Iodine immobilization by materials through sorption and redox-driven processes: A literature review
Radioiodine-129 (129I) in the subsurface is mobile and limited information is available on treatment technologies. Scientific literature was reviewed to compile information on materials that could potentially be used to immobilize 129I through sorption and redox-driven processes, with an emphasis on...
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| Published in | The Science of the total environment Vol. 716; p. 132820 |
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| Main Authors | , , , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Netherlands
Elsevier B.V
10.05.2020
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| Abstract | Radioiodine-129 (129I) in the subsurface is mobile and limited information is available on treatment technologies. Scientific literature was reviewed to compile information on materials that could potentially be used to immobilize 129I through sorption and redox-driven processes, with an emphasis on ex-situ processes. Candidate materials to immobilize 129I include iron minerals, sulfur-based materials, silver-based materials, bismuth-based materials, ion exchange resins, activated carbon, modified clays, and tailored materials (metal organic frameworks (MOFS), layered double hydroxides (LDHs) and aerogels). Where available, compiled information includes material performance in terms of (i) capacity for 129I uptake; (ii) long-term performance (i.e., solubility of a precipitated phase); (iii) technology maturity; (iv) cost; (v) available quantity; (vi) environmental impact; (vii) ability to emplace the technology for in situ use at the field-scale; and (viii) ex situ treatment (for media extracted from the subsurface or secondary waste streams). Because it can be difficult to compare materials due to differences in experimental conditions applied in the literature, materials will be selected for subsequent standardized batch loading tests.
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•Iodine immobilization processes include precipitation, sorption or encapsulation.•Fe, Cu & Bi materials sorb iodine species & are useful for remediation.•Bi materials are readily available, inexpensive & insensitive to redox processes.•IX resins, activated carbon & organoclays are effective sorbants for I− but not IO3−.•MOFs, LDHs & aerogels require further investigation for iodine immobilization. |
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| AbstractList | Radioiodine-129 (129I) in the subsurface is mobile and limited information is available on treatment technologies. Scientific literature was reviewed to compile information on materials that could potentially be used to immobilize 129I through sorption and redox-driven processes, with an emphasis on ex-situ processes. Candidate materials to immobilize 129I include iron minerals, sulfur-based materials, silver-based materials, bismuth-based materials, ion exchange resins, activated carbon, modified clays, and tailored materials (metal organic frameworks (MOFS), layered double hydroxides (LDHs) and aerogels). Where available, compiled information includes material performance in terms of (i) capacity for 129I uptake; (ii) long-term performance (i.e., solubility of a precipitated phase); (iii) technology maturity; (iv) cost; (v) available quantity; (vi) environmental impact; (vii) ability to emplace the technology for in situ use at the field-scale; and (viii) ex situ treatment (for media extracted from the subsurface or secondary waste streams). Because it can be difficult to compare materials due to differences in experimental conditions applied in the literature, materials will be selected for subsequent standardized batch loading tests.Radioiodine-129 (129I) in the subsurface is mobile and limited information is available on treatment technologies. Scientific literature was reviewed to compile information on materials that could potentially be used to immobilize 129I through sorption and redox-driven processes, with an emphasis on ex-situ processes. Candidate materials to immobilize 129I include iron minerals, sulfur-based materials, silver-based materials, bismuth-based materials, ion exchange resins, activated carbon, modified clays, and tailored materials (metal organic frameworks (MOFS), layered double hydroxides (LDHs) and aerogels). Where available, compiled information includes material performance in terms of (i) capacity for 129I uptake; (ii) long-term performance (i.e., solubility of a precipitated phase); (iii) technology maturity; (iv) cost; (v) available quantity; (vi) environmental impact; (vii) ability to emplace the technology for in situ use at the field-scale; and (viii) ex situ treatment (for media extracted from the subsurface or secondary waste streams). Because it can be difficult to compare materials due to differences in experimental conditions applied in the literature, materials will be selected for subsequent standardized batch loading tests. Radioiodine-129 (129I) in the subsurface is mobile and limited information is available on treatment technologies. Scientific literature was reviewed to compile information on materials that could potentially be used to immobilize 129I through sorption and redox-driven processes, with an emphasis on ex-situ processes. Candidate materials to immobilize 129I include iron minerals, sulfur-based materials, silver-based materials, bismuth-based materials, ion exchange resins, activated carbon, modified clays, and tailored materials (metal organic frameworks (MOFS), layered double hydroxides (LDHs) and aerogels). Where available, compiled information includes material performance in terms of (i) capacity for 129I uptake; (ii) long-term performance (i.e., solubility of a precipitated phase); (iii) technology maturity; (iv) cost; (v) available quantity; (vi) environmental impact; (vii) ability to emplace the technology for in situ use at the field-scale; and (viii) ex situ treatment (for media extracted from the subsurface or secondary waste streams). Because it can be difficult to compare materials due to differences in experimental conditions applied in the literature, materials will be selected for subsequent standardized batch loading tests. [Display omitted] •Iodine immobilization processes include precipitation, sorption or encapsulation.•Fe, Cu & Bi materials sorb iodine species & are useful for remediation.•Bi materials are readily available, inexpensive & insensitive to redox processes.•IX resins, activated carbon & organoclays are effective sorbants for I− but not IO3−.•MOFs, LDHs & aerogels require further investigation for iodine immobilization. Radioiodine-129 ( I) in the subsurface is mobile and limited information is available on treatment technologies. Scientific literature was reviewed to compile information on materials that could potentially be used to immobilize I through sorption and redox-driven processes, with an emphasis on ex-situ processes. Candidate materials to immobilize I include iron minerals, sulfur-based materials, silver-based materials, bismuth-based materials, ion exchange resins, activated carbon, modified clays, and tailored materials (metal organic frameworks (MOFS), layered double hydroxides (LDHs) and aerogels). Where available, compiled information includes material performance in terms of (i) capacity for I uptake; (ii) long-term performance (i.e., solubility of a precipitated phase); (iii) technology maturity; (iv) cost; (v) available quantity; (vi) environmental impact; (vii) ability to emplace the technology for in situ use at the field-scale; and (viii) ex situ treatment (for media extracted from the subsurface or secondary waste streams). Because it can be difficult to compare materials due to differences in experimental conditions applied in the literature, materials will be selected for subsequent standardized batch loading tests. Radioiodine-129 (¹²⁹I) in the subsurface is mobile and limited information is available on treatment technologies. Scientific literature was reviewed to compile information on materials that could potentially be used to immobilize ¹²⁹I through sorption and redox-driven processes, with an emphasis on ex-situ processes. Candidate materials to immobilize ¹²⁹I include iron minerals, sulfur-based materials, silver-based materials, bismuth-based materials, ion exchange resins, activated carbon, modified clays, and tailored materials (metal organic frameworks (MOFS), layered double hydroxides (LDHs) and aerogels). Where available, compiled information includes material performance in terms of (i) capacity for ¹²⁹I uptake; (ii) long-term performance (i.e., solubility of a precipitated phase); (iii) technology maturity; (iv) cost; (v) available quantity; (vi) environmental impact; (vii) ability to emplace the technology for in situ use at the field-scale; and (viii) ex situ treatment (for media extracted from the subsurface or secondary waste streams). Because it can be difficult to compare materials due to differences in experimental conditions applied in the literature, materials will be selected for subsequent standardized batch loading tests. |
| ArticleNumber | 132820 |
| Author | Saslow, Sarah A. Levitskaia, Tatiana G. Szecsody, Jim E. Freedman, Vicky L. Pearce, Carolyn I. Lawter, Amanda R. Moore, Robert C. Asmussen, Robert M. Neeway, James J. Thallapally, Praveen K. Chatterjee, Sayandev Wang, Guohui Morad, Joseph W. Qafoku, Nikolla P. Rigali, Mark J. |
| Author_xml | – sequence: 1 givenname: Robert C. surname: Moore fullname: Moore, Robert C. organization: Pacific Northwest National Laboratory, Richland, WA, United States of America – sequence: 2 givenname: Carolyn I. orcidid: 0000-0003-3098-1615 surname: Pearce fullname: Pearce, Carolyn I. email: carolyn.pearce@pnnl.gov organization: Pacific Northwest National Laboratory, Richland, WA, United States of America – sequence: 3 givenname: Joseph W. surname: Morad fullname: Morad, Joseph W. organization: Pacific Northwest National Laboratory, Richland, WA, United States of America – sequence: 4 givenname: Sayandev orcidid: 0000-0003-2218-5635 surname: Chatterjee fullname: Chatterjee, Sayandev organization: Pacific Northwest National Laboratory, Richland, WA, United States of America – sequence: 5 givenname: Tatiana G. surname: Levitskaia fullname: Levitskaia, Tatiana G. organization: Pacific Northwest National Laboratory, Richland, WA, United States of America – sequence: 6 givenname: Robert M. surname: Asmussen fullname: Asmussen, Robert M. organization: Pacific Northwest National Laboratory, Richland, WA, United States of America – sequence: 7 givenname: Amanda R. surname: Lawter fullname: Lawter, Amanda R. organization: Pacific Northwest National Laboratory, Richland, WA, United States of America – sequence: 8 givenname: James J. surname: Neeway fullname: Neeway, James J. organization: Pacific Northwest National Laboratory, Richland, WA, United States of America – sequence: 9 givenname: Nikolla P. surname: Qafoku fullname: Qafoku, Nikolla P. organization: Pacific Northwest National Laboratory, Richland, WA, United States of America – sequence: 10 givenname: Mark J. surname: Rigali fullname: Rigali, Mark J. organization: Sandia National Laboratories, Albuquerque, NM, United States of America – sequence: 11 givenname: Sarah A. surname: Saslow fullname: Saslow, Sarah A. organization: Pacific Northwest National Laboratory, Richland, WA, United States of America – sequence: 12 givenname: Jim E. surname: Szecsody fullname: Szecsody, Jim E. organization: Pacific Northwest National Laboratory, Richland, WA, United States of America – sequence: 13 givenname: Praveen K. surname: Thallapally fullname: Thallapally, Praveen K. organization: Pacific Northwest National Laboratory, Richland, WA, United States of America – sequence: 14 givenname: Guohui surname: Wang fullname: Wang, Guohui organization: Pacific Northwest National Laboratory, Richland, WA, United States of America – sequence: 15 givenname: Vicky L. surname: Freedman fullname: Freedman, Vicky L. organization: Pacific Northwest National Laboratory, Richland, WA, United States of America |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/31982189$$D View this record in MEDLINE/PubMed |
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| Keywords | Bismuth-based materials Metal organic frameworks Sorbents Subsurface contamination Hydroxyapatite Iron oxides Iodine Layered double hydroxides |
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| Snippet | Radioiodine-129 (129I) in the subsurface is mobile and limited information is available on treatment technologies. Scientific literature was reviewed to... Radioiodine-129 ( I) in the subsurface is mobile and limited information is available on treatment technologies. Scientific literature was reviewed to compile... Radioiodine-129 (¹²⁹I) in the subsurface is mobile and limited information is available on treatment technologies. Scientific literature was reviewed to... |
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| SubjectTerms | activated carbon aerogels Bismuth-based materials coordination polymers environmental impact hydroxides Hydroxyapatite Iodine ion exchange resins iron Iron oxides Layered double hydroxides Metal organic frameworks minerals radionuclides solubility Sorbents sorption Subsurface contamination |
| Title | Iodine immobilization by materials through sorption and redox-driven processes: A literature review |
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