MOF-derived Cobalt Sulfide Grown on 3D Graphene Foam as an Efficient Sulfur Host for Long-Life Lithium-Sulfur Batteries
Lithium-sulfur (Li-S) batteries are an appealing candidate for advanced energy storage systems because of their high theoretical energy density and low cost. However, rapid capacity decay and short cycle life, mainly resulting from polysulfide dissolution, remains a great challenge for practical app...
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| Published in | iScience Vol. 4; no. C; pp. 36 - 43 |
|---|---|
| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
Elsevier Inc
29.06.2018
Elsevier |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Lithium-sulfur (Li-S) batteries are an appealing candidate for advanced energy storage systems because of their high theoretical energy density and low cost. However, rapid capacity decay and short cycle life, mainly resulting from polysulfide dissolution, remains a great challenge for practical applications. Herein, we present a metal-organic framework (MOF)-derived Co9S8 array anchored onto a chemical vapor deposition (CVD)-grown three-dimensional graphene foam (Co9S8-3DGF) as an efficient sulfur host for long-life Li-S batteries with good performance. Without polymeric binders, conductive additives, or metallic current collectors, the free-standing Co9S8-3DGF/S cathode achieves a high areal capacity of 10.9 mA hr cm−2 even at a very high sulfur loading (10.4 mg cm−2) and sulfur content (86.9 wt%). These results are attributed to the unique hierarchical nanoarchitecture of Co9S8-3DGF/S. This work is expected to open up a promising direction for the practical viability of high-energy Li-S batteries.
[Display omitted]
•Metal-organic framework-derived Co9S8 arrays are grown onto 3D graphene foam•Co9S8-3DGF serves as a free-standing, binder-free host for sulfur cathodes•Co9S8-3DGF/S cathode exhibits high capacity with long cycle life•Co9S8-3DGF/S cathode displays a remarkably high areal capacity
Inorganic Chemistry; Energy Materials; Porous Material |
|---|---|
| AbstractList | Lithium-sulfur (Li-S) batteries are an appealing candidate for advanced energy storage systems because of their high theoretical energy density and low cost. Yet, rapid capacity decay and short cycle life, mainly resulting from polysulfide dissolution, remains a great challenge for practical applications. Herein, we present a metal-organic framework (MOF)-derived Co9S8 array anchored onto a chemical vapor deposition (CVD)-grown three-dimensional graphene foam (Co9S8-3DGF) as an efficient sulfur host for long-life Li-S batteries with good performance. Without polymeric binders, conductive additives, or metallic current collectors, the free-standing Co9S8-3DGF/S cathode achieves a high areal capacity of 10.9 mA hr cm-2 even at a very high sulfur loading (10.4 mg cm-2) and sulfur content (86.9 wt%). These results are attributed to the unique hierarchical nanoarchitecture of Co9S8-3DGF/S. Our work is expected to open up a promising direction for the practical viability of high-energy Li-S batteries Lithium-sulfur (Li-S) batteries are an appealing candidate for advanced energy storage systems because of their high theoretical energy density and low cost. However, rapid capacity decay and short cycle life, mainly resulting from polysulfide dissolution, remains a great challenge for practical applications. Herein, we present a metal-organic framework (MOF)-derived Co9S8 array anchored onto a chemical vapor deposition (CVD)-grown three-dimensional graphene foam (Co9S8-3DGF) as an efficient sulfur host for long-life Li-S batteries with good performance. Without polymeric binders, conductive additives, or metallic current collectors, the free-standing Co9S8-3DGF/S cathode achieves a high areal capacity of 10.9 mA hr cm-2 even at a very high sulfur loading (10.4 mg cm-2) and sulfur content (86.9 wt%). These results are attributed to the unique hierarchical nanoarchitecture of Co9S8-3DGF/S. This work is expected to open up a promising direction for the practical viability of high-energy Li-S batteries.Lithium-sulfur (Li-S) batteries are an appealing candidate for advanced energy storage systems because of their high theoretical energy density and low cost. However, rapid capacity decay and short cycle life, mainly resulting from polysulfide dissolution, remains a great challenge for practical applications. Herein, we present a metal-organic framework (MOF)-derived Co9S8 array anchored onto a chemical vapor deposition (CVD)-grown three-dimensional graphene foam (Co9S8-3DGF) as an efficient sulfur host for long-life Li-S batteries with good performance. Without polymeric binders, conductive additives, or metallic current collectors, the free-standing Co9S8-3DGF/S cathode achieves a high areal capacity of 10.9 mA hr cm-2 even at a very high sulfur loading (10.4 mg cm-2) and sulfur content (86.9 wt%). These results are attributed to the unique hierarchical nanoarchitecture of Co9S8-3DGF/S. This work is expected to open up a promising direction for the practical viability of high-energy Li-S batteries. Lithium-sulfur (Li-S) batteries are an appealing candidate for advanced energy storage systems because of their high theoretical energy density and low cost. However, rapid capacity decay and short cycle life, mainly resulting from polysulfide dissolution, remains a great challenge for practical applications. Herein, we present a metal-organic framework (MOF)-derived Co9S8 array anchored onto a chemical vapor deposition (CVD)-grown three-dimensional graphene foam (Co9S8-3DGF) as an efficient sulfur host for long-life Li-S batteries with good performance. Without polymeric binders, conductive additives, or metallic current collectors, the free-standing Co9S8-3DGF/S cathode achieves a high areal capacity of 10.9 mA hr cm−2 even at a very high sulfur loading (10.4 mg cm−2) and sulfur content (86.9 wt%). These results are attributed to the unique hierarchical nanoarchitecture of Co9S8-3DGF/S. This work is expected to open up a promising direction for the practical viability of high-energy Li-S batteries. : Inorganic Chemistry; Energy Materials; Porous Material Subject Areas: Inorganic Chemistry, Energy Materials, Porous Material Lithium-sulfur (Li-S) batteries are an appealing candidate for advanced energy storage systems because of their high theoretical energy density and low cost. However, rapid capacity decay and short cycle life, mainly resulting from polysulfide dissolution, remains a great challenge for practical applications. Herein, we present a metal-organic framework (MOF)-derived Co S array anchored onto a chemical vapor deposition (CVD)-grown three-dimensional graphene foam (Co S -3DGF) as an efficient sulfur host for long-life Li-S batteries with good performance. Without polymeric binders, conductive additives, or metallic current collectors, the free-standing Co S -3DGF/S cathode achieves a high areal capacity of 10.9 mA hr cm even at a very high sulfur loading (10.4 mg cm ) and sulfur content (86.9 wt%). These results are attributed to the unique hierarchical nanoarchitecture of Co S -3DGF/S. This work is expected to open up a promising direction for the practical viability of high-energy Li-S batteries. Lithium-sulfur (Li-S) batteries are an appealing candidate for advanced energy storage systems because of their high theoretical energy density and low cost. However, rapid capacity decay and short cycle life, mainly resulting from polysulfide dissolution, remains a great challenge for practical applications. Herein, we present a metal-organic framework (MOF)-derived Co 9 S 8 array anchored onto a chemical vapor deposition (CVD)-grown three-dimensional graphene foam (Co 9 S 8 -3DGF) as an efficient sulfur host for long-life Li-S batteries with good performance. Without polymeric binders, conductive additives, or metallic current collectors, the free-standing Co 9 S 8 -3DGF/S cathode achieves a high areal capacity of 10.9 mA hr cm −2 even at a very high sulfur loading (10.4 mg cm −2 ) and sulfur content (86.9 wt%). These results are attributed to the unique hierarchical nanoarchitecture of Co 9 S 8 -3DGF/S. This work is expected to open up a promising direction for the practical viability of high-energy Li-S batteries. • Metal-organic framework-derived Co 9 S 8 arrays are grown onto 3D graphene foam • Co 9 S 8 -3DGF serves as a free-standing, binder-free host for sulfur cathodes • Co 9 S 8 -3DGF/S cathode exhibits high capacity with long cycle life • Co 9 S 8 -3DGF/S cathode displays a remarkably high areal capacity Inorganic Chemistry; Energy Materials; Porous Material Lithium-sulfur (Li-S) batteries are an appealing candidate for advanced energy storage systems because of their high theoretical energy density and low cost. However, rapid capacity decay and short cycle life, mainly resulting from polysulfide dissolution, remains a great challenge for practical applications. Herein, we present a metal-organic framework (MOF)-derived Co9S8 array anchored onto a chemical vapor deposition (CVD)-grown three-dimensional graphene foam (Co9S8-3DGF) as an efficient sulfur host for long-life Li-S batteries with good performance. Without polymeric binders, conductive additives, or metallic current collectors, the free-standing Co9S8-3DGF/S cathode achieves a high areal capacity of 10.9 mA hr cm−2 even at a very high sulfur loading (10.4 mg cm−2) and sulfur content (86.9 wt%). These results are attributed to the unique hierarchical nanoarchitecture of Co9S8-3DGF/S. This work is expected to open up a promising direction for the practical viability of high-energy Li-S batteries. [Display omitted] •Metal-organic framework-derived Co9S8 arrays are grown onto 3D graphene foam•Co9S8-3DGF serves as a free-standing, binder-free host for sulfur cathodes•Co9S8-3DGF/S cathode exhibits high capacity with long cycle life•Co9S8-3DGF/S cathode displays a remarkably high areal capacity Inorganic Chemistry; Energy Materials; Porous Material |
| Author | Manthiram, Arumugam He, Jiarui Chen, Yuanfu |
| AuthorAffiliation | 2 State Key Laboratory of Electronic Thin Films and Integrated Devices, University of Electronic Science and Technology of China, Chengdu 610054, PR China 1 Materials Science and Engineering Program & Texas Materials Institute, The University of Texas at Austin, Austin, TX 78712, USA |
| AuthorAffiliation_xml | – name: 2 State Key Laboratory of Electronic Thin Films and Integrated Devices, University of Electronic Science and Technology of China, Chengdu 610054, PR China – name: 1 Materials Science and Engineering Program & Texas Materials Institute, The University of Texas at Austin, Austin, TX 78712, USA |
| Author_xml | – sequence: 1 givenname: Jiarui surname: He fullname: He, Jiarui organization: Materials Science and Engineering Program & Texas Materials Institute, The University of Texas at Austin, Austin, TX 78712, USA – sequence: 2 givenname: Yuanfu surname: Chen fullname: Chen, Yuanfu email: yfchen@uestc.edu.cn organization: State Key Laboratory of Electronic Thin Films and Integrated Devices, University of Electronic Science and Technology of China, Chengdu 610054, PR China – sequence: 3 givenname: Arumugam orcidid: 0000-0003-0237-9563 surname: Manthiram fullname: Manthiram, Arumugam email: manth@austin.utexas.edu organization: Materials Science and Engineering Program & Texas Materials Institute, The University of Texas at Austin, Austin, TX 78712, USA |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/30240751$$D View this record in MEDLINE/PubMed https://www.osti.gov/biblio/1438514$$D View this record in Osti.gov |
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| Title | MOF-derived Cobalt Sulfide Grown on 3D Graphene Foam as an Efficient Sulfur Host for Long-Life Lithium-Sulfur Batteries |
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