Space-Confinement-Induced Synthesis of Pyridinic- and Pyrrolic-Nitrogen-Doped Graphene for the Catalysis of Oxygen Reduction
Forced obedience: Layer‐structured montmorillonite (MMT) was used as a nanoreactor for the generation of planar pyridinic and pyrrolic N sites in nitrogen‐doped graphene (NG; see picture). The selectivity for the formation of planar N sites was inversely proportional to the interspace width (δ) of t...
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| Published in | Angewandte Chemie International Edition Vol. 52; no. 45; pp. 11755 - 11759 |
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| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Weinheim
WILEY-VCH Verlag
04.11.2013
WILEY‐VCH Verlag Wiley Subscription Services, Inc |
| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Forced obedience: Layer‐structured montmorillonite (MMT) was used as a nanoreactor for the generation of planar pyridinic and pyrrolic N sites in nitrogen‐doped graphene (NG; see picture). The selectivity for the formation of planar N sites was inversely proportional to the interspace width (δ) of the MMT and reached a maximum of 90.27 %. The NG catalyst exhibited low electrical resistance, high electrocatalytic activity, and good stability. |
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| AbstractList | Forced obedience: Layer-structured montmorillonite (MMT) was used as a nanoreactor for the generation of planar pyridinic and pyrrolic Nsites in nitrogen-doped graphene (NG; see picture). The selectivity for the formation of planar N sites was inversely proportional to the interspace width (δ) of the MMT and reached a maximum of 90.27%. The NG catalyst exhibited low electrical resistance, high electrocatalytic activity, and good stability. Forced obedience: Layer‐structured montmorillonite (MMT) was used as a nanoreactor for the generation of planar pyridinic and pyrrolic N sites in nitrogen‐doped graphene (NG; see picture). The selectivity for the formation of planar N sites was inversely proportional to the interspace width (δ) of the MMT and reached a maximum of 90.27 %. The NG catalyst exhibited low electrical resistance, high electrocatalytic activity, and good stability. Forced obedience: Layer-structured montmorillonite (MMT) was used as a nanoreactor for the generation of planar pyridinic and pyrrolic Nsites in nitrogen-doped graphene (NG; see picture). The selectivity for the formation of planar N sites was inversely proportional to the interspace width ([delta]) of the MMT and reached a maximum of 90.27%. The NG catalyst exhibited low electrical resistance, high electrocatalytic activity, and good stability. |
| Author | Li, Li Yang, Tao Wang, Dong Qi, Xueqiang Wan, Li-Jun Chen, Siguo Hu, Jinsong Alvi, Shahnaz Fatima Wei, Zidong Ding, Wei |
| Author_xml | – sequence: 1 givenname: Wei surname: Ding fullname: Ding, Wei organization: The State Key Laboratory of Power Transmission Equipment and System Security and New Technology, College of Chemistry and Chemical Engineering, Chongqing University, Shapingba 174, Chongqing (China) – sequence: 2 givenname: Zidong surname: Wei fullname: Wei, Zidong email: zdwei@cqu.edu.cn organization: The State Key Laboratory of Power Transmission Equipment and System Security and New Technology, College of Chemistry and Chemical Engineering, Chongqing University, Shapingba 174, Chongqing (China) – sequence: 3 givenname: Siguo surname: Chen fullname: Chen, Siguo organization: The State Key Laboratory of Power Transmission Equipment and System Security and New Technology, College of Chemistry and Chemical Engineering, Chongqing University, Shapingba 174, Chongqing (China) – sequence: 4 givenname: Xueqiang surname: Qi fullname: Qi, Xueqiang organization: The State Key Laboratory of Power Transmission Equipment and System Security and New Technology, College of Chemistry and Chemical Engineering, Chongqing University, Shapingba 174, Chongqing (China) – sequence: 5 givenname: Tao surname: Yang fullname: Yang, Tao organization: The State Key Laboratory of Power Transmission Equipment and System Security and New Technology, College of Chemistry and Chemical Engineering, Chongqing University, Shapingba 174, Chongqing (China) – sequence: 6 givenname: Jinsong surname: Hu fullname: Hu, Jinsong organization: Institute of Chemistry, The Chinese Academy of Sciences, Beijing 100190 (China) – sequence: 7 givenname: Dong surname: Wang fullname: Wang, Dong organization: Institute of Chemistry, The Chinese Academy of Sciences, Beijing 100190 (China) – sequence: 8 givenname: Li-Jun surname: Wan fullname: Wan, Li-Jun email: wanlijun@iccas.ac.cn organization: Institute of Chemistry, The Chinese Academy of Sciences, Beijing 100190 (China) – sequence: 9 givenname: Shahnaz Fatima surname: Alvi fullname: Alvi, Shahnaz Fatima organization: The State Key Laboratory of Power Transmission Equipment and System Security and New Technology, College of Chemistry and Chemical Engineering, Chongqing University, Shapingba 174, Chongqing (China) – sequence: 10 givenname: Li surname: Li fullname: Li, Li organization: The State Key Laboratory of Power Transmission Equipment and System Security and New Technology, College of Chemistry and Chemical Engineering, Chongqing University, Shapingba 174, Chongqing (China) |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/24038758$$D View this record in MEDLINE/PubMed |
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| CODEN | ACIEAY |
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| Keywords | fuel cells space confinement electrocatalysis N-doped graphene oxygen reduction |
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| PublicationDecade | 2010 |
| PublicationPlace | Weinheim |
| PublicationPlace_xml | – name: Weinheim – name: Germany |
| PublicationTitle | Angewandte Chemie International Edition |
| PublicationTitleAlternate | Angew. Chem. Int. Ed |
| PublicationYear | 2013 |
| Publisher | WILEY-VCH Verlag WILEY‐VCH Verlag Wiley Subscription Services, Inc |
| Publisher_xml | – name: WILEY-VCH Verlag – name: WILEY‐VCH Verlag – name: Wiley Subscription Services, Inc |
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| Snippet | Forced obedience: Layer‐structured montmorillonite (MMT) was used as a nanoreactor for the generation of planar pyridinic and pyrrolic N sites in... Forced obedience: Layer-structured montmorillonite (MMT) was used as a nanoreactor for the generation of planar pyridinic and pyrrolic Nsites in nitrogen-doped... |
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| SubjectTerms | Catalysis Deltas Electrical resistance electrocatalysis Formations fuel cells Graphene Montmorillonite N-doped graphene Nanostructure Nitrogen oxygen reduction space confinement Stability Synthesis |
| Title | Space-Confinement-Induced Synthesis of Pyridinic- and Pyrrolic-Nitrogen-Doped Graphene for the Catalysis of Oxygen Reduction |
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