Absorption detection using optical waveguide cavities
Cavity ring-down spectroscopy is a spectroscopic method that uses a high quality optical cavity to amplify the optical loss due to the light absorption by a sample. In this presentation we highlight two applications of phase-shift cavity ring-down spectroscopy that are suited for absorption measurem...
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| Published in | Canadian journal of chemistry Vol. 88; no. 5; pp. 401 - 410 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Ottawa
NRC Research Press
01.05.2010
Canadian Science Publishing NRC Research Press |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Cavity ring-down spectroscopy is a spectroscopic method that uses a high quality optical cavity to amplify the optical loss due to the light absorption by a sample. In this presentation we highlight two applications of phase-shift cavity ring-down spectroscopy that are suited for absorption measurements in the condensed phase and make use of waveguide cavities. In the first application, a fiber loop is used as an optical cavity and the sample is introduced in a gap in the loop to allow absorption measurements of nanoliters of solution at the micromolar level. A second application involves silica microspheres as high finesse cavities. Information on the refractive index and absorption of a thin film of ethylene diamine on the surface of the microresonator is obtained simultaneously by the measurements of the wavelength shift of the cavity mode spectrum and the change in optical decay time, respectively. |
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| AbstractList | Cavity ring-down spectroscopy is a spectroscopic method that uses a high quality optical cavity to amplify the optical loss due to the light absorption by a sample. In this presentation we highlight two applications of phase-shift cavity ring-down spectroscopy that are suited for absorption measurements in the condensed phase and make use of waveguide cavities. In the first application, a fiber loop is used as an optical cavity and the sample is introduced in a gap in the loop to allow absorption measurements of nanoliters of solution at the micromolar level. A second application involves silica microspheres as high finesse cavities. Information on the refractive index and absorption of a thin film of ethylene diamine on the surface of the microresonator is obtained simultaneously by the measurements of the wavelength shift of the cavity mode spectrum and the change in optical decay time, respectively. Cavity ring-down spectroscopy is a spectroscopic method that uses a high quality optical cavity to amplify the optical loss due to the light absorption by a sample. In this presentation we highlight two applications of phase-shift cavity ring-down spectroscopy that are suited for absorption measurements in the condensed phase and make use of waveguide cavities. In the first application, a fiber loop is used as an optical cavity and the sample is introduced in a gap in the loop to allow absorption measurements of nanoliters of solution at the micromolar level. A second application involves silica microspheres as high finesse cavities. Information on the refractive index and absorption of a thin film of ethylene diamine on the surface of the microresonator is obtained simultaneously by the measurements of the wavelength shift of the cavity mode spectrum and the change in optical decay time, respectively. Key words: cavity ring-down spectroscopy, microresonator, microsphere, fiber loop. La spectroscopie a cavite ring-down est une meethode spectroscopique qui utilise une cavite optique de haute qualite pour amplifier la perte optique due a l'absorption de lumiere par l'echantillon. Durant cette presentation, nous mettons en evidence deux applications de la spectroscopie a cavite; ring-down avec deeplacement de phase qui convient aux mesures d'absorption en phase condenseee et fait usage de caviteesa guide d'onde. Dans la premiere application, une boucle de fibre est utiliseie comme cavite optique et l'eechantillon est introduit dans un intervalle de la boucle pour permettre des mesures d'absorption sur des nanolitres de solution au niveau micromolaire. Une seconde application est basee sur des microspheres de silice comme caviteesa haute finesse. Des informations sur l'index de refraction et l'absorption d'un film mince d'ethylene diamine sur la surface d'un micro-resonateur sont obtenues simultaneement par des mesures de deplacement de longueur d'onde du spectre modal de la cavite et de changement de temps de decroissance optique, respectivement. Mots-cles: spectroscopie a cavite; ring-down, micro-resonateur, microsphere, boucle de fibre. Cavity ring-down spectroscopy is a spectroscopic method that uses a high quality optical cavity to amplify the optical loss due to the light absorption by a sample. In this presentation we highlight two applications of phase-shift cavity ring-down spectroscopy that are suited for absorption measurements in the condensed phase and make use of waveguide cavities. In the first application, a fiber loop is used as an optical cavity and the sample is introduced in a gap in the loop to allow absorption measurements of nanoliters of solution at the micromolar level. A second application involves silica microspheres as high finesse cavities. Information on the refractive index and absorption of a thin film of ethylene diamine on the surface of the microresonator is obtained simultaneously by the measurements of the wavelength shift of the cavity mode spectrum and the change in optical decay time, respectively. [PUBLICATION ABSTRACT] |
| Abstract_FL | La spectroscopie à cavité ring-down est une méthode spectroscopique qui utilise une cavité optique de haute qualité pour amplifier la perte optique due à l'absorption de lumière par l'échantillon. Durant cette présentation, nous mettons en évidence deux applications de la spectroscopie à cavité ring-down avec déplacement de phase qui convient aux mesures d'absorption en phase condensée et fait usage de cavités à guide d'onde. Dans la première application, une boucle de fibre est utilisée comme cavité optique et l'échantillon est introduit dans un intervalle de la boucle pour permettre des mesures d'absorption sur des nanolitres de solution au niveau micromolaire. Une seconde application est basée sur des microsphères de silice comme cavités à haute finesse. Des informations sur l'index de réfraction et l'absorption d'un film mince d'éthylène diamine sur la surface d'un micro-résonateur sont obtenues simultanément par des mesures de déplacement de longueur d'onde du spectre modal de la cavité et de changement de temps de décroissance optique, respectivement. |
| Audience | Academic |
| Author | Oleschuk, Richard D Gagliardi, Gianluca Wächter, Helen Loock, Hans-Peter Li, Runkai Barnes, Jack A |
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| SubjectTerms | Absorption Absorption of light boucle de fibre cavity ring-down spectroscopy Ethylene fiber loop Measurement micro-résonateur microresonator microsphere microsphère Optics Silica Sorption spectroscopie à cavité ring-down Spectroscopy Spectrum analysis Thin films Waveguides |
| Title | Absorption detection using optical waveguide cavities |
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