On the Importance of Morphology Control in Polymer Solar Cells

Nanostructured polymer‐based solar cells (PSCs) have emerged as a promising low‐cost alternative to conventional inorganic photovoltaic devices and are now a subject of intensive research both in academia and industry. For PSCs to become practical efficient devices, several issues should still be ad...

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Published inMacromolecular rapid communications. Vol. 31; no. 21; pp. 1835 - 1845
Main Authors van Bavel, Svetlana, Veenstra, Sjoerd, Loos, Joachim
Format Journal Article
LanguageEnglish
Published Weinheim WILEY-VCH Verlag 01.11.2010
WILEY‐VCH Verlag
Wiley
Subjects
Application fields
Applied sciences
bulk heterojunction
Devices
electron tomography
Energy
Exact sciences and technology
Heterojunctions
Morphology
Nanocomposites
Nanomaterials
Nanostructure
Natural energy
Photovoltaic cells
Photovoltaic conversion
Polymer industry, paints, wood
polymer solar cells
Solar cells
Solar cells. Photoelectrochemical cells
Solar energy
Technology of polymers
films
bulk heterojunction
Morphology
Polymer
Property structure relationship
polymer solar cells
Review
Surface topography
Organic solar cells
electron tomography
Electrical characteristic
Heterojunction
Online AccessGet full text
ISSN1022-1336
1521-3927
1521-3927
DOI10.1002/marc.201000080

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Abstract Nanostructured polymer‐based solar cells (PSCs) have emerged as a promising low‐cost alternative to conventional inorganic photovoltaic devices and are now a subject of intensive research both in academia and industry. For PSCs to become practical efficient devices, several issues should still be addressed, including further understanding of their operation and stability, which in turn are largely determined by the morphological organisation in the photoactive layer. The latter is typically a few hundred nanometres thick film and is a blend composed of two materials: the bulk heterojunction consisting of the electron donor and the electron acceptor. The main requirements for the morphology of efficient photoactive layers are nanoscale phase segregation for a high donor/acceptor interface area and hence efficient exciton dissociation, short and continuous percolation pathways of both components leading through the layer thickness to the corresponding electrodes for efficient charge transport and collection, and high crystallinity of both donor and acceptor materials for high charge mobility. In this paper, we review recent progress of our understanding on how the efficiency of a bulk heterojunction PSC largely depends on the local nanoscale volume organisation of the photoactive layer. The volume morphology of the bulk heterojunction photoactive layer determines the performance of polymer solar cells. In this paper the critical parameters are discussed influencing morphology creation and thus the ultimate light conversion efficiency for a given electron acceptor and donor system.
AbstractList Nanostructured polymer-based solar cells (PSCs) have emerged as a promising low-cost alternative to conventional inorganic photovoltaic devices and are now a subject of intensive research both in academia and industry. For PSCs to become practical efficient devices, several issues should still be addressed, including further understanding of their operation and stability, which in turn are largely determined by the morphological organisation in the photoactive layer. The latter is typically a few hundred nanometres thick film and is a blend composed of two materials: the bulk heterojunction consisting of the electron donor and the electron acceptor. The main requirements for the morphology of efficient photoactive layers are nanoscale phase segregation for a high donor/acceptor interface area and hence efficient exciton dissociation, short and continuous percolation pathways of both components leading through the layer thickness to the corresponding electrodes for efficient charge transport and collection, and high crystallinity of both donor and acceptor materials for high charge mobility. In this paper, we review recent progress of our understanding on how the efficiency of a bulk heterojunction PSC largely depends on the local nanoscale volume organisation of the photoactive layer.
Nanostructured polymer‐based solar cells (PSCs) have emerged as a promising low‐cost alternative to conventional inorganic photovoltaic devices and are now a subject of intensive research both in academia and industry. For PSCs to become practical efficient devices, several issues should still be addressed, including further understanding of their operation and stability, which in turn are largely determined by the morphological organisation in the photoactive layer. The latter is typically a few hundred nanometres thick film and is a blend composed of two materials: the bulk heterojunction consisting of the electron donor and the electron acceptor. The main requirements for the morphology of efficient photoactive layers are nanoscale phase segregation for a high donor/acceptor interface area and hence efficient exciton dissociation, short and continuous percolation pathways of both components leading through the layer thickness to the corresponding electrodes for efficient charge transport and collection, and high crystallinity of both donor and acceptor materials for high charge mobility. In this paper, we review recent progress of our understanding on how the efficiency of a bulk heterojunction PSC largely depends on the local nanoscale volume organisation of the photoactive layer. magnified image
Nanostructured polymer-based solar cells (PSCs) have emerged as a promising low-cost alternative to conventional inorganic photovoltaic devices and are now a subject of intensive research both in academia and industry. For PSCs to become practical efficient devices, several issues should still be addressed, including further understanding of their operation and stability, which in turn are largely determined by the morphological organisation in the photoactive layer. The latter is typically a few hundred nanometres thick film and is a blend composed of two materials: the bulk heterojunction consisting of the electron donor and the electron acceptor. The main requirements for the morphology of efficient photoactive layers are nanoscale phase segregation for a high donor/acceptor interface area and hence efficient exciton dissociation, short and continuous percolation pathways of both components leading through the layer thickness to the corresponding electrodes for efficient charge transport and collection, and high crystallinity of both donor and acceptor materials for high charge mobility. In this paper, we review recent progress of our understanding on how the efficiency of a bulk heterojunction PSC largely depends on the local nanoscale volume organisation of the photoactive layer.Nanostructured polymer-based solar cells (PSCs) have emerged as a promising low-cost alternative to conventional inorganic photovoltaic devices and are now a subject of intensive research both in academia and industry. For PSCs to become practical efficient devices, several issues should still be addressed, including further understanding of their operation and stability, which in turn are largely determined by the morphological organisation in the photoactive layer. The latter is typically a few hundred nanometres thick film and is a blend composed of two materials: the bulk heterojunction consisting of the electron donor and the electron acceptor. The main requirements for the morphology of efficient photoactive layers are nanoscale phase segregation for a high donor/acceptor interface area and hence efficient exciton dissociation, short and continuous percolation pathways of both components leading through the layer thickness to the corresponding electrodes for efficient charge transport and collection, and high crystallinity of both donor and acceptor materials for high charge mobility. In this paper, we review recent progress of our understanding on how the efficiency of a bulk heterojunction PSC largely depends on the local nanoscale volume organisation of the photoactive layer.
Nanostructured polymer‐based solar cells (PSCs) have emerged as a promising low‐cost alternative to conventional inorganic photovoltaic devices and are now a subject of intensive research both in academia and industry. For PSCs to become practical efficient devices, several issues should still be addressed, including further understanding of their operation and stability, which in turn are largely determined by the morphological organisation in the photoactive layer. The latter is typically a few hundred nanometres thick film and is a blend composed of two materials: the bulk heterojunction consisting of the electron donor and the electron acceptor. The main requirements for the morphology of efficient photoactive layers are nanoscale phase segregation for a high donor/acceptor interface area and hence efficient exciton dissociation, short and continuous percolation pathways of both components leading through the layer thickness to the corresponding electrodes for efficient charge transport and collection, and high crystallinity of both donor and acceptor materials for high charge mobility. In this paper, we review recent progress of our understanding on how the efficiency of a bulk heterojunction PSC largely depends on the local nanoscale volume organisation of the photoactive layer. The volume morphology of the bulk heterojunction photoactive layer determines the performance of polymer solar cells. In this paper the critical parameters are discussed influencing morphology creation and thus the ultimate light conversion efficiency for a given electron acceptor and donor system.
Author van Bavel, Svetlana
Veenstra, Sjoerd
Loos, Joachim
Author_xml – sequence: 1
  givenname: Svetlana
  surname: van Bavel
  fullname: van Bavel, Svetlana
  organization: Dutch Polymer Institute, P.O. Box 902, 5600 AX Eindhoven, The Netherlands
– sequence: 2
  givenname: Sjoerd
  surname: Veenstra
  fullname: Veenstra, Sjoerd
  organization: Dutch Polymer Institute, P.O. Box 902, 5600 AX Eindhoven, The Netherlands
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  givenname: Joachim
  surname: Loos
  fullname: Loos, Joachim
  email: j.loos@physics.gla.ac.uk
  organization: Dutch Polymer Institute, P.O. Box 902, 5600 AX Eindhoven, The Netherlands
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Issue 21
Keywords films
bulk heterojunction
Morphology
Polymer
Property structure relationship
polymer solar cells
Review
Surface topography
Organic solar cells
electron tomography
Electrical characteristic
Heterojunction
Language English
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Snippet Nanostructured polymer‐based solar cells (PSCs) have emerged as a promising low‐cost alternative to conventional inorganic photovoltaic devices and are now a...
Nanostructured polymer-based solar cells (PSCs) have emerged as a promising low-cost alternative to conventional inorganic photovoltaic devices and are now a...
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SubjectTerms Application fields
Applied sciences
bulk heterojunction
Devices
electron tomography
Energy
Exact sciences and technology
Heterojunctions
Morphology
Nanocomposites
Nanomaterials
Nanostructure
Natural energy
Photovoltaic cells
Photovoltaic conversion
Polymer industry, paints, wood
polymer solar cells
Solar cells
Solar cells. Photoelectrochemical cells
Solar energy
Technology of polymers
Title On the Importance of Morphology Control in Polymer Solar Cells
URI https://api.istex.fr/ark:/67375/WNG-X484F1JN-K/fulltext.pdf
https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fmarc.201000080
https://www.ncbi.nlm.nih.gov/pubmed/21567602
https://www.proquest.com/docview/866536524
https://www.proquest.com/docview/901660009
Volume 31
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