Fabrication of All-Water-Based Self-Repairing Superhydrophobic Coatings Based on UV-Responsive Microcapsules

Superhydrophobic coatings that are also self‐healing have drawn much attention in recent years for improved durability in practical applications. Typically, the release of the self‐healing agents is triggered by temperature and moisture change. In this study, UV‐responsive microcapsules are successf...

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Published in	Advanced functional materials Vol. 25; no. 7; pp. 1035 - 1041
Main Authors	Chen, Kunlin, Zhou, Shuxue, Yang, Shu, Wu, Limin
Format	Journal Article
Language	English
Published	Blackwell Publishing Ltd 18.02.2015
Subjects	Coatings Contamination Damage Nanoparticles Outdoor Self healing materials self-repairing Silicon dioxide superhydrophobic coatings Titanium dioxide UV-responsive microcapsules waterborne
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Abstract	Superhydrophobic coatings that are also self‐healing have drawn much attention in recent years for improved durability in practical applications. Typically, the release of the self‐healing agents is triggered by temperature and moisture change. In this study, UV‐responsive microcapsules are successfully synthesized by Pickering emulsion polymerization using titania (TiO2) and silica (SiO2) nanoparticles as the Pickering agents to fabricate all‐water‐based self‐repairing, superhydrophobic coatings. These coatings are environmentally friendly and can be readily coated on various substrates. Compared to conventional superhydrophobic coatings, these coatings can regenerate superhydrophobicity and self‐cleaning ability under UV light, mimicking the outdoor environment, after they are mechanically damaged or contaminated with organics. They can maintain the superhydrophobicity after multiple cycles of accelerated weathering tests. An environmentally benign, all‐water‐based self‐repairing superhydrophobic coating based on UV‐responsive microcapsules is fabricated, which exhibits excellent self‐healing and self‐cleaning ability in an outdoor environment, and after mechanical damage and contamination by organics.
AbstractList	Superhydrophobic coatings that are also self‐healing have drawn much attention in recent years for improved durability in practical applications. Typically, the release of the self‐healing agents is triggered by temperature and moisture change. In this study, UV‐responsive microcapsules are successfully synthesized by Pickering emulsion polymerization using titania (TiO 2 ) and silica (SiO 2 ) nanoparticles as the Pickering agents to fabricate all‐water‐based self‐repairing, superhydrophobic coatings. These coatings are environmentally friendly and can be readily coated on various substrates. Compared to conventional superhydrophobic coatings, these coatings can regenerate superhydrophobicity and self‐cleaning ability under UV light, mimicking the outdoor environment, after they are mechanically damaged or contaminated with organics. They can maintain the superhydrophobicity after multiple cycles of accelerated weathering tests. Superhydrophobic coatings that are also self-healing have drawn much attention in recent years for improved durability in practical applications. Typically, the release of the self-healing agents is triggered by temperature and moisture change. In this study, UV-responsive microcapsules are successfully synthesized by Pickering emulsion polymerization using titania (TiO sub(2)) and silica (SiO sub(2)) nanoparticles as the Pickering agents to fabricate all-water-based self-repairing, superhydrophobic coatings. These coatings are environmentally friendly and can be readily coated on various substrates. Compared to conventional superhydrophobic coatings, these coatings can regenerate superhydrophobicity and self-cleaning ability under UV light, mimicking the outdoor environment, after they are mechanically damaged or contaminated with organics. They can maintain the superhydrophobicity after multiple cycles of accelerated weathering tests. An environmentally benign, all-water-based self-repairing superhydrophobic coating based on UV-responsive microcapsules is fabricated, which exhibits excellent self-healing and self-cleaning ability in an outdoor environment, and after mechanical damage and contamination by organics. Superhydrophobic coatings that are also self‐healing have drawn much attention in recent years for improved durability in practical applications. Typically, the release of the self‐healing agents is triggered by temperature and moisture change. In this study, UV‐responsive microcapsules are successfully synthesized by Pickering emulsion polymerization using titania (TiO2) and silica (SiO2) nanoparticles as the Pickering agents to fabricate all‐water‐based self‐repairing, superhydrophobic coatings. These coatings are environmentally friendly and can be readily coated on various substrates. Compared to conventional superhydrophobic coatings, these coatings can regenerate superhydrophobicity and self‐cleaning ability under UV light, mimicking the outdoor environment, after they are mechanically damaged or contaminated with organics. They can maintain the superhydrophobicity after multiple cycles of accelerated weathering tests. An environmentally benign, all‐water‐based self‐repairing superhydrophobic coating based on UV‐responsive microcapsules is fabricated, which exhibits excellent self‐healing and self‐cleaning ability in an outdoor environment, and after mechanical damage and contamination by organics.
Author	Zhou, Shuxue Yang, Shu Wu, Limin Chen, Kunlin
Author_xml	– sequence: 1 givenname: Kunlin surname: Chen fullname: Chen, Kunlin organization: Department of Materials Science and State Key Laboratory of Molecular Engineering of Polymers, Advanced Coatings Research Center of Ministry of Education of China, Fudan University, 200433, Shanghai, China – sequence: 2 givenname: Shuxue surname: Zhou fullname: Zhou, Shuxue email: zhoushuxue@fudan.edu.cn organization: Department of Materials Science and State Key Laboratory of Molecular Engineering of Polymers, Advanced Coatings Research Center of Ministry of Education of China, Fudan University, 200433, Shanghai, China – sequence: 3 givenname: Shu surname: Yang fullname: Yang, Shu organization: Department of Materials Science and Engineering, University of Pennsylvania, 3231 Walnut Street, PA, 19104, Philadelphia, USA – sequence: 4 givenname: Limin surname: Wu fullname: Wu, Limin email: zhoushuxue@fudan.edu.cn organization: Department of Materials Science and State Key Laboratory of Molecular Engineering of Polymers, Advanced Coatings Research Center of Ministry of Education of China, Fudan University, 200433, Shanghai, China
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Snippet	Superhydrophobic coatings that are also self‐healing have drawn much attention in recent years for improved durability in practical applications. Typically,... Superhydrophobic coatings that are also self-healing have drawn much attention in recent years for improved durability in practical applications. Typically,...
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SubjectTerms	Coatings Contamination Damage Nanoparticles Outdoor Self healing materials self-repairing Silicon dioxide superhydrophobic coatings Titanium dioxide UV-responsive microcapsules waterborne
Title	Fabrication of All-Water-Based Self-Repairing Superhydrophobic Coatings Based on UV-Responsive Microcapsules
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