Hypercrosslinked phenothiazine-based polymers as high redox potential organic cathode materials for lithium-ion batteries
Organic cathode materials have been demonstrated to be highly promising sustainable cathode materials for rechargeable lithium-ion batteries. However, the low redox potentials, low electrical conductivity, and the undesirable dissolution in organic electrolytes greatly limit their applications. Here...
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| Published in | RSC advances Vol. 1; no. 28; pp. 16732 - 16736 |
|---|---|
| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
England
Royal Society of Chemistry
29.04.2020
The Royal Society of Chemistry |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Organic cathode materials have been demonstrated to be highly promising sustainable cathode materials for rechargeable lithium-ion batteries. However, the low redox potentials, low electrical conductivity, and the undesirable dissolution in organic electrolytes greatly limit their applications. Herein, two insoluble hypercrosslinked porous conductive polymers with phenothiazine motifs,
HPEPT
and
HPPT
, were successfully accomplished with high and stable discharge potentials at 3.65 and 3.48 V
versus
Li/Li
+
.
HPEPT
and
HPPT
with good electrical conductivity exhibited outstanding rate capabilities (up to 800 mA g
−1
) even at a high mass loading up to 70 wt%. This study shows that excellent organic cathode materials could be achieved readily through this prudent design.
Hypercrosslinked conductive polymers with phenothiazine motifs were achieved and studied as organic cathode materials, exhibiting excellent electrochemical performance. |
|---|---|
| AbstractList | Organic cathode materials have been demonstrated to be highly promising sustainable cathode materials for rechargeable lithium-ion batteries. However, the low redox potentials, low electrical conductivity, and the undesirable dissolution in organic electrolytes greatly limit their applications. Herein, two insoluble hypercrosslinked porous conductive polymers with phenothiazine motifs, HPEPT and HPPT, were successfully accomplished with high and stable discharge potentials at 3.65 and 3.48 V versus Li/Li+. HPEPT and HPPT with good electrical conductivity exhibited outstanding rate capabilities (up to 800 mA g−1) even at a high mass loading up to 70 wt%. This study shows that excellent organic cathode materials could be achieved readily through this prudent design. Organic cathode materials have been demonstrated to be highly promising sustainable cathode materials for rechargeable lithium-ion batteries. However, the low redox potentials, low electrical conductivity, and the undesirable dissolution in organic electrolytes greatly limit their applications. Herein, two insoluble hypercrosslinked porous conductive polymers with phenothiazine motifs, HPEPT and HPPT , were successfully accomplished with high and stable discharge potentials at 3.65 and 3.48 V versus Li/Li + . HPEPT and HPPT with good electrical conductivity exhibited outstanding rate capabilities (up to 800 mA g −1 ) even at a high mass loading up to 70 wt%. This study shows that excellent organic cathode materials could be achieved readily through this prudent design. Organic cathode materials have been demonstrated to be highly promising sustainable cathode materials for rechargeable lithium-ion batteries. However, the low redox potentials, low electrical conductivity, and the undesirable dissolution in organic electrolytes greatly limit their applications. Herein, two insoluble hypercrosslinked porous conductive polymers with phenothiazine motifs, HPEPT and HPPT , were successfully accomplished with high and stable discharge potentials at 3.65 and 3.48 V versus Li/Li + . HPEPT and HPPT with good electrical conductivity exhibited outstanding rate capabilities (up to 800 mA g −1 ) even at a high mass loading up to 70 wt%. This study shows that excellent organic cathode materials could be achieved readily through this prudent design. Hypercrosslinked conductive polymers with phenothiazine motifs were achieved and studied as organic cathode materials, exhibiting excellent electrochemical performance. Organic cathode materials have been demonstrated to be highly promising sustainable cathode materials for rechargeable lithium-ion batteries. However, the low redox potentials, low electrical conductivity, and the undesirable dissolution in organic electrolytes greatly limit their applications. Herein, two insoluble hypercrosslinked porous conductive polymers with phenothiazine motifs, HPEPT and HPPT, were successfully accomplished with high and stable discharge potentials at 3.65 and 3.48 V versus Li/Li⁺. HPEPT and HPPT with good electrical conductivity exhibited outstanding rate capabilities (up to 800 mA g⁻¹) even at a high mass loading up to 70 wt%. This study shows that excellent organic cathode materials could be achieved readily through this prudent design. Organic cathode materials have been demonstrated to be highly promising sustainable cathode materials for rechargeable lithium-ion batteries. However, the low redox potentials, low electrical conductivity, and the undesirable dissolution in organic electrolytes greatly limit their applications. Herein, two insoluble hypercrosslinked porous conductive polymers with phenothiazine motifs, HPEPT and HPPT, were successfully accomplished with high and stable discharge potentials at 3.65 and 3.48 V versus Li/Li + . HPEPT and HPPT with good electrical conductivity exhibited outstanding rate capabilities (up to 800 mA g −1 ) even at a high mass loading up to 70 wt%. This study shows that excellent organic cathode materials could be achieved readily through this prudent design. Hypercrosslinked conductive polymers with phenothiazine motifs were achieved and studied as organic cathode materials, exhibiting excellent electrochemical performance. Organic cathode materials have been demonstrated to be highly promising sustainable cathode materials for rechargeable lithium-ion batteries. However, the low redox potentials, low electrical conductivity, and the undesirable dissolution in organic electrolytes greatly limit their applications. Herein, two insoluble hypercrosslinked porous conductive polymers with phenothiazine motifs, HPEPT and HPPT, were successfully accomplished with high and stable discharge potentials at 3.65 and 3.48 V versus Li/Li+. HPEPT and HPPT with good electrical conductivity exhibited outstanding rate capabilities (up to 800 mA g-1) even at a high mass loading up to 70 wt%. This study shows that excellent organic cathode materials could be achieved readily through this prudent design.Organic cathode materials have been demonstrated to be highly promising sustainable cathode materials for rechargeable lithium-ion batteries. However, the low redox potentials, low electrical conductivity, and the undesirable dissolution in organic electrolytes greatly limit their applications. Herein, two insoluble hypercrosslinked porous conductive polymers with phenothiazine motifs, HPEPT and HPPT, were successfully accomplished with high and stable discharge potentials at 3.65 and 3.48 V versus Li/Li+. HPEPT and HPPT with good electrical conductivity exhibited outstanding rate capabilities (up to 800 mA g-1) even at a high mass loading up to 70 wt%. This study shows that excellent organic cathode materials could be achieved readily through this prudent design. Organic cathode materials have been demonstrated to be highly promising sustainable cathode materials for rechargeable lithium-ion batteries. However, the low redox potentials, low electrical conductivity, and the undesirable dissolution in organic electrolytes greatly limit their applications. Herein, two insoluble hypercrosslinked porous conductive polymers with phenothiazine motifs, HPEPT and HPPT, were successfully accomplished with high and stable discharge potentials at 3.65 and 3.48 V Li/Li . HPEPT and HPPT with good electrical conductivity exhibited outstanding rate capabilities (up to 800 mA g ) even at a high mass loading up to 70 wt%. This study shows that excellent organic cathode materials could be achieved readily through this prudent design. |
| Author | Yang, Haishen Du, Ya Zhang, Ruiqiang Zhang, Ying Chen, Han Guo, Xinya Gao, Panpan Wang, Baofeng |
| AuthorAffiliation | School of Chemistry and Molecular Engineering Shanghai University of Electric Power Nanjing Tech University Institute of Advanced Synthesis College of Environmental and Chemical Engineering Shanghai Key Laboratory of Materials Protection and Advanced Materials in Electric Power |
| AuthorAffiliation_xml | – name: Shanghai Key Laboratory of Materials Protection and Advanced Materials in Electric Power – name: Nanjing Tech University – name: College of Environmental and Chemical Engineering – name: School of Chemistry and Molecular Engineering – name: Shanghai University of Electric Power – name: Institute of Advanced Synthesis |
| Author_xml | – sequence: 1 givenname: Ying surname: Zhang fullname: Zhang, Ying – sequence: 2 givenname: Panpan surname: Gao fullname: Gao, Panpan – sequence: 3 givenname: Xinya surname: Guo fullname: Guo, Xinya – sequence: 4 givenname: Han surname: Chen fullname: Chen, Han – sequence: 5 givenname: Ruiqiang surname: Zhang fullname: Zhang, Ruiqiang – sequence: 6 givenname: Ya surname: Du fullname: Du, Ya – sequence: 7 givenname: Baofeng surname: Wang fullname: Wang, Baofeng – sequence: 8 givenname: Haishen surname: Yang fullname: Yang, Haishen |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/35498833$$D View this record in MEDLINE/PubMed |
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| SubjectTerms | Cathodes Chemistry Conducting polymers crosslinking electrical conductivity Electrical resistivity Electrode materials Lithium Lithium-ion batteries Nonaqueous electrolytes phenothiazine Rechargeable batteries redox potential |
| Title | Hypercrosslinked phenothiazine-based polymers as high redox potential organic cathode materials for lithium-ion batteries |
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