Giant energy-storage density with ultrahigh efficiency in lead-free relaxors via high-entropy design
Next-generation advanced high/pulsed power capacitors rely heavily on dielectric ceramics with high energy storage performance. However, thus far, the huge challenge of realizing ultrahigh recoverable energy storage density ( W rec ) accompanied by ultrahigh efficiency ( η ) still existed and has be...
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| Published in | Nature communications Vol. 13; no. 1; pp. 3089 - 8 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
02.06.2022
Nature Publishing Group Nature Portfolio |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Next-generation advanced high/pulsed power capacitors rely heavily on dielectric ceramics with high energy storage performance. However, thus far, the huge challenge of realizing ultrahigh recoverable energy storage density (
W
rec
) accompanied by ultrahigh efficiency (
η
) still existed and has become a key bottleneck restricting the development of dielectric materials in cutting-edge energy storage applications. Here, we propose a high-entropy strategy to design “local polymorphic distortion” including rhombohedral-orthorhombic-tetragonal-cubic multiphase nanoclusters and random oxygen octahedral tilt, resulting in ultrasmall polar nanoregions, an enhanced breakdown electric field, and delayed polarization saturation. A giant
W
rec
~10.06 J cm
−3
is realized in lead-free relaxor ferroelectrics, especially with an ultrahigh
η
~90.8%, showing breakthrough progress in the comprehensive energy storage performance for lead-free bulk ceramics. This work opens up an effective avenue to design dielectric materials with ultrahigh comprehensive energy storage performance to meet the demanding requirements of advanced energy storage applications.
Dielectric ceramics are widely used in advanced high/pulsed power capacitors. Here, the authors propose a high-entropy strategy to design “local polymorphic distortion” in lead-free ceramics, achieving high energy storage performance. |
|---|---|
| AbstractList | Next-generation advanced high/pulsed power capacitors rely heavily on dielectric ceramics with high energy storage performance. However, thus far, the huge challenge of realizing ultrahigh recoverable energy storage density (
W
rec
) accompanied by ultrahigh efficiency (
η
) still existed and has become a key bottleneck restricting the development of dielectric materials in cutting-edge energy storage applications. Here, we propose a high-entropy strategy to design “local polymorphic distortion” including rhombohedral-orthorhombic-tetragonal-cubic multiphase nanoclusters and random oxygen octahedral tilt, resulting in ultrasmall polar nanoregions, an enhanced breakdown electric field, and delayed polarization saturation. A giant
W
rec
~10.06 J cm
−3
is realized in lead-free relaxor ferroelectrics, especially with an ultrahigh
η
~90.8%, showing breakthrough progress in the comprehensive energy storage performance for lead-free bulk ceramics. This work opens up an effective avenue to design dielectric materials with ultrahigh comprehensive energy storage performance to meet the demanding requirements of advanced energy storage applications.
Dielectric ceramics are widely used in advanced high/pulsed power capacitors. Here, the authors propose a high-entropy strategy to design “local polymorphic distortion” in lead-free ceramics, achieving high energy storage performance. Next-generation advanced high/pulsed power capacitors rely heavily on dielectric ceramics with high energy storage performance. However, thus far, the huge challenge of realizing ultrahigh recoverable energy storage density (W ) accompanied by ultrahigh efficiency (η) still existed and has become a key bottleneck restricting the development of dielectric materials in cutting-edge energy storage applications. Here, we propose a high-entropy strategy to design "local polymorphic distortion" including rhombohedral-orthorhombic-tetragonal-cubic multiphase nanoclusters and random oxygen octahedral tilt, resulting in ultrasmall polar nanoregions, an enhanced breakdown electric field, and delayed polarization saturation. A giant W ~10.06 J cm is realized in lead-free relaxor ferroelectrics, especially with an ultrahigh η ~90.8%, showing breakthrough progress in the comprehensive energy storage performance for lead-free bulk ceramics. This work opens up an effective avenue to design dielectric materials with ultrahigh comprehensive energy storage performance to meet the demanding requirements of advanced energy storage applications. Next-generation advanced high/pulsed power capacitors rely heavily on dielectric ceramics with high energy storage performance. However, thus far, the huge challenge of realizing ultrahigh recoverable energy storage density (Wrec) accompanied by ultrahigh efficiency (η) still existed and has become a key bottleneck restricting the development of dielectric materials in cutting-edge energy storage applications. Here, we propose a high-entropy strategy to design "local polymorphic distortion" including rhombohedral-orthorhombic-tetragonal-cubic multiphase nanoclusters and random oxygen octahedral tilt, resulting in ultrasmall polar nanoregions, an enhanced breakdown electric field, and delayed polarization saturation. A giant Wrec ~10.06 J cm-3 is realized in lead-free relaxor ferroelectrics, especially with an ultrahigh η ~90.8%, showing breakthrough progress in the comprehensive energy storage performance for lead-free bulk ceramics. This work opens up an effective avenue to design dielectric materials with ultrahigh comprehensive energy storage performance to meet the demanding requirements of advanced energy storage applications.Next-generation advanced high/pulsed power capacitors rely heavily on dielectric ceramics with high energy storage performance. However, thus far, the huge challenge of realizing ultrahigh recoverable energy storage density (Wrec) accompanied by ultrahigh efficiency (η) still existed and has become a key bottleneck restricting the development of dielectric materials in cutting-edge energy storage applications. Here, we propose a high-entropy strategy to design "local polymorphic distortion" including rhombohedral-orthorhombic-tetragonal-cubic multiphase nanoclusters and random oxygen octahedral tilt, resulting in ultrasmall polar nanoregions, an enhanced breakdown electric field, and delayed polarization saturation. A giant Wrec ~10.06 J cm-3 is realized in lead-free relaxor ferroelectrics, especially with an ultrahigh η ~90.8%, showing breakthrough progress in the comprehensive energy storage performance for lead-free bulk ceramics. This work opens up an effective avenue to design dielectric materials with ultrahigh comprehensive energy storage performance to meet the demanding requirements of advanced energy storage applications. Dielectric ceramics are widely used in advanced high/pulsed power capacitors. Here, the authors propose a high-entropy strategy to design “local polymorphic distortion” in lead-free ceramics, achieving high energy storage performance. Next-generation advanced high/pulsed power capacitors rely heavily on dielectric ceramics with high energy storage performance. However, thus far, the huge challenge of realizing ultrahigh recoverable energy storage density (Wrec) accompanied by ultrahigh efficiency (η) still existed and has become a key bottleneck restricting the development of dielectric materials in cutting-edge energy storage applications. Here, we propose a high-entropy strategy to design “local polymorphic distortion” including rhombohedral-orthorhombic-tetragonal-cubic multiphase nanoclusters and random oxygen octahedral tilt, resulting in ultrasmall polar nanoregions, an enhanced breakdown electric field, and delayed polarization saturation. A giant Wrec ~10.06 J cm-3 is realized in lead-free relaxor ferroelectrics, especially with an ultrahigh η ~90.8%, showing breakthrough progress in the comprehensive energy storage performance for lead-free bulk ceramics. This work opens up an effective avenue to design dielectric materials with ultrahigh comprehensive energy storage performance to meet the demanding requirements of advanced energy storage applications. Next-generation advanced high/pulsed power capacitors rely heavily on dielectric ceramics with high energy storage performance. However, thus far, the huge challenge of realizing ultrahigh recoverable energy storage density (Wrec) accompanied by ultrahigh efficiency (η) still existed and has become a key bottleneck restricting the development of dielectric materials in cutting-edge energy storage applications. Here, we propose a high-entropy strategy to design “local polymorphic distortion” including rhombohedral-orthorhombic-tetragonal-cubic multiphase nanoclusters and random oxygen octahedral tilt, resulting in ultrasmall polar nanoregions, an enhanced breakdown electric field, and delayed polarization saturation. A giant Wrec ~10.06 J cm−3 is realized in lead-free relaxor ferroelectrics, especially with an ultrahigh η ~90.8%, showing breakthrough progress in the comprehensive energy storage performance for lead-free bulk ceramics. This work opens up an effective avenue to design dielectric materials with ultrahigh comprehensive energy storage performance to meet the demanding requirements of advanced energy storage applications.Dielectric ceramics are widely used in advanced high/pulsed power capacitors. Here, the authors propose a high-entropy strategy to design “local polymorphic distortion” in lead-free ceramics, achieving high energy storage performance. Next-generation advanced high/pulsed power capacitors rely heavily on dielectric ceramics with high energy storage performance. However, thus far, the huge challenge of realizing ultrahigh recoverable energy storage density ( W rec ) accompanied by ultrahigh efficiency ( η ) still existed and has become a key bottleneck restricting the development of dielectric materials in cutting-edge energy storage applications. Here, we propose a high-entropy strategy to design “local polymorphic distortion” including rhombohedral-orthorhombic-tetragonal-cubic multiphase nanoclusters and random oxygen octahedral tilt, resulting in ultrasmall polar nanoregions, an enhanced breakdown electric field, and delayed polarization saturation. A giant W rec ~10.06 J cm −3 is realized in lead-free relaxor ferroelectrics, especially with an ultrahigh η ~90.8%, showing breakthrough progress in the comprehensive energy storage performance for lead-free bulk ceramics. This work opens up an effective avenue to design dielectric materials with ultrahigh comprehensive energy storage performance to meet the demanding requirements of advanced energy storage applications. |
| ArticleNumber | 3089 |
| Author | Deng, Shiqing Chen, Jun Liu, Hui Chen, Liang Wu, Jie Qi, He |
| Author_xml | – sequence: 1 givenname: Liang surname: Chen fullname: Chen, Liang organization: Beijing Advanced Innovation Center for Materials Genome Engineering, University of Science and Technology Beijing, Department of Physical Chemistry, University of Science and Technology Beijing – sequence: 2 givenname: Shiqing surname: Deng fullname: Deng, Shiqing organization: Beijing Advanced Innovation Center for Materials Genome Engineering, University of Science and Technology Beijing, School of Mathematics and Physics, University of Science and Technology Beijing – sequence: 3 givenname: Hui surname: Liu fullname: Liu, Hui organization: Beijing Advanced Innovation Center for Materials Genome Engineering, University of Science and Technology Beijing, School of Mathematics and Physics, University of Science and Technology Beijing – sequence: 4 givenname: Jie surname: Wu fullname: Wu, Jie organization: School of Mathematics and Physics, University of Science and Technology Beijing – sequence: 5 givenname: He orcidid: 0000-0002-3094-3574 surname: Qi fullname: Qi, He email: qiheustb@ustb.edu.cn organization: Beijing Advanced Innovation Center for Materials Genome Engineering, University of Science and Technology Beijing, Department of Physical Chemistry, University of Science and Technology Beijing – sequence: 6 givenname: Jun orcidid: 0000-0002-7330-8976 surname: Chen fullname: Chen, Jun email: junchen@ustb.edu.cn organization: Beijing Advanced Innovation Center for Materials Genome Engineering, University of Science and Technology Beijing, Department of Physical Chemistry, University of Science and Technology Beijing |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/35654831$$D View this record in MEDLINE/PubMed https://www.osti.gov/servlets/purl/1879729$$D View this record in Osti.gov |
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| Snippet | Next-generation advanced high/pulsed power capacitors rely heavily on dielectric ceramics with high energy storage performance. However, thus far, the huge... Next-generation advanced high/pulsed power capacitors rely heavily on dielectric ceramics with high energy storage performance. However, thus far, the huge... Dielectric ceramics are widely used in advanced high/pulsed power capacitors. Here, the authors propose a high-entropy strategy to design “local polymorphic... |
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| SubjectTerms | 140/133 147/135 147/137 147/143 639/301/1023/1024 639/301/119/996 639/301/299 639/4077/4079/4105 Capacitors Ceramics Density Design Dielectrics Distortion Electric fields ENERGY STORAGE Entropy Ferroelectric materials Ferroelectricity ferroelectrics and multiferroics Humanities and Social Sciences Lead free materials for energy and catalysis multidisciplinary Nanoclusters Relaxors Science Science (multidisciplinary) supercapacitors |
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| Title | Giant energy-storage density with ultrahigh efficiency in lead-free relaxors via high-entropy design |
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