Tracking Regulatory Mechanism of Trace Fe on Graphene Electromagnetic Wave Absorption
Highlights A carrier injection strategy is firstly proposed by designing Fe/reduced graphene oxide (RGO) heterogeneous interfacial material for giving full play to the dielectric dispersion properties of graphene. The electromagnetic wave absorption mechanisms mainly include enhanced conductance los...
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| Published in | Nano-micro letters Vol. 16; no. 1; pp. 66 - 18 |
|---|---|
| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Singapore
Springer Nature Singapore
01.12.2024
Springer Nature B.V SpringerOpen |
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| Abstract | Highlights
A carrier injection strategy is firstly proposed by designing Fe/reduced graphene oxide (RGO) heterogeneous interfacial material for giving full play to the dielectric dispersion properties of graphene.
The electromagnetic wave absorption mechanisms mainly include enhanced conductance loss, dipole polarization and interfacial polarization.
Outstanding reflection loss value (− 53.38 dB, 2.45 mm) and broadband wave absorption (7.52 GHz with only 2 wt% filling) of Fe/RGO composite were acquired, which is superior to single-component graphene.
Polarization and conductance losses are the fundamental dielectric attenuation mechanisms for graphene-based absorbers, but it is not fully understood in revealing the loss mechanism of affect graphene itself. For the first time, the reduced graphene oxide (RGO) based absorbers are developed with regulatory absorption properties and the absorption mechanism of RGO is mainly originated from the carrier injection behavior of trace metal Fe nanosheets on graphene. Accordingly, the minimum reflection loss (RL
min
) of Fe/RGO-2 composite reaches − 53.38 dB (2.45 mm), and the effective absorption bandwidth achieves 7.52 GHz (2.62 mm) with lower filling loading of 2 wt%. Using off-axis electron hologram testing combined with simulation calculation and carrier transport property experiments, we demonstrate here the carrier injection behavior from Fe to graphene at the interface and the induced charge accumulation and rearrangement, resulting in the increased interfacial and dipole polarization and the conductance loss. This work has confirmed that regulating the dielectric property of graphene itself by adding trace metals can not only ensure good impedance matching, but also fully exploit the dielectric loss ability of graphene at low filler content, which opens up an efficient way for designing lightweight absorbers and may be extended to other types materials. |
|---|---|
| AbstractList | Polarization and conductance losses are the fundamental dielectric attenuation mechanisms for graphene-based absorbers, but it is not fully understood in revealing the loss mechanism of affect graphene itself. For the first time, the reduced graphene oxide (RGO) based absorbers are developed with regulatory absorption properties and the absorption mechanism of RGO is mainly originated from the carrier injection behavior of trace metal Fe nanosheets on graphene. Accordingly, the minimum reflection loss (RLmin) of Fe/RGO-2 composite reaches - 53.38 dB (2.45 mm), and the effective absorption bandwidth achieves 7.52 GHz (2.62 mm) with lower filling loading of 2 wt%. Using off-axis electron hologram testing combined with simulation calculation and carrier transport property experiments, we demonstrate here the carrier injection behavior from Fe to graphene at the interface and the induced charge accumulation and rearrangement, resulting in the increased interfacial and dipole polarization and the conductance loss. This work has confirmed that regulating the dielectric property of graphene itself by adding trace metals can not only ensure good impedance matching, but also fully exploit the dielectric loss ability of graphene at low filler content, which opens up an efficient way for designing lightweight absorbers and may be extended to other types materials.Polarization and conductance losses are the fundamental dielectric attenuation mechanisms for graphene-based absorbers, but it is not fully understood in revealing the loss mechanism of affect graphene itself. For the first time, the reduced graphene oxide (RGO) based absorbers are developed with regulatory absorption properties and the absorption mechanism of RGO is mainly originated from the carrier injection behavior of trace metal Fe nanosheets on graphene. Accordingly, the minimum reflection loss (RLmin) of Fe/RGO-2 composite reaches - 53.38 dB (2.45 mm), and the effective absorption bandwidth achieves 7.52 GHz (2.62 mm) with lower filling loading of 2 wt%. Using off-axis electron hologram testing combined with simulation calculation and carrier transport property experiments, we demonstrate here the carrier injection behavior from Fe to graphene at the interface and the induced charge accumulation and rearrangement, resulting in the increased interfacial and dipole polarization and the conductance loss. This work has confirmed that regulating the dielectric property of graphene itself by adding trace metals can not only ensure good impedance matching, but also fully exploit the dielectric loss ability of graphene at low filler content, which opens up an efficient way for designing lightweight absorbers and may be extended to other types materials. Highlights A carrier injection strategy is firstly proposed by designing Fe/reduced graphene oxide (RGO) heterogeneous interfacial material for giving full play to the dielectric dispersion properties of graphene. The electromagnetic wave absorption mechanisms mainly include enhanced conductance loss, dipole polarization and interfacial polarization. Outstanding reflection loss value (− 53.38 dB, 2.45 mm) and broadband wave absorption (7.52 GHz with only 2 wt% filling) of Fe/RGO composite were acquired, which is superior to single-component graphene. Polarization and conductance losses are the fundamental dielectric attenuation mechanisms for graphene-based absorbers, but it is not fully understood in revealing the loss mechanism of affect graphene itself. For the first time, the reduced graphene oxide (RGO) based absorbers are developed with regulatory absorption properties and the absorption mechanism of RGO is mainly originated from the carrier injection behavior of trace metal Fe nanosheets on graphene. Accordingly, the minimum reflection loss (RL min ) of Fe/RGO-2 composite reaches − 53.38 dB (2.45 mm), and the effective absorption bandwidth achieves 7.52 GHz (2.62 mm) with lower filling loading of 2 wt%. Using off-axis electron hologram testing combined with simulation calculation and carrier transport property experiments, we demonstrate here the carrier injection behavior from Fe to graphene at the interface and the induced charge accumulation and rearrangement, resulting in the increased interfacial and dipole polarization and the conductance loss. This work has confirmed that regulating the dielectric property of graphene itself by adding trace metals can not only ensure good impedance matching, but also fully exploit the dielectric loss ability of graphene at low filler content, which opens up an efficient way for designing lightweight absorbers and may be extended to other types materials. Polarization and conductance losses are the fundamental dielectric attenuation mechanisms for graphene-based absorbers, but it is not fully understood in revealing the loss mechanism of affect graphene itself. For the first time, the reduced graphene oxide (RGO) based absorbers are developed with regulatory absorption properties and the absorption mechanism of RGO is mainly originated from the carrier injection behavior of trace metal Fe nanosheets on graphene. Accordingly, the minimum reflection loss (RL ) of Fe/RGO-2 composite reaches - 53.38 dB (2.45 mm), and the effective absorption bandwidth achieves 7.52 GHz (2.62 mm) with lower filling loading of 2 wt%. Using off-axis electron hologram testing combined with simulation calculation and carrier transport property experiments, we demonstrate here the carrier injection behavior from Fe to graphene at the interface and the induced charge accumulation and rearrangement, resulting in the increased interfacial and dipole polarization and the conductance loss. This work has confirmed that regulating the dielectric property of graphene itself by adding trace metals can not only ensure good impedance matching, but also fully exploit the dielectric loss ability of graphene at low filler content, which opens up an efficient way for designing lightweight absorbers and may be extended to other types materials. Highlights A carrier injection strategy is firstly proposed by designing Fe/reduced graphene oxide (RGO) heterogeneous interfacial material for giving full play to the dielectric dispersion properties of graphene. The electromagnetic wave absorption mechanisms mainly include enhanced conductance loss, dipole polarization and interfacial polarization. Outstanding reflection loss value (− 53.38 dB, 2.45 mm) and broadband wave absorption (7.52 GHz with only 2 wt% filling) of Fe/RGO composite were acquired, which is superior to single-component graphene. HighlightsA carrier injection strategy is firstly proposed by designing Fe/reduced graphene oxide (RGO) heterogeneous interfacial material for giving full play to the dielectric dispersion properties of graphene.The electromagnetic wave absorption mechanisms mainly include enhanced conductance loss, dipole polarization and interfacial polarization.Outstanding reflection loss value (− 53.38 dB, 2.45 mm) and broadband wave absorption (7.52 GHz with only 2 wt% filling) of Fe/RGO composite were acquired, which is superior to single-component graphene.Polarization and conductance losses are the fundamental dielectric attenuation mechanisms for graphene-based absorbers, but it is not fully understood in revealing the loss mechanism of affect graphene itself. For the first time, the reduced graphene oxide (RGO) based absorbers are developed with regulatory absorption properties and the absorption mechanism of RGO is mainly originated from the carrier injection behavior of trace metal Fe nanosheets on graphene. Accordingly, the minimum reflection loss (RLmin) of Fe/RGO-2 composite reaches − 53.38 dB (2.45 mm), and the effective absorption bandwidth achieves 7.52 GHz (2.62 mm) with lower filling loading of 2 wt%. Using off-axis electron hologram testing combined with simulation calculation and carrier transport property experiments, we demonstrate here the carrier injection behavior from Fe to graphene at the interface and the induced charge accumulation and rearrangement, resulting in the increased interfacial and dipole polarization and the conductance loss. This work has confirmed that regulating the dielectric property of graphene itself by adding trace metals can not only ensure good impedance matching, but also fully exploit the dielectric loss ability of graphene at low filler content, which opens up an efficient way for designing lightweight absorbers and may be extended to other types materials. Polarization and conductance losses are the fundamental dielectric attenuation mechanisms for graphene-based absorbers, but it is not fully understood in revealing the loss mechanism of affect graphene itself. For the first time, the reduced graphene oxide (RGO) based absorbers are developed with regulatory absorption properties and the absorption mechanism of RGO is mainly originated from the carrier injection behavior of trace metal Fe nanosheets on graphene. Accordingly, the minimum reflection loss (RL min ) of Fe/RGO-2 composite reaches − 53.38 dB (2.45 mm), and the effective absorption bandwidth achieves 7.52 GHz (2.62 mm) with lower filling loading of 2 wt%. Using off-axis electron hologram testing combined with simulation calculation and carrier transport property experiments, we demonstrate here the carrier injection behavior from Fe to graphene at the interface and the induced charge accumulation and rearrangement, resulting in the increased interfacial and dipole polarization and the conductance loss. This work has confirmed that regulating the dielectric property of graphene itself by adding trace metals can not only ensure good impedance matching, but also fully exploit the dielectric loss ability of graphene at low filler content, which opens up an efficient way for designing lightweight absorbers and may be extended to other types materials. |
| ArticleNumber | 66 |
| Author | Huang, Xiaoxiao Che, Renchao Yan, Yuefeng Ma, Guansheng Zhong, Bo Liu, Yuhao Zhang, Kaili Liu, Yanan |
| Author_xml | – sequence: 1 givenname: Kaili surname: Zhang fullname: Zhang, Kaili organization: School of Materials Science and Engineering, Harbin Institute of Technology, MIIT Key Laboratory of Advanced Structural-Functional Integration Materials & Green Manufacturing Technology, Harbin Institute of Technology – sequence: 2 givenname: Yuhao surname: Liu fullname: Liu, Yuhao organization: School of Materials Science and Engineering, Harbin Institute of Technology, MIIT Key Laboratory of Advanced Structural-Functional Integration Materials & Green Manufacturing Technology, Harbin Institute of Technology – sequence: 3 givenname: Yanan surname: Liu fullname: Liu, Yanan organization: School of Materials Science and Engineering, Harbin Institute of Technology, MIIT Key Laboratory of Advanced Structural-Functional Integration Materials & Green Manufacturing Technology, Harbin Institute of Technology – sequence: 4 givenname: Yuefeng surname: Yan fullname: Yan, Yuefeng organization: School of Materials Science and Engineering, Harbin Institute of Technology, MIIT Key Laboratory of Advanced Structural-Functional Integration Materials & Green Manufacturing Technology, Harbin Institute of Technology – sequence: 5 givenname: Guansheng surname: Ma fullname: Ma, Guansheng organization: School of Materials Science and Engineering, Harbin Institute of Technology, MIIT Key Laboratory of Advanced Structural-Functional Integration Materials & Green Manufacturing Technology, Harbin Institute of Technology – sequence: 6 givenname: Bo surname: Zhong fullname: Zhong, Bo organization: School of Materials Science and Engineering, Harbin Institute of Technology at Weihai – sequence: 7 givenname: Renchao surname: Che fullname: Che, Renchao email: rcche@fudan.edu.cn organization: Laboratory of Advanced Materials, Shanghai Key Lab of Molecular Catalysis and Innovative Materials, Fudan University – sequence: 8 givenname: Xiaoxiao surname: Huang fullname: Huang, Xiaoxiao email: swliza@hit.edu.cn organization: School of Materials Science and Engineering, Harbin Institute of Technology, MIIT Key Laboratory of Advanced Structural-Functional Integration Materials & Green Manufacturing Technology, Harbin Institute of Technology |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/38175333$$D View this record in MEDLINE/PubMed |
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A carrier injection strategy is firstly proposed by designing Fe/reduced graphene oxide (RGO) heterogeneous interfacial material for giving full... Polarization and conductance losses are the fundamental dielectric attenuation mechanisms for graphene-based absorbers, but it is not fully understood in... HighlightsA carrier injection strategy is firstly proposed by designing Fe/reduced graphene oxide (RGO) heterogeneous interfacial material for giving full play... Highlights A carrier injection strategy is firstly proposed by designing Fe/reduced graphene oxide (RGO) heterogeneous interfacial material for giving full... |
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| SubjectTerms | Absorbers Absorption Broadband Carrier injection Carrier transport Dielectric loss Dielectric properties Dipoles Electromagnetic radiation Electromagnetic wave absorption Engineering Fe nanosheets Graphene Impedance matching Iron Microwave absorption and EMI shielding Nanoscale Science and Technology Nanotechnology Nanotechnology and Microengineering Polarization Reduced graphene oxide Regulatory mechanisms (biology) Trace metals Transport properties |
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| Title | Tracking Regulatory Mechanism of Trace Fe on Graphene Electromagnetic Wave Absorption |
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