Direct On-Surface Patterning of a Crystalline Laminar Covalent Organic Framework Synthesized at Room Temperature

We report herein an efficient, fast, and simple synthesis of an imine‐based covalent organic framework (COF) at room temperature (hereafter, RT‐COF‐1). RT‐COF‐1 shows a layered hexagonal structure exhibiting channels, is robust, and is porous to N2 and CO2. The room‐temperature synthesis has enabled...

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Published inChemistry : a European journal Vol. 21; no. 30; pp. 10666 - 10670
Main Authors de la Peña Ruigómez, Alejandro, Rodríguez-San-Miguel, David, Stylianou, Kyriakos C., Cavallini, Massimiliano, Gentili, Denis, Liscio, Fabiola, Milita, Silvia, Roscioni , Otello Maria, Ruiz-González, Maria Luisa, Carbonell, Carlos, Maspoch, Daniel, Mas-Ballesté, Rubén, Segura, José Luis, Zamora, Félix
Format Journal Article
LanguageEnglish
Published Weinheim WILEY-VCH Verlag 20.07.2015
WILEY‐VCH Verlag
Wiley
Wiley Subscription Services, Inc
Subjects
Carbon dioxide
Channels
Chemistry
Chemistry, Multidisciplinary
Covalence
covalent organic frameworks
Crystal structure
Crystals
ink-jet printing
Laminar
Physical Sciences
porous crystalline materials
Printing
processability
Science & Technology
soft-lithography
Synthesis
Temperature
STORAGE
covalent organic frameworks
soft-lithography
SINGLE-LAYER GRAPHENE
SCHIFF-BASE CHEMISTRY
NETWORKS
MICROPOROUS POLYMER
processability
ink-jet printing
porous crystalline materials
ORIENTED THIN-FILMS
CAGE COMPOUNDS
CONSTRUCTION
GROWTH
CARBON-DIOXIDE
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Abstract We report herein an efficient, fast, and simple synthesis of an imine‐based covalent organic framework (COF) at room temperature (hereafter, RT‐COF‐1). RT‐COF‐1 shows a layered hexagonal structure exhibiting channels, is robust, and is porous to N2 and CO2. The room‐temperature synthesis has enabled us to fabricate and position low‐cost micro‐ and submicropatterns of RT‐COF‐1 on several surfaces, including solid SiO2 substrates and flexible acetate paper, by using lithographically controlled wetting and conventional ink‐jet printing. Printed crystals: An efficient, fast and simple synthesis of an imine‐based porous covalent organic framework (COF) at room temperature is reported. The room‐temperature synthesis enables fabricating micro‐ and submicropatterns of this COF on a variety of surfaces by ink‐jet printing and wet lithographically techniques.
AbstractList We report herein an efficient, fast, and simple synthesis of an imine-based covalent organic framework (COF) at room temperature (hereafter, RT-COF-1). RT-COF-1 shows a layered hexagonal structure exhibiting channels, is robust, and is porous to N sub(2) and CO sub(2). The room-temperature synthesis has enabled us to fabricate and position low-cost micro- and submicropatterns of RT-COF-1 on several surfaces, including solid SiO sub(2) substrates and flexible acetate paper, by using lithographically controlled wetting and conventional ink-jet printing. Printed crystals: An efficient, fast and simple synthesis of an imine-based porous covalent organic framework (COF) at room temperature is reported. The room-temperature synthesis enables fabricating micro- and submicropatterns of this COF on a variety of surfaces by ink-jet printing and wet lithographically techniques.
We report herein an efficient, fast, and simple synthesis of an imine-based covalent organic framework (COF) at room temperature (hereafter, RT-COF-1). RT-COF-1 shows a layered hexagonal structure exhibiting channels, is robust, and is porous to N2 and CO2 . The room-temperature synthesis has enabled us to fabricate and position low-cost micro- and submicropatterns of RT-COF-1 on several surfaces, including solid SiO2 substrates and flexible acetate paper, by using lithographically controlled wetting and conventional ink-jet printing.
We report herein an efficient, fast, and simple synthesis of an imine‐based covalent organic framework (COF) at room temperature (hereafter, RT‐COF‐1). RT‐COF‐1 shows a layered hexagonal structure exhibiting channels, is robust, and is porous to N2 and CO2. The room‐temperature synthesis has enabled us to fabricate and position low‐cost micro‐ and submicropatterns of RT‐COF‐1 on several surfaces, including solid SiO2 substrates and flexible acetate paper, by using lithographically controlled wetting and conventional ink‐jet printing. Printed crystals: An efficient, fast and simple synthesis of an imine‐based porous covalent organic framework (COF) at room temperature is reported. The room‐temperature synthesis enables fabricating micro‐ and submicropatterns of this COF on a variety of surfaces by ink‐jet printing and wet lithographically techniques.
We report herein an efficient, fast, and simple synthesis of an imine-based covalent organic framework (COF) at room temperature (hereafter, RT-COF-1). RT-COF-1 shows a layered hexagonal structure exhibiting channels, is robust, and is porous to N-2 and CO2. The room-temperature synthesis has enabled us to fabricate and position low-cost micro- and submicropatterns of RT-COF-1 on several surfaces, including solid SiO2 substrates and flexible acetate paper, by using lithographically controlled wetting and conventional ink-jet printing.
Abstract We report herein an efficient, fast, and simple synthesis of an imine‐based covalent organic framework (COF) at room temperature (hereafter, RT‐COF‐1 ). RT‐COF‐1 shows a layered hexagonal structure exhibiting channels, is robust, and is porous to N 2 and CO 2 . The room‐temperature synthesis has enabled us to fabricate and position low‐cost micro‐ and submicropatterns of RT‐COF‐1 on several surfaces, including solid SiO 2 substrates and flexible acetate paper, by using lithographically controlled wetting and conventional ink‐jet printing.
Author Cavallini, Massimiliano
Mas-Ballesté, Rubén
Carbonell, Carlos
Stylianou, Kyriakos C.
Milita, Silvia
Ruiz-González, Maria Luisa
Liscio, Fabiola
Segura, José Luis
Roscioni , Otello Maria
de la Peña Ruigómez, Alejandro
Rodríguez-San-Miguel, David
Zamora, Félix
Gentili, Denis
Maspoch, Daniel
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  givenname: Kyriakos C.
  surname: Stylianou
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  organization: Consiglio Nazionale delle Ricerche, Instituto per lo Studio dei Materiali, Nanostrutturati (CNR-ISMN), Via Gobetti 101, 40129 Bologna (Italy)
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  organization: CNR-IMM, Instituto per la Microelettronica e Microsistemi via P. Gobetti 101, 40129 Bologna (Italy)
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  givenname: Silvia
  surname: Milita
  fullname: Milita, Silvia
  organization: CNR-IMM, Instituto per la Microelettronica e Microsistemi via P. Gobetti 101, 40129 Bologna (Italy)
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  givenname: Otello Maria
  surname: Roscioni 
  fullname: Roscioni , Otello Maria
  organization: Universitàdi Bologna, Dipartimento di Chimica Industriale, "Toso Montanari", Viale Risorgimento 4, 40136, Bologna (Italy)
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  givenname: Maria Luisa
  surname: Ruiz-González
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  organization: Departamento de Química Inorgánica, Universidad Complutense de Madrid, 28040 Madrid (Spain)
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  organization: ICN2-Institut Catala de Nanociencia i Nanotecnologia, Campus UAB, 08193 Bellaterra, Barcelona (Spain)
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  organization: Departamento de Química Inorgánica, Universidad Autónoma de Madrid, 28049 Madrid (Spain)
– sequence: 13
  givenname: José Luis
  surname: Segura
  fullname: Segura, José Luis
  organization: Departamento de Química Orgánica, Facultad de Ciencias Químicas, Universidad Complutense de Madrid, Avda. Complutense s/n 28040 Madrid (Spain)
– sequence: 14
  givenname: Félix
  surname: Zamora
  fullname: Zamora, Félix
  email: felix.zamora@uam.es
  organization: Departamento de Química Inorgánica, Universidad Autónoma de Madrid, 28049 Madrid (Spain)
BackLink https://www.ncbi.nlm.nih.gov/pubmed/26095511$$D View this record in MEDLINE/PubMed
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ContentType Journal Article
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2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim
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Issue 30
Keywords STORAGE
covalent organic frameworks
soft-lithography
SINGLE-LAYER GRAPHENE
SCHIFF-BASE CHEMISTRY
NETWORKS
MICROPOROUS POLYMER
processability
ink-jet printing
porous crystalline materials
ORIENTED THIN-FILMS
CAGE COMPOUNDS
CONSTRUCTION
GROWTH
CARBON-DIOXIDE
Language English
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2011; 2
2009; 21
2009; 65
2013; 49
2012
2005; 310
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2013; 42
2014; 26
2006; 18
2008 2008; 47 120
2009; 131
2013; 7
2011; 5
2011; 332
2011; 133
2014; 20
2013; 19
2010; 22
2007; 316
2013; 15
2014; 5
2012; 134
2012; 112
2014; 2
2012 2012; 51 124
2003; 3
2013; 135
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2011 2011; 50 123
2008; 20
2011; 47
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2010; 2
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2012; 7
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e_1_2_3_50_2
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e_1_2_3_4_2
e_1_2_3_16_2
e_1_2_3_37_2
e_1_2_3_2_2
e_1_2_3_18_2
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Warren B. E. (e_1_2_3_46_2) 1969
e_1_2_3_21_2
e_1_2_3_42_2
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SSID ssj0009633
Score 2.5577698
Snippet We report herein an efficient, fast, and simple synthesis of an imine‐based covalent organic framework (COF) at room temperature (hereafter, RT‐COF‐1)....
We report herein an efficient, fast, and simple synthesis of an imine-based covalent organic framework (COF) at room temperature (hereafter, RT-COF-1)....
Abstract We report herein an efficient, fast, and simple synthesis of an imine‐based covalent organic framework (COF) at room temperature (hereafter, RT‐COF‐1...
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StartPage 10666
SubjectTerms Carbon dioxide
Channels
Chemistry
Chemistry, Multidisciplinary
Covalence
covalent organic frameworks
Crystal structure
Crystals
ink-jet printing
Laminar
Physical Sciences
porous crystalline materials
Printing
processability
Science & Technology
soft-lithography
Synthesis
Temperature
Title Direct On-Surface Patterning of a Crystalline Laminar Covalent Organic Framework Synthesized at Room Temperature
URI https://api.istex.fr/ark:/67375/WNG-4S5BCH9G-9/fulltext.pdf
https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fchem.201501692
http://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcApp=Summon&SrcAuth=ProQuest&DestApp=WOS&DestLinkType=FullRecord&UT=000357984900011
https://www.ncbi.nlm.nih.gov/pubmed/26095511
https://www.proquest.com/docview/1696005805/abstract/
https://search.proquest.com/docview/1697216056
https://search.proquest.com/docview/1786207544
Volume 21
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