combines good CO2 adsorption capacity in the core with high CO2/CH4 selectivity from the surrounding shell, and tunable surface hydrophobicity. |
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| AbstractList | The first examples of core–shell porous molecular crystals are described. The physical properties of the core–shell crystals, such as surface hydrophobicity, CO
2
/CH
4
selectivity, are controlled by the chemical composition of the shell. This shows that porous core–shell molecular crystals can exhibit synergistic properties that out‐perform materials built from the individual, constituent molecules. The first examples of core–shell porous molecular crystals are described. The physical properties of the core–shell crystals, such as surface hydrophobicity, CO2 /CH4 selectivity, are controlled by the chemical composition of the shell. This shows that porous core–shell molecular crystals can exhibit synergistic properties that out‐perform materials built from the individual, constituent molecules. Synergistic properties: A defect‐free core–shell molecular cocrystal was constructed. It combines good CO2 adsorption capacity in the core with high CO2/CH4 selectivity from the surrounding shell, and tunable surface hydrophobicity. The first examples of core–shell porous molecular crystals are described. The physical properties of the core–shell crystals, such as surface hydrophobicity, CO2 /CH4 selectivity, are controlled by the chemical composition of the shell. This shows that porous core–shell molecular crystals can exhibit synergistic properties that out‐perform materials built from the individual, constituent molecules. The first examples of core-shell porous molecular crystals are described. The physical properties of the core-shell crystals, such as surface hydrophobicity, CO2 /CH4 selectivity, are controlled by the chemical composition of the shell. This shows that porous core-shell molecular crystals can exhibit synergistic properties that out-perform materials built from the individual, constituent molecules.The first examples of core-shell porous molecular crystals are described. The physical properties of the core-shell crystals, such as surface hydrophobicity, CO2 /CH4 selectivity, are controlled by the chemical composition of the shell. This shows that porous core-shell molecular crystals can exhibit synergistic properties that out-perform materials built from the individual, constituent molecules. The first examples of core-shell porous molecular crystals are described. The physical properties of the core-shell crystals, such as surface hydrophobicity, CO /CH selectivity, are controlled by the chemical composition of the shell. This shows that porous core-shell molecular crystals can exhibit synergistic properties that out-perform materials built from the individual, constituent molecules. |
| Author | Hasell, Tom Cooper, Andrew I. Marcello, Marco Corcoran, Edward W. Jiang, Shan Calabro, David C. Du, Yi Chong, Samantha Y. Chen, Linjiang Clowes, Rob |
| AuthorAffiliation | 2 Corporate Strategic Research ExxonMobil Research and Engineering Company 1545 U.S. Highway 22 Annandale NJ 08801 USA 1 Department of Chemistry, Materials Innovation Factory University of Liverpool Liverpool L69 7ZD UK 3 Institute of Integrative Biology University of Liverpool Crown Street Liverpool L69 7ZD UK |
| AuthorAffiliation_xml | – name: 2 Corporate Strategic Research ExxonMobil Research and Engineering Company 1545 U.S. Highway 22 Annandale NJ 08801 USA – name: 3 Institute of Integrative Biology University of Liverpool Crown Street Liverpool L69 7ZD UK – name: 1 Department of Chemistry, Materials Innovation Factory University of Liverpool Liverpool L69 7ZD UK |
| Author_xml | – sequence: 1 givenname: Shan surname: Jiang fullname: Jiang, Shan organization: University of Liverpool – sequence: 2 givenname: Yi surname: Du fullname: Du, Yi organization: ExxonMobil Research and Engineering Company – sequence: 3 givenname: Marco surname: Marcello fullname: Marcello, Marco organization: University of Liverpool – sequence: 4 givenname: Edward W. surname: Corcoran fullname: Corcoran, Edward W. organization: ExxonMobil Research and Engineering Company – sequence: 5 givenname: David C. surname: Calabro fullname: Calabro, David C. organization: ExxonMobil Research and Engineering Company – sequence: 6 givenname: Samantha Y. orcidid: 0000-0002-3095-875X surname: Chong fullname: Chong, Samantha Y. organization: University of Liverpool – sequence: 7 givenname: Linjiang surname: Chen fullname: Chen, Linjiang organization: University of Liverpool – sequence: 8 givenname: Rob surname: Clowes fullname: Clowes, Rob organization: University of Liverpool – sequence: 9 givenname: Tom orcidid: 0000-0003-4736-0604 surname: Hasell fullname: Hasell, Tom email: T.Hasell@liverpool.ac.uk organization: University of Liverpool – sequence: 10 givenname: Andrew I. orcidid: 0000-0003-0201-1021 surname: Cooper fullname: Cooper, Andrew I. email: aicooper@liverpool.ac.uk organization: University of Liverpool |
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| Keywords | surface hydrophobicity adsorption selectivity core-shell crystals porous cage crystals |
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| Snippet | The first examples of core–shell porous molecular crystals are described. The physical properties of the core–shell crystals, such as surface hydrophobicity,... The first examples of core-shell porous molecular crystals are described. The physical properties of the core-shell crystals, such as surface hydrophobicity,... |
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| SubjectTerms | adsorption selectivity Cages Carbon dioxide Chemical composition Communication Communications Construction materials core–shell crystals Crystals Hydrophobicity Organic chemistry Physical properties porous cage crystals surface hydrophobicity |
| Title | Core–Shell Crystals of Porous Organic Cages |
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