A Rational Approach to Organo‐Photocatalysis: Novel Designs and Structure‐Property Relationships
Organic photocatalysts are emerging as viable and more sustainable tools than metal complexes. Recently, the field of organo‐photocatalysis has experienced an explosion in terms of applications, redesign of well‐established systems, and identification of novel scaffolds. A rational approach to the s...
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| Published in | Angewandte Chemie International Edition Vol. 60; no. 3; pp. 1082 - 1097 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
18.01.2021
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| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
| ISSN | 1433-7851 1521-3773 1521-3773 |
| DOI | 10.1002/anie.202006416 |
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| Abstract | Organic photocatalysts are emerging as viable and more sustainable tools than metal complexes. Recently, the field of organo‐photocatalysis has experienced an explosion in terms of applications, redesign of well‐established systems, and identification of novel scaffolds. A rational approach to the structural modification of the different photocatalysts is key to accessing unprecedented reactivity, while improving their catalytic performances. We herein discuss the concepts underpinning the scaffold modification of some of the most recently used photocatalysts and analyze how specific structural changes alter their physicochemical and redox properties.
No more trial and error! This Minireview outlines how a careful physicochemical properties analysis is instrumental towards the rational selection of a photocatalyst while delineating future applications and structural evolution. |
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| AbstractList | Organic photocatalysts are emerging as viable and more sustainable tools than metal complexes. Recently, the field of organo‐photocatalysis has experienced an explosion in terms of applications, redesign of well‐established systems, and identification of novel scaffolds. A rational approach to the structural modification of the different photocatalysts is key to accessing unprecedented reactivity, while improving their catalytic performances. We herein discuss the concepts underpinning the scaffold modification of some of the most recently used photocatalysts and analyze how specific structural changes alter their physicochemical and redox properties.
No more trial and error! This Minireview outlines how a careful physicochemical properties analysis is instrumental towards the rational selection of a photocatalyst while delineating future applications and structural evolution. Organic photocatalysts are emerging as viable and more sustainable tools than metal complexes. Recently, the field of organo-photocatalysis has experienced an explosion in terms of applications, redesign of well-established systems, and identification of novel scaffolds. A rational approach to the structural modification of the different photocatalysts is key to accessing unprecedented reactivity, while improving their catalytic performances. We herein discuss the concepts underpinning the scaffold modification of some of the most recently used photocatalysts and analyze how specific structural changes alter their physicochemical and redox properties. Organic photocatalysts are emerging as viable and more sustainable tools than metal complexes. Recently, the field of organo-photocatalysis has experienced an explosion in terms of applications, redesign of well-established systems, and identification of novel scaffolds. A rational approach to the structural modification of the different photocatalysts is key to accessing unprecedented reactivity, while improving their catalytic performances. We herein discuss the concepts underpinning the scaffold modification of some of the most recently used photocatalysts and analyze how specific structural changes alter their physicochemical and redox properties.Organic photocatalysts are emerging as viable and more sustainable tools than metal complexes. Recently, the field of organo-photocatalysis has experienced an explosion in terms of applications, redesign of well-established systems, and identification of novel scaffolds. A rational approach to the structural modification of the different photocatalysts is key to accessing unprecedented reactivity, while improving their catalytic performances. We herein discuss the concepts underpinning the scaffold modification of some of the most recently used photocatalysts and analyze how specific structural changes alter their physicochemical and redox properties. |
| Author | Dell'Amico, Luca Escudero‐Casao, Margarita Companyó, Xavier Mateos, Javier Vega‐Peñaloza, Alberto |
| Author_xml | – sequence: 1 givenname: Alberto orcidid: 0000-0003-0374-8033 surname: Vega‐Peñaloza fullname: Vega‐Peñaloza, Alberto organization: University of Padova – sequence: 2 givenname: Javier orcidid: 0000-0002-2358-9183 surname: Mateos fullname: Mateos, Javier organization: University of Padova – sequence: 3 givenname: Xavier orcidid: 0000-0001-8969-7315 surname: Companyó fullname: Companyó, Xavier organization: University of Padova – sequence: 4 givenname: Margarita surname: Escudero‐Casao fullname: Escudero‐Casao, Margarita organization: University of Padova – sequence: 5 givenname: Luca orcidid: 0000-0003-0423-9628 surname: Dell'Amico fullname: Dell'Amico, Luca email: luca.dellamico@unipd.it organization: University of Padova |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/32568437$$D View this record in MEDLINE/PubMed |
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| Keywords | organocatalysis synthetic photochemistry photoredox catalysis photocatalysis catalyst design |
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| Snippet | Organic photocatalysts are emerging as viable and more sustainable tools than metal complexes. Recently, the field of organo‐photocatalysis has experienced an... Organic photocatalysts are emerging as viable and more sustainable tools than metal complexes. Recently, the field of organo-photocatalysis has experienced an... |
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| SubjectTerms | catalyst design Coordination compounds Metal complexes organocatalysis Photocatalysis Photocatalysts photoredox catalysis Redesign Redox properties Scaffolds synthetic photochemistry |
| Title | A Rational Approach to Organo‐Photocatalysis: Novel Designs and Structure‐Property Relationships |
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