Enhancement of Sodium Ion Battery Performance Enabled by Oxygen Vacancies
The utilization of oxygen vacancies (OVs) in sodium ion batteries (SIBs) is expected to enhance performance, but as yet it has rarely been reported. Taking the MoO3−x nanosheet anode as an example, for the first time we demonstrate the benefits of OVs on SIB performance. Moreover, the benefits at de...
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| Published in | Angewandte Chemie International Edition Vol. 54; no. 30; pp. 8768 - 8771 |
|---|---|
| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Weinheim
WILEY-VCH Verlag
20.07.2015
WILEY‐VCH Verlag Wiley Subscription Services, Inc |
| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | The utilization of oxygen vacancies (OVs) in sodium ion batteries (SIBs) is expected to enhance performance, but as yet it has rarely been reported. Taking the MoO3−x nanosheet anode as an example, for the first time we demonstrate the benefits of OVs on SIB performance. Moreover, the benefits at deep‐discharge conditions can be further promoted by an ultrathin Al2O3 coating. A series of measurements show that the OVs increase the electric conductivity and Na‐ion diffusion coefficient, and the promotion from ultrathin coating lies in the effective reduction of cycling‐induced solid‐electrolyte interphase. The coated nanosheets exhibited high reversible capacity and great rate capability with the capacities of 283.9 (50 mA g−1) and 179.3 mAh g−1 (1 A g−1) after 100 cycles. This work may not only arouse future attention on OVs for sodium energy storage, but also open up new possibilities for designing strategies to utilize defects in other energy storage systems.
The benefits of oxygen vacancies on sodium ion battery performance were demonstrated by using ultrathin Al2O3‐coated MoO3−x nanosheets as anodes. Owing to the increased electric conductivity and sodium ion diffusion coefficient as well as the reduced solid–electrolyte interphase at deep‐discharge conditions, the anodes exhibited high reversible capacity and great rate capability over long‐term cycling. |
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| AbstractList | The utilization of oxygen vacancies (OVs) in sodium ion batteries (SIBs) is expected to enhance performance, but as yet it has rarely been reported. Taking the MoO(3-x) nanosheet anode as an example, for the first time we demonstrate the benefits of OVs on SIB performance. Moreover, the benefits at deep-discharge conditions can be further promoted by an ultrathin Al2O3 coating. A series of measurements show that the OVs increase the electric conductivity and Na-ion diffusion coefficient, and the promotion from ultrathin coating lies in the effective reduction of cycling-induced solid-electrolyte interphase. The coated nanosheets exhibited high reversible capacity and great rate capability with the capacities of 283.9 (50 mA g(-1)) and 179.3 mAh g(-1) (1 A g(-1)) after 100 cycles. This work may not only arouse future attention on OVs for sodium energy storage, but also open up new possibilities for designing strategies to utilize defects in other energy storage systems. The utilization of oxygen vacancies (OVs) in sodium ion batteries (SIBs) is expected to enhance performance, but as yet it has rarely been reported. Taking the MoO sub(3-x) nanosheet anode as an example, for the first time we demonstrate the benefits of OVs on SIB performance. Moreover, the benefits at deep-discharge conditions can be further promoted by an ultrathin Al sub(2)O sub(3) coating. A series of measurements show that the OVs increase the electric conductivity and Na-ion diffusion coefficient, and the promotion from ultrathin coating lies in the effective reduction of cycling-induced solid-electrolyte interphase. The coated nanosheets exhibited high reversible capacity and great rate capability with the capacities of 283.9 (50mAg super(-1)) and 179.3mAhg super(-1) (1Ag super(-1)) after 100 cycles. This work may not only arouse future attention on OVs for sodium energy storage, but also open up new possibilities for designing strategies to utilize defects in other energy storage systems. The benefits of oxygen vacancies on sodium ion battery performance were demonstrated by using ultrathin Al sub(2)O sub(3)-coated MoO sub(3-x) nanosheets as anodes. Owing to the increased electric conductivity and sodium ion diffusion coefficient as well as the reduced solid-electrolyte interphase at deep-discharge conditions, the anodes exhibited high reversible capacity and great rate capability over long-term cycling. The utilization of oxygen vacancies (OVs) in sodium ion batteries (SIBs) is expected to enhance performance, but as yet it has rarely been reported. Taking the MoO 3− x nanosheet anode as an example, for the first time we demonstrate the benefits of OVs on SIB performance. Moreover, the benefits at deep‐discharge conditions can be further promoted by an ultrathin Al 2 O 3 coating. A series of measurements show that the OVs increase the electric conductivity and Na‐ion diffusion coefficient, and the promotion from ultrathin coating lies in the effective reduction of cycling‐induced solid‐electrolyte interphase. The coated nanosheets exhibited high reversible capacity and great rate capability with the capacities of 283.9 (50 mA g −1 ) and 179.3 mAh g −1 (1 A g −1 ) after 100 cycles. This work may not only arouse future attention on OVs for sodium energy storage, but also open up new possibilities for designing strategies to utilize defects in other energy storage systems. The utilization of oxygen vacancies (OVs) in sodium ion batteries (SIBs) is expected to enhance performance, but as yet it has rarely been reported. Taking the MoO3−x nanosheet anode as an example, for the first time we demonstrate the benefits of OVs on SIB performance. Moreover, the benefits at deep‐discharge conditions can be further promoted by an ultrathin Al2O3 coating. A series of measurements show that the OVs increase the electric conductivity and Na‐ion diffusion coefficient, and the promotion from ultrathin coating lies in the effective reduction of cycling‐induced solid‐electrolyte interphase. The coated nanosheets exhibited high reversible capacity and great rate capability with the capacities of 283.9 (50 mA g−1) and 179.3 mAh g−1 (1 A g−1) after 100 cycles. This work may not only arouse future attention on OVs for sodium energy storage, but also open up new possibilities for designing strategies to utilize defects in other energy storage systems. The benefits of oxygen vacancies on sodium ion battery performance were demonstrated by using ultrathin Al2O3‐coated MoO3−x nanosheets as anodes. Owing to the increased electric conductivity and sodium ion diffusion coefficient as well as the reduced solid–electrolyte interphase at deep‐discharge conditions, the anodes exhibited high reversible capacity and great rate capability over long‐term cycling. The utilization of oxygen vacancies (OVs) in sodium ion batteries (SIBs) is expected to enhance performance, but as yet it has rarely been reported. Taking the MoO3-x nanosheet anode as an example, for the first time we demonstrate the benefits of OVs on SIB performance. Moreover, the benefits at deep-discharge conditions can be further promoted by an ultrathin Al2O3 coating. A series of measurements show that the OVs increase the electric conductivity and Na-ion diffusion coefficient, and the promotion from ultrathin coating lies in the effective reduction of cycling-induced solid-electrolyte interphase. The coated nanosheets exhibited high reversible capacity and great rate capability with the capacities of 283.9 (50mAg-1) and 179.3mAhg-1 (1Ag-1) after 100 cycles. This work may not only arouse future attention on OVs for sodium energy storage, but also open up new possibilities for designing strategies to utilize defects in other energy storage systems. |
| Author | Xu, Yang Wang, Chengliang Zhou, Min Wang, Xin Liang, Liying Wu, Minghong Lei, Yong Grote, Fabian Mi, Yan |
| Author_xml | – sequence: 1 givenname: Yang surname: Xu fullname: Xu, Yang organization: Institute für Physics & IMN MacroNano (ZIK), Technische Universität Ilmenau, Prof-Schemidt-Strasse 26, 98693 Ilmenau (Germany) – sequence: 2 givenname: Min surname: Zhou fullname: Zhou, Min organization: Institute für Physics & IMN MacroNano (ZIK), Technische Universität Ilmenau, Prof-Schemidt-Strasse 26, 98693 Ilmenau (Germany) – sequence: 3 givenname: Xin surname: Wang fullname: Wang, Xin organization: Institute of Nanochemistry and Nanobiology, School of Environment and Chemical Engineering, Shanghai University, Shanghai, 200444 (P.R. China) – sequence: 4 givenname: Chengliang surname: Wang fullname: Wang, Chengliang organization: Institute für Physics & IMN MacroNano (ZIK), Technische Universität Ilmenau, Prof-Schemidt-Strasse 26, 98693 Ilmenau (Germany) – sequence: 5 givenname: Liying surname: Liang fullname: Liang, Liying organization: Institute für Physics & IMN MacroNano (ZIK), Technische Universität Ilmenau, Prof-Schemidt-Strasse 26, 98693 Ilmenau (Germany) – sequence: 6 givenname: Fabian surname: Grote fullname: Grote, Fabian organization: Institute für Physics & IMN MacroNano (ZIK), Technische Universität Ilmenau, Prof-Schemidt-Strasse 26, 98693 Ilmenau (Germany) – sequence: 7 givenname: Minghong surname: Wu fullname: Wu, Minghong organization: Institute of Nanochemistry and Nanobiology, School of Environment and Chemical Engineering, Shanghai University, Shanghai, 200444 (P.R. China) – sequence: 8 givenname: Yan surname: Mi fullname: Mi, Yan organization: Institute für Physics & IMN MacroNano (ZIK), Technische Universität Ilmenau, Prof-Schemidt-Strasse 26, 98693 Ilmenau (Germany) – sequence: 9 givenname: Yong surname: Lei fullname: Lei, Yong email: yong.lei@tu-ilmenau.de organization: Institute für Physics & IMN MacroNano (ZIK), Technische Universität Ilmenau, Prof-Schemidt-Strasse 26, 98693 Ilmenau (Germany) |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/26111350$$D View this record in MEDLINE/PubMed |
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| Copyright | 2015 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim |
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| Keywords | alumina nanomaterials sodium ion batteries molybdenum oxygen vacancies |
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| Notes | Shanghai Thousand Talent Plan and Innovative Research Team - No. IRT13078 istex:8745267D800F42F57B44C695B2BC5847DFF938B5 BMBF - No. 03Z1MN11 ark:/67375/WNG-23P99W11-Z ArticleID:ANIE201503477 European Research Council - No. 240144 Volkswagen-Stiftung - No. I/83 984 This work was financially supported by the European Research Council (ThreeDsurface: 240144), BMBF (ZIK-3DNanoDevice: 03Z1MN11), Volkswagen-Stiftung (Herstellung funktionaler Oberflächen: I/83 984), and the Shanghai Thousand Talent Plan and Innovative Research Team (No. IRT13078). We thank Mr. Yong Yan for his assistant of the XRD measurement. We also thank Dr. Xiaodong Zhang for his assistant of the XPS measurement. This work was financially supported by the European Research Council (ThreeDsurface: 240144), BMBF (ZIK‐3DNanoDevice: 03Z1MN11), Volkswagen‐Stiftung (Herstellung funktionaler Oberflächen: I/83 984), and the Shanghai Thousand Talent Plan and Innovative Research Team (No. IRT13078). We thank Mr. Yong Yan for his assistant of the XRD measurement. We also thank Dr. Xiaodong Zhang for his assistant of the XPS measurement. These authors contributed equally to this work. ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 14 content type line 23 |
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| Snippet | The utilization of oxygen vacancies (OVs) in sodium ion batteries (SIBs) is expected to enhance performance, but as yet it has rarely been reported. Taking the... |
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| SubjectTerms | alumina Anodes Coating Diffusion coefficient Electric batteries Electrical conductivity Energy storage molybdenum nanomaterials Nanostructure Oxygen oxygen vacancies Sodium sodium ion batteries Vacancies |
| Title | Enhancement of Sodium Ion Battery Performance Enabled by Oxygen Vacancies |
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