Electrochemical Preparation of Nanocatalysts and Their Application in Electrocatalysis
In order to solve the basic problem of high-temperature sintering of molybdenum carbide restricting the efficient construction of molybdenum carbide nanostructures and the full play of hydrogen evolution performance, this article studies the preparation of nano molybdenum carbide/boron nitrogen codo...
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| Published in | International journal of analytical chemistry Vol. 2022; pp. 1 - 6 |
|---|---|
| Main Author | |
| Format | Journal Article |
| Language | English |
| Published |
New York
Hindawi
27.08.2022
John Wiley & Sons, Inc Wiley |
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| Online Access | Get full text |
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| Abstract | In order to solve the basic problem of high-temperature sintering of molybdenum carbide restricting the efficient construction of molybdenum carbide nanostructures and the full play of hydrogen evolution performance, this article studies the preparation of nano molybdenum carbide/boron nitrogen codoped two-dimensional carbon composite structure catalysts and the electrochemical hydrogen evolution reaction performance. Based on the self-assembly process of gelatin molecules on the surface of a two-dimensional layered boric acid crystal template, a new strategy for constructing a high-performance electrochemical hydrogen evolution reaction catalyst based on molybdenum carbide/boron nitrogen codoped two-dimensional nanocarbon composite structure (η-MoC@ BN-CSs) was established. The experimental results show that the overpotential of hydrogen evolution reaction based on molybdenum carbide/boron nitrogen codoped two-dimensional nanocarbon composite structure catalyst is 159 mV, which is slightly higher than 67 mV of commercial Pt/C catalyst, but lower than the reported literature value in the list. The Tafel slope is 68 mV·dec−1, which is slightly higher than that of the commercial Pt/C catalyst (40 mV·dec−1) and the reference value (58 mV·dec−1), but lower than those of other reported literature values in the list, indicating that the molybdenum carbide/boron nitrogen codoped two-dimensional carbon nanocomposites have excellent catalytic performance under alkaline conditions. Conclusion. This kind of two-dimensional nanocomposite structure shows platinum-like catalytic activity when used as an electrochemical hydrogen evolution catalyst in alkaline electrolyte. It has better reaction kinetics and better stability. |
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| AbstractList | In order to solve the basic problem of high-temperature sintering of molybdenum carbide restricting the efficient construction of molybdenum carbide nanostructures and the full play of hydrogen evolution performance, this article studies the preparation of nano molybdenum carbide/boron nitrogen codoped two-dimensional carbon composite structure catalysts and the electrochemical hydrogen evolution reaction performance. Based on the self-assembly process of gelatin molecules on the surface of a two-dimensional layered boric acid crystal template, a new strategy for constructing a high-performance electrochemical hydrogen evolution reaction catalyst based on molybdenum carbide/boron nitrogen codoped two-dimensional nanocarbon composite structure (η-MoC@ BN-CSs) was established. The experimental results show that the overpotential of hydrogen evolution reaction based on molybdenum carbide/boron nitrogen codoped two-dimensional nanocarbon composite structure catalyst is 159 mV, which is slightly higher than 67 mV of commercial Pt/C catalyst, but lower than the reported literature value in the list. The Tafel slope is 68 mV·dec−1, which is slightly higher than that of the commercial Pt/C catalyst (40 mV·dec−1) and the reference value (58 mV·dec−1), but lower than those of other reported literature values in the list, indicating that the molybdenum carbide/boron nitrogen codoped two-dimensional carbon nanocomposites have excellent catalytic performance under alkaline conditions. Conclusion. This kind of two-dimensional nanocomposite structure shows platinum-like catalytic activity when used as an electrochemical hydrogen evolution catalyst in alkaline electrolyte. It has better reaction kinetics and better stability. In order to solve the basic problem of high-temperature sintering of molybdenum carbide restricting the efficient construction of molybdenum carbide nanostructures and the full play of hydrogen evolution performance, this article studies the preparation of nano molybdenum carbide/boron nitrogen codoped two-dimensional carbon composite structure catalysts and the electrochemical hydrogen evolution reaction performance. Based on the self-assembly process of gelatin molecules on the surface of a two-dimensional layered boric acid crystal template, a new strategy for constructing a high-performance electrochemical hydrogen evolution reaction catalyst based on molybdenum carbide/boron nitrogen codoped two-dimensional nanocarbon composite structure ( η -MoC@ BN-CSs) was established. The experimental results show that the overpotential of hydrogen evolution reaction based on molybdenum carbide/boron nitrogen codoped two-dimensional nanocarbon composite structure catalyst is 159 mV, which is slightly higher than 67 mV of commercial Pt/C catalyst, but lower than the reported literature value in the list. The Tafel slope is 68 mV·dec −1 , which is slightly higher than that of the commercial Pt/C catalyst (40 mV·dec −1 ) and the reference value (58 mV·dec −1 ), but lower than those of other reported literature values in the list, indicating that the molybdenum carbide/boron nitrogen codoped two-dimensional carbon nanocomposites have excellent catalytic performance under alkaline conditions. Conclusion . This kind of two-dimensional nanocomposite structure shows platinum-like catalytic activity when used as an electrochemical hydrogen evolution catalyst in alkaline electrolyte. It has better reaction kinetics and better stability. In order to solve the basic problem of high-temperature sintering of molybdenum carbide restricting the efficient construction of molybdenum carbide nanostructures and the full play of hydrogen evolution performance, this article studies the preparation of nano molybdenum carbide/boron nitrogen codoped two-dimensional carbon composite structure catalysts and the electrochemical hydrogen evolution reaction performance. Based on the self-assembly process of gelatin molecules on the surface of a two-dimensional layered boric acid crystal template, a new strategy for constructing a high-performance electrochemical hydrogen evolution reaction catalyst based on molybdenum carbide/boron nitrogen codoped two-dimensional nanocarbon composite structure (η-MoC@ BN-CSs) was established. The experimental results show that the overpotential of hydrogen evolution reaction based on molybdenum carbide/boron nitrogen codoped two-dimensional nanocarbon composite structure catalyst is 159 mV, which is slightly higher than 67 mV of commercial Pt/C catalyst, but lower than the reported literature value in the list. The Tafel slope is 68 mV·dec-1, which is slightly higher than that of the commercial Pt/C catalyst (40 mV·dec-1) and the reference value (58 mV·dec-1), but lower than those of other reported literature values in the list, indicating that the molybdenum carbide/boron nitrogen codoped two-dimensional carbon nanocomposites have excellent catalytic performance under alkaline conditions. Conclusion. This kind of two-dimensional nanocomposite structure shows platinum-like catalytic activity when used as an electrochemical hydrogen evolution catalyst in alkaline electrolyte. It has better reaction kinetics and better stability.In order to solve the basic problem of high-temperature sintering of molybdenum carbide restricting the efficient construction of molybdenum carbide nanostructures and the full play of hydrogen evolution performance, this article studies the preparation of nano molybdenum carbide/boron nitrogen codoped two-dimensional carbon composite structure catalysts and the electrochemical hydrogen evolution reaction performance. Based on the self-assembly process of gelatin molecules on the surface of a two-dimensional layered boric acid crystal template, a new strategy for constructing a high-performance electrochemical hydrogen evolution reaction catalyst based on molybdenum carbide/boron nitrogen codoped two-dimensional nanocarbon composite structure (η-MoC@ BN-CSs) was established. The experimental results show that the overpotential of hydrogen evolution reaction based on molybdenum carbide/boron nitrogen codoped two-dimensional nanocarbon composite structure catalyst is 159 mV, which is slightly higher than 67 mV of commercial Pt/C catalyst, but lower than the reported literature value in the list. The Tafel slope is 68 mV·dec-1, which is slightly higher than that of the commercial Pt/C catalyst (40 mV·dec-1) and the reference value (58 mV·dec-1), but lower than those of other reported literature values in the list, indicating that the molybdenum carbide/boron nitrogen codoped two-dimensional carbon nanocomposites have excellent catalytic performance under alkaline conditions. Conclusion. This kind of two-dimensional nanocomposite structure shows platinum-like catalytic activity when used as an electrochemical hydrogen evolution catalyst in alkaline electrolyte. It has better reaction kinetics and better stability. In order to solve the basic problem of high-temperature sintering of molybdenum carbide restricting the efficient construction of molybdenum carbide nanostructures and the full play of hydrogen evolution performance, this article studies the preparation of nano molybdenum carbide/boron nitrogen codoped two-dimensional carbon composite structure catalysts and the electrochemical hydrogen evolution reaction performance. Based on the self-assembly process of gelatin molecules on the surface of a two-dimensional layered boric acid crystal template, a new strategy for constructing a high-performance electrochemical hydrogen evolution reaction catalyst based on molybdenum carbide/boron nitrogen codoped two-dimensional nanocarbon composite structure (η -MoC@ BN-CSs) was established. The experimental results show that the overpotential of hydrogen evolution reaction based on molybdenum carbide/boron nitrogen codoped two-dimensional nanocarbon composite structure catalyst is 159mV, which is slightly higher than 67mV of commercial Pt/C catalyst, but lower than the reported literature value in the list. The Tafel slope is 68mV·dec[sup.-1], which is slightly higher than that of the commercial Pt/C catalyst (40mV·dec[sup.-1]) and the reference value (58mV·dec[sup.-1]), but lower than those of other reported literature values in the list, indicating that the molybdenum carbide/boron nitrogen codoped two-dimensional carbon nanocomposites have excellent catalytic performance under alkaline conditions. Conclusion. This kind of two-dimensional nanocomposite structure shows platinum-like catalytic activity when used as an electrochemical hydrogen evolution catalyst in alkaline electrolyte. It has better reaction kinetics and better stability. |
| Audience | Academic |
| Author | Zhou, Hao |
| AuthorAffiliation | JiangSu Vocational College of Business, NanTong 226011, JiangSu, China |
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| CitedBy_id | crossref_primary_10_1155_2023_9867946 crossref_primary_10_1080_15435075_2024_2396070 |
| Cites_doi | 10.1016/j.ijhydene.2020.07.174 10.4028/www.scientific.net/msf.979.89 10.1016/j.matlet.2019.126819 10.1039/c9ra09661b 10.1016/s1002-0721(14)60086-7 10.1155/2021/5325116 10.1016/j.carbon.2020.01.098 10.1016/j.ijhydene.2019.10.241 10.1016/j.jcat.2020.02.020 10.1108/ijicc-10-2020-0142 10.4028/www.scientific.net/msf.1004.265 10.1037/xlm0000987 10.1016/j.scitotenv.2019.135104 10.1016/j.carbon.2020.09.037 10.1007/s12274-020-3156-3 10.1021/acscatal.0c05634 10.1021/acs.jpcc.0c07968 |
| ContentType | Journal Article |
| Copyright | Copyright © 2022 Hao Zhou. COPYRIGHT 2022 John Wiley & Sons, Inc. Copyright © 2022 Hao Zhou. This is an open access article distributed under the Creative Commons Attribution License (the “License”), which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited. Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License. https://creativecommons.org/licenses/by/4.0 Copyright © 2022 Hao Zhou. 2022 |
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| DOI | 10.1155/2022/9884302 |
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| SubjectTerms | Alternative energy sources Amino acids Analytical chemistry Boric acid Boron Carbon Catalysts Catalytic activity Chemical reaction, Rate of Clean technology Composite structures Electric properties Electrodes Electrolytes Electron microscopes Gelatin High temperature Hydrogen Hydrogen evolution reactions Molybdenum Molybdenum carbide Nanocomposites Nanoparticles Nanowires Nitrogen Platinum Precious metals Reaction kinetics Self-assembly |
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| Title | Electrochemical Preparation of Nanocatalysts and Their Application in Electrocatalysis |
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