Strain engineering in alloy nanoparticles
The deformation of interatomic distances with respect to those of the perfect crystal generates atomic-level strain. In nanoalloys, strain can arise because of finite size, morphology, domain structure and lattice mismatch between their atomic compounds. Strain can strongly affect the functional pro...
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| Published in | Advances in physics: X Vol. 8; no. 1 |
|---|---|
| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
Abingdon
Taylor & Francis
31.12.2023
Taylor & Francis Ltd Taylor & Francis Group |
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| Online Access | Get full text |
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| Abstract | The deformation of interatomic distances with respect to those of the perfect crystal generates atomic-level strain. In nanoalloys, strain can arise because of finite size, morphology, domain structure and lattice mismatch between their atomic compounds. Strain can strongly affect the functional properties of nanoalloys, as it alters their electronic energy levels. Moreover, atomic-level strain generates atomic-level stress, which in turn results in distortions induced by strain. When the stress accumulated in a nanoalloy exceeds a certain level, the particle can relax that stress by undergoing structural transitions such as shape and/or chemical ordering transitions. Atomic-level strain is then a powerful tool to control and manipulate the structural and functional properties of nanoalloys. This requires a combined theoretical and experimental approach both to deeply understand the physical origin of strain, and to characterize it with a sub-angstrom resolution. Here, we present a theoretical analysis of the main sources of strain in nanoalloys, we analyse how atomic-level strain can be experimentally measured with transmission electron microscopy, we discuss its effect on the functional properties of nanoalloys, finally we describe how atomic-level stress arises from atomic-level strain, and how stress can induce structural transformations at the nanoscale. |
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| AbstractList | The deformation of interatomic distances with respect to those of the perfect crystal generates atomic-level strain. In nanoalloys, strain can arise because of finite size, morphology, domain structure and lattice mismatch between their atomic compounds. Strain can strongly affect the functional properties of nanoalloys, as it alters their electronic energy levels. Moreover, atomic-level strain generates atomic-level stress, which in turn results in distortions induced by strain. When the stress accumulated in a nanoalloy exceeds a certain level, the particle can relax that stress by undergoing structural transitions such as shape and/or chemical ordering transitions. Atomic-level strain is then a powerful tool to control and manipulate the structural and functional properties of nanoalloys. This requires a combined theoretical and experimental approach both to deeply understand the physical origin of strain, and to characterize it with a sub-angstrom resolution. Here, we present a theoretical analysis of the main sources of strain in nanoalloys, we analyse how atomic-level strain can be experimentally measured with transmission electron microscopy, we discuss its effect on the functional properties of nanoalloys, finally we describe how atomic-level stress arises from atomic-level strain, and how stress can induce structural transformations at the nanoscale. ABSTRACTThe deformation of interatomic distances with respect to those of the perfect crystal generates atomic-level strain. In nanoalloys, strain can arise because of finite size, morphology, domain structure and lattice mismatch between their atomic compounds. Strain can strongly affect the functional properties of nanoalloys, as it alters their electronic energy levels. Moreover, atomic-level strain generates atomic-level stress, which in turn results in distortions induced by strain. When the stress accumulated in a nanoalloy exceeds a certain level, the particle can relax that stress by undergoing structural transitions such as shape and/or chemical ordering transitions. Atomic-level strain is then a powerful tool to control and manipulate the structural and functional properties of nanoalloys. This requires a combined theoretical and experimental approach both to deeply understand the physical origin of strain, and to characterize it with a sub-angstrom resolution. Here, we present a theoretical analysis of the main sources of strain in nanoalloys, we analyse how atomic-level strain can be experimentally measured with transmission electron microscopy, we discuss its effect on the functional properties of nanoalloys, finally we describe how atomic-level stress arises from atomic-level strain, and how stress can induce structural transformations at the nanoscale. |
| Author | Nelli, Diana Minnai, Chloé Roncaglia, Cesare |
| Author_xml | – sequence: 1 givenname: Diana surname: Nelli fullname: Nelli, Diana email: diana.nelli@edu.unige.it organization: University of Genoa – sequence: 2 givenname: Cesare surname: Roncaglia fullname: Roncaglia, Cesare organization: University of Genoa – sequence: 3 givenname: Chloé surname: Minnai fullname: Minnai, Chloé email: chloe.minnai@oist.jp organization: Okinawa Institute of Science and Technology Graduate University |
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| Snippet | The deformation of interatomic distances with respect to those of the perfect crystal generates atomic-level strain. In nanoalloys, strain can arise because of... ABSTRACTThe deformation of interatomic distances with respect to those of the perfect crystal generates atomic-level strain. In nanoalloys, strain can arise... |
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| SubjectTerms | atomistic simulations Deformation Electrons Energy levels Engineering HRTEM lattice mismatch Nanoalloys Nanoparticles Strain strain engineering stress Transmission electron microscopy |
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| Title | Strain engineering in alloy nanoparticles |
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