Decolorization of an azo dye Orange G in aqueous solution by Fenton oxidation process: Effect of system parameters and kinetic study
To establish cost-efficient operating conditions for potential application of Fenton oxidation process to treat wastewater containing an azo dye Orange G (OG), some important operating parameters such as pH value of solutions, dosages of H 2O 2 and Fe 2+, temperature, presence/absence of chloride io...
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| Published in | Journal of hazardous materials Vol. 161; no. 2; pp. 1052 - 1057 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Kidlington
Elsevier B.V
30.01.2009
Elsevier |
| Subjects | |
| Online Access | Get full text |
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| Abstract | To establish cost-efficient operating conditions for potential application of Fenton oxidation process to treat wastewater containing an azo dye Orange G (OG), some important operating parameters such as pH value of solutions, dosages of H
2O
2 and Fe
2+, temperature, presence/absence of chloride ion and concentration of the dye, which effect on the decolorization of OG in aqueous solution by Fenton oxidation have been investigated systematically. In addition, the decolorization kinetics of OG was also elucidated based on the experimental data. The results showed that a suitable decolorization condition was selected as initial pH 4.0, H
2O
2 dosage 1.0
×
10
−2
M and molar ratio of [H
2O
2]/[Fe
2+] 286:1. The decolorization of OG enhanced with the increasing of reaction temperature but decreased as a presence of chloride ion. On the given conditions, for 2.21
×
10
−5 to 1.11
×
10
−4
M of OG, the decolorization efficiencies within 60
min were more than 94.6%. The decolorization kinetics of OG by Fenton oxidation process followed the second-order reaction kinetics, and the apparent activation energy
E, was detected to be 34.84
kJ
mol
−1. The results can provide fundamental knowledge for the treatment of wastewater containing OG and/or other azo dyes by Fenton oxidation process. |
|---|---|
| AbstractList | To establish cost-efficient operating conditions for potential application of Fenton oxidation process to treat wastewater containing an azo dye Orange G (OG), some important operating parameters such as pH value of solutions, dosages of H sub(2)O sub(2) and Fe super(2) super(+), temperature, presence/absence of chloride ion and concentration of the dye, which effect on the decolorization of OG in aqueous solution by Fenton oxidation have been investigated systematically. In addition, the decolorization kinetics of OG was also elucidated based on the experimental data. The results showed that a suitable decolorization condition was selected as initial pH 4.0, H sub(2)O sub(2) dosage 1.0x10 super(-) super(2)M and molar ratio of [H sub(2)O sub(2)] /[Fe super(2) super(+)] 286:1. The decolorization of OG enhanced with the increasing of reaction temperature but decreased as a presence of chloride ion. On the given conditions, for 2.21x10 super(-) super(5) to 1.11x10 super(-) super(4)M of OG, the decolorization efficiencies within 60min were more than 94.6%. The decolorization kinetics of OG by Fenton oxidation process followed the second-order reaction kinetics, and the apparent activation energy E, was detected to be 34.84kJmol super(-) super(1). The results can provide fundamental knowledge for the treatment of wastewater containing OG and/or other azo dyes by Fenton oxidation process. To establish cost-efficient operating conditions for potential application of Fenton oxidation process to treat wastewater containing an azo dye Orange G (OG), some important operating parameters such as pH value of solutions, dosages of H(2)O(2) and Fe(2+), temperature, presence/absence of chloride ion and concentration of the dye, which effect on the decolorization of OG in aqueous solution by Fenton oxidation have been investigated systematically. In addition, the decolorization kinetics of OG was also elucidated based on the experimental data. The results showed that a suitable decolorization condition was selected as initial pH 4.0, H(2)O(2) dosage 1.0 x 10(-2)M and molar ratio of [H(2)O(2)]/[Fe(2+)] 286:1. The decolorization of OG enhanced with the increasing of reaction temperature but decreased as a presence of chloride ion. On the given conditions, for 2.21 x 10(-5) to 1.11 x 10(-4)M of OG, the decolorization efficiencies within 60 min were more than 94.6%. The decolorization kinetics of OG by Fenton oxidation process followed the second-order reaction kinetics, and the apparent activation energy E, was detected to be 34.84 kJ mol(-1). The results can provide fundamental knowledge for the treatment of wastewater containing OG and/or other azo dyes by Fenton oxidation process.To establish cost-efficient operating conditions for potential application of Fenton oxidation process to treat wastewater containing an azo dye Orange G (OG), some important operating parameters such as pH value of solutions, dosages of H(2)O(2) and Fe(2+), temperature, presence/absence of chloride ion and concentration of the dye, which effect on the decolorization of OG in aqueous solution by Fenton oxidation have been investigated systematically. In addition, the decolorization kinetics of OG was also elucidated based on the experimental data. The results showed that a suitable decolorization condition was selected as initial pH 4.0, H(2)O(2) dosage 1.0 x 10(-2)M and molar ratio of [H(2)O(2)]/[Fe(2+)] 286:1. The decolorization of OG enhanced with the increasing of reaction temperature but decreased as a presence of chloride ion. On the given conditions, for 2.21 x 10(-5) to 1.11 x 10(-4)M of OG, the decolorization efficiencies within 60 min were more than 94.6%. The decolorization kinetics of OG by Fenton oxidation process followed the second-order reaction kinetics, and the apparent activation energy E, was detected to be 34.84 kJ mol(-1). The results can provide fundamental knowledge for the treatment of wastewater containing OG and/or other azo dyes by Fenton oxidation process. To establish cost-efficient operating conditions for potential application of Fenton oxidation process to treat wastewater containing an azo dye Orange G (OG), some important operating parameters such as pH value of solutions, dosages of H2O2 and Fe2+, temperature, presence/absence of chloride ion and concentration of the dye, which effect on the decolorization of OG in aqueous solution by Fenton oxidation have been investigated systematically. In addition, the decolorization kinetics of OG was also elucidated based on the experimental data. The results showed that a suitable decolorization condition was selected as initial pH 4.0, H2O2 dosage 1.0 X 10-2 M and molar ratio of [H2O2]/[Fe2+] 286:1. The decolorization of OG enhanced with the increasing of reaction temperature but decreased as a presence of chloride ion. On the given conditions, for 2.21 X 10-5 to 1.11 X 10-4 M of OG, the decolorization efficiencies within 60 min were more than 94.6%. The decolorization kinetics of OG by Fenton oxidation process followed the second-order reaction kinetics, and the apparent activation energy E, was detected to be 34.84 kJ mol-1. The results can provide fundamental knowledge for the treatment of wastewater containing OG and/or other azo dyes by Fenton oxidation process. To establish cost-efficient operating conditions for potential application of Fenton oxidation process to treat wastewater containing an azo dye Orange G (OG), some important operating parameters such as pH value of solutions, dosages of H(2)O(2) and Fe(2+), temperature, presence/absence of chloride ion and concentration of the dye, which effect on the decolorization of OG in aqueous solution by Fenton oxidation have been investigated systematically. In addition, the decolorization kinetics of OG was also elucidated based on the experimental data. The results showed that a suitable decolorization condition was selected as initial pH 4.0, H(2)O(2) dosage 1.0 x 10(-2)M and molar ratio of [H(2)O(2)]/[Fe(2+)] 286:1. The decolorization of OG enhanced with the increasing of reaction temperature but decreased as a presence of chloride ion. On the given conditions, for 2.21 x 10(-5) to 1.11 x 10(-4)M of OG, the decolorization efficiencies within 60 min were more than 94.6%. The decolorization kinetics of OG by Fenton oxidation process followed the second-order reaction kinetics, and the apparent activation energy E, was detected to be 34.84 kJ mol(-1). The results can provide fundamental knowledge for the treatment of wastewater containing OG and/or other azo dyes by Fenton oxidation process. To establish cost-efficient operating conditions for potential application of Fenton oxidation process to treat wastewater containing an azo dye Orange G (OG), some important operating parameters such as pH value of solutions, dosages of H 2O 2 and Fe 2+, temperature, presence/absence of chloride ion and concentration of the dye, which effect on the decolorization of OG in aqueous solution by Fenton oxidation have been investigated systematically. In addition, the decolorization kinetics of OG was also elucidated based on the experimental data. The results showed that a suitable decolorization condition was selected as initial pH 4.0, H 2O 2 dosage 1.0 × 10 −2 M and molar ratio of [H 2O 2]/[Fe 2+] 286:1. The decolorization of OG enhanced with the increasing of reaction temperature but decreased as a presence of chloride ion. On the given conditions, for 2.21 × 10 −5 to 1.11 × 10 −4 M of OG, the decolorization efficiencies within 60 min were more than 94.6%. The decolorization kinetics of OG by Fenton oxidation process followed the second-order reaction kinetics, and the apparent activation energy E, was detected to be 34.84 kJ mol −1. The results can provide fundamental knowledge for the treatment of wastewater containing OG and/or other azo dyes by Fenton oxidation process. |
| Author | Shi, Shao-Hui Zhou, Qi Sun, Sheng-Peng Fan, Mao-Hong Sun, Jian-Hui Li, Cheng-Jie |
| Author_xml | – sequence: 1 givenname: Sheng-Peng surname: Sun fullname: Sun, Sheng-Peng organization: State Key Laboratory of Pollution Control and Resources Reuse, College of Environmental Science and Engineering, Tongji University, Shanghai 200092, PR China – sequence: 2 givenname: Cheng-Jie surname: Li fullname: Li, Cheng-Jie organization: School of Resources and Environment, Henan Polytechnic University, Jiaozuo, Henan 454000, PR China – sequence: 3 givenname: Jian-Hui surname: Sun fullname: Sun, Jian-Hui email: sunsp_hj@yahoo.com.cn organization: Henan Key Laboratory for Environmental Pollution Control, College of Chemistry and Environmental Sciences, Henan Normal University, Xinxiang, Henan 453007, PR China – sequence: 4 givenname: Shao-Hui surname: Shi fullname: Shi, Shao-Hui organization: Henan Key Laboratory for Environmental Pollution Control, College of Chemistry and Environmental Sciences, Henan Normal University, Xinxiang, Henan 453007, PR China – sequence: 5 givenname: Mao-Hong surname: Fan fullname: Fan, Mao-Hong organization: School of Materials Science and Engineering, Georgia Institute of Technology, Atlanta, GA 30332, USA – sequence: 6 givenname: Qi surname: Zhou fullname: Zhou, Qi organization: State Key Laboratory of Pollution Control and Resources Reuse, College of Environmental Science and Engineering, Tongji University, Shanghai 200092, PR China |
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| Keywords | Fenton's reaction Orange G Kinetic Azo dye Hydroxyl radical Second order Discoloration Hydrogen peroxide Operating conditions Waste water Chlorides Hydroxyl radicals pH Fenton reaction Physicochemical purification Oxidation Kinetics Aqueous solution Thermodynamic properties Activation energy |
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| SubjectTerms | Applied sciences Azo Compounds - chemistry Azo dye Chemical engineering Chlorides - chemistry Coloring Agents - chemistry Exact sciences and technology Fenton's reaction General purification processes Hydrogen Peroxide - chemistry Hydrogen-Ion Concentration Hydroxyl radical Ions Iron - chemistry Kinetic Kinetics Models, Chemical Orange G Oxygen - chemistry Pollution Pressure Reactors Spectrophotometry, Ultraviolet Temperature Time Factors Wastewaters Water treatment and pollution |
| Title | Decolorization of an azo dye Orange G in aqueous solution by Fenton oxidation process: Effect of system parameters and kinetic study |
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