Approaching White-Light Emission from a Phosphorescent Trinuclear Gold(I) Cluster by Modulating Its Aggregation Behavior

White light: [{Au(L)}3] (L=3‐(2‐thienyl)pyrazolate) gives dual emission, one from an organic chromophore the other from aurophilic stacking interactions. The resulting blue–green and orange–red emissions can be tuned to approach white‐light by modulating the aggregation behavior of the cluster....

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Published inAngewandte Chemie International Edition Vol. 52; no. 50; pp. 13472 - 13476
Main Authors Ni, Wen-Xiu, Li, Mian, Zheng, Ji, Zhan, Shun-Ze, Qiu, Yu-Min, Ng, Seik Weng, Li, Dan
Format Journal Article
LanguageEnglish
Published Weinheim WILEY-VCH Verlag 09.12.2013
WILEY‐VCH Verlag
Wiley Subscription Services, Inc
EditionInternational ed. in English
Subjects
Agglomeration
aurophilicity
Chromophores
Clusters
Emission
excited states
gold cluster
phosphorescence
Stacking
White light
white light emission
gold cluster
aurophilicity
phosphorescence
excited states
white light emission
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Abstract White light: [{Au(L)}3] (L=3‐(2‐thienyl)pyrazolate) gives dual emission, one from an organic chromophore the other from aurophilic stacking interactions. The resulting blue–green and orange–red emissions can be tuned to approach white‐light by modulating the aggregation behavior of the cluster.
AbstractList White light: [{Au(L)}3] (L=3‐(2‐thienyl)pyrazolate) gives dual emission, one from an organic chromophore the other from aurophilic stacking interactions. The resulting blue–green and orange–red emissions can be tuned to approach white‐light by modulating the aggregation behavior of the cluster.
White light: [{Au(L)} sub(3)] (L=3-(2-thienyl)pyrazolate) gives dual emission, one from an organic chromophore the other from aurophilic stacking interactions. The resulting blue-green and orange-red emissions can be tuned to approach white-light by modulating the aggregation behavior of the cluster.
Author Zheng, Ji
Zhan, Shun-Ze
Qiu, Yu-Min
Li, Dan
Ni, Wen-Xiu
Li, Mian
Ng, Seik Weng
Author_xml – sequence: 1
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  fullname: Li, Mian
  organization: Department of Chemistry and Research Institute for Biomedical and Advanced Materials, Shantou University, Guangdong 515063 (P. R. China)
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  surname: Zheng
  fullname: Zheng, Ji
  organization: Department of Chemistry and Research Institute for Biomedical and Advanced Materials, Shantou University, Guangdong 515063 (P. R. China)
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  givenname: Shun-Ze
  surname: Zhan
  fullname: Zhan, Shun-Ze
  organization: Department of Chemistry and Research Institute for Biomedical and Advanced Materials, Shantou University, Guangdong 515063 (P. R. China)
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  givenname: Yu-Min
  surname: Qiu
  fullname: Qiu, Yu-Min
  organization: Department of Chemistry and Research Institute for Biomedical and Advanced Materials, Shantou University, Guangdong 515063 (P. R. China)
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  surname: Ng
  fullname: Ng, Seik Weng
  organization: Department of Chemistry, University of Malaya, 50603 Kuala Lumpur (Malaysia)
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  surname: Li
  fullname: Li, Dan
  email: dli@stu.edu.cn
  organization: Department of Chemistry and Research Institute for Biomedical and Advanced Materials, Shantou University, Guangdong 515063 (P. R. China)
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Keywords gold cluster
aurophilicity
phosphorescence
excited states
white light emission
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Notes The work was supported by 973 Program (Nos. 2013CB834803 and 2012CB821706), the National Natural Science Foundation for Distinguished Young Scholars of China (No. 20825102), and the National Natural Science Foundation of China (Nos. 21171114 and 91222202). W.-X.N. thanks the funding of China Postdoctoral Science Foundation (No. 2012M521622) and Guangdong Natural Science Foundation (No. S2012040006968). S.W.N. thanks the funding of the Ministry of Higher Education of Malaysia (Grant No. UM.C/HIR-MOHE/SC/03). We thank Prof. Tai-Chu Lau of the City University of Hong Kong for help on physical measurements.
Guangdong Natural Science Foundation - No. S2012040006968
Ministry of Higher Education of Malaysia - No. UM.C/HIR-MOHE/SC/03
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National Natural Science Foundation of China - No. 21171114; No. 91222202
The work was supported by 973 Program (Nos. 2013CB834803 and 2012CB821706), the National Natural Science Foundation for Distinguished Young Scholars of China (No. 20825102), and the National Natural Science Foundation of China (Nos. 21171114 and 91222202). W.‐X.N. thanks the funding of China Postdoctoral Science Foundation (No. 2012M521622) and Guangdong Natural Science Foundation (No. S2012040006968). S.W.N. thanks the funding of the Ministry of Higher Education of Malaysia (Grant No. UM.C/HIR‐MOHE/SC/03). We thank Prof. Tai‐Chu Lau of the City University of Hong Kong for help on physical measurements.
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2013; 19
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2008; 20
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2008
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2006
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2011; 255
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2009 2009; 121 48
2011; 133
2006; 45
2004; 16
2002; 124
2007; 111
2005; 127
2005; 249
2010; 132
2011; 44
2012 2012; 124 51
2012; 48
2011; 47
2005; 94
2007 2007; 119 46
2012; 7
2008; 130
2012; 41
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Snippet White light: [{Au(L)}3] (L=3‐(2‐thienyl)pyrazolate) gives dual emission, one from an organic chromophore the other from aurophilic stacking interactions. The...
White light: [{Au(L)} sub(3)] (L=3-(2-thienyl)pyrazolate) gives dual emission, one from an organic chromophore the other from aurophilic stacking interactions....
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SubjectTerms Agglomeration
aurophilicity
Chromophores
Clusters
Emission
excited states
gold cluster
phosphorescence
Stacking
White light
white light emission
Title Approaching White-Light Emission from a Phosphorescent Trinuclear Gold(I) Cluster by Modulating Its Aggregation Behavior
URI https://api.istex.fr/ark:/67375/WNG-9X9LR82B-3/fulltext.pdf
https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fanie.201308135
https://www.ncbi.nlm.nih.gov/pubmed/24254790
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Volume 52
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