Microwave-enhanced photocatalysis on CdS quantum dots - Evidence of acceleration of photoinduced electron transfer
The rate of electron transfer is critical in determining the efficiency of photoenergy conversion systems and is controlled by changing the relative energy gap of components, their geometries, or surroundings. However, the rate of electron transfer has not been controlled by the remote input of an e...
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| Published in | Scientific reports Vol. 5; no. 1; p. 11308 |
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| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
17.06.2015
Nature Publishing Group |
| Subjects | |
| Online Access | Get full text |
| ISSN | 2045-2322 2045-2322 |
| DOI | 10.1038/srep11308 |
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| Abstract | The rate of electron transfer is critical in determining the efficiency of photoenergy conversion systems and is controlled by changing the relative energy gap of components, their geometries, or surroundings. However, the rate of electron transfer has not been controlled by the remote input of an external field without changing the geometries or materials of the systems. We demonstrate here that an applied microwave field can enhance the photocatalytic reduction of bipyridinium ion using CdS quantum dots (QDs) by accelerating electron transfer. Analysis of the time-resolved emission decay profiles of CdS quantum dots immersed in aqueous solutions of bipyridinium exhibited the shortening of their emission lifetimes, because of the accelerated electron transfer from QDs to bipyridinium under microwave irradiation. This discovery leads us to a new methodology using microwaves as an external field to enhance photocatalytic reactions. |
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| AbstractList | The rate of electron transfer is critical in determining the efficiency of photoenergy conversion systems and is controlled by changing the relative energy gap of components, their geometries, or surroundings. However, the rate of electron transfer has not been controlled by the remote input of an external field without changing the geometries or materials of the systems. We demonstrate here that an applied microwave field can enhance the photocatalytic reduction of bipyridinium ion using CdS quantum dots (QDs) by accelerating electron transfer. Analysis of the time-resolved emission decay profiles of CdS quantum dots immersed in aqueous solutions of bipyridinium exhibited the shortening of their emission lifetimes, because of the accelerated electron transfer from QDs to bipyridinium under microwave irradiation. This discovery leads us to a new methodology using microwaves as an external field to enhance photocatalytic reactions. The rate of electron transfer is critical in determining the efficiency of photoenergy conversion systems and is controlled by changing the relative energy gap of components, their geometries, or surroundings. However, the rate of electron transfer has not been controlled by the remote input of an external field without changing the geometries or materials of the systems. We demonstrate here that an applied microwave field can enhance the photocatalytic reduction of bipyridinium ion using CdS quantum dots (QDs) by accelerating electron transfer. Analysis of the time-resolved emission decay profiles of CdS quantum dots immersed in aqueous solutions of bipyridinium exhibited the shortening of their emission lifetimes, because of the accelerated electron transfer from QDs to bipyridinium under microwave irradiation. This discovery leads us to a new methodology using microwaves as an external field to enhance photocatalytic reactions.The rate of electron transfer is critical in determining the efficiency of photoenergy conversion systems and is controlled by changing the relative energy gap of components, their geometries, or surroundings. However, the rate of electron transfer has not been controlled by the remote input of an external field without changing the geometries or materials of the systems. We demonstrate here that an applied microwave field can enhance the photocatalytic reduction of bipyridinium ion using CdS quantum dots (QDs) by accelerating electron transfer. Analysis of the time-resolved emission decay profiles of CdS quantum dots immersed in aqueous solutions of bipyridinium exhibited the shortening of their emission lifetimes, because of the accelerated electron transfer from QDs to bipyridinium under microwave irradiation. This discovery leads us to a new methodology using microwaves as an external field to enhance photocatalytic reactions. |
| ArticleNumber | 11308 |
| Author | Fujii, Satoshi Suzuki, Eiichi Wada, Yuji Imai, Takashi Kishimoto, Fuminao Mochizuki, Dai Maitani, Masato M. |
| Author_xml | – sequence: 1 givenname: Fuminao surname: Kishimoto fullname: Kishimoto, Fuminao organization: Department of Applied Chemistry, Tokyo Institute of Technology – sequence: 2 givenname: Takashi surname: Imai fullname: Imai, Takashi organization: Department of Applied Chemistry, Tokyo Institute of Technology – sequence: 3 givenname: Satoshi surname: Fujii fullname: Fujii, Satoshi organization: Department of Applied Chemistry, Tokyo Institute of Technology, Knowledge-Intensive Collaborative Research Center, Chiba University, Okinawa National College of Technology, Department of Information and Communication System Engineering – sequence: 4 givenname: Dai surname: Mochizuki fullname: Mochizuki, Dai organization: Department of Applied Chemistry, Tokyo Institute of Technology, Interdisciplinary Cluster for Cutting Edge Research, Center for Energy and Environmental Science, Shinshu University – sequence: 5 givenname: Masato M. surname: Maitani fullname: Maitani, Masato M. organization: Department of Applied Chemistry, Tokyo Institute of Technology – sequence: 6 givenname: Eiichi surname: Suzuki fullname: Suzuki, Eiichi organization: Department of Applied Chemistry, Tokyo Institute of Technology – sequence: 7 givenname: Yuji surname: Wada fullname: Wada, Yuji organization: Department of Applied Chemistry, Tokyo Institute of Technology |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/26080653$$D View this record in MEDLINE/PubMed |
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| Cites_doi | 10.1021/jp3072074 10.1021/ja00358a006 10.1002/anie.200400655 10.1063/1.447218 10.1016/j.jphotochemrev.2009.06.001 10.1002/pola.1992.080300817 10.1063/1.1742723 10.1016/j.jphotochemrev.2011.02.003 10.1021/jp809269m 10.1002/chem.200390182 10.1002/adma.200400271 10.1002/1521-3773(20020703)41:13<2368::AID-ANIE2368>3.0.CO;2-G 10.1021/cr900356p 10.1002/jhet.5570200455 10.1016/S0040-4039(00)83996-9 10.1021/ja408936j 10.1246/cl.2012.1409 10.1021/op100202j 10.1021/jp011291g 10.1021/jp2075995 10.1021/j100373a089 10.1021/jo7022697 10.1021/jp100509h 10.1073/pnas.1011972107 10.1021/ar980112j 10.1039/B800489G |
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| Notes | ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 14 content type line 23 Present address: Interdisciplinary Cluster for Cutting Edge Research, Center for Energy and Environmental Science, Shinshu University, 3-15-1 Tokida, Ueda, Nagano 386-8567, Japan. Present address: Okinawa National College of Technology, Department of Information and Communication System Engineering, 905 Henoko, Nago-city, Okinawa, Japan. |
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| Title | Microwave-enhanced photocatalysis on CdS quantum dots - Evidence of acceleration of photoinduced electron transfer |
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