Joint Charge Storage for High‐Rate Aqueous Zinc–Manganese Dioxide Batteries
Aqueous rechargeable zinc–manganese dioxide batteries show great promise for large‐scale energy storage due to their use of environmentally friendly, abundant, and rechargeable Zn metal anodes and MnO2 cathodes. In the literature various intercalation and conversion reaction mechanisms in MnO2 have...
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| Published in | Advanced materials (Weinheim) Vol. 31; no. 29; pp. e1900567 - n/a |
|---|---|
| Main Authors | , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
01.07.2019
Wiley Blackwell (John Wiley & Sons) |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Aqueous rechargeable zinc–manganese dioxide batteries show great promise for large‐scale energy storage due to their use of environmentally friendly, abundant, and rechargeable Zn metal anodes and MnO2 cathodes. In the literature various intercalation and conversion reaction mechanisms in MnO2 have been reported, but it is not clear how these mechanisms can be simultaneously manipulated to improve the charge storage and transport properties. A systematical study to understand the charge storage mechanisms in a layered δ‐MnO2 cathode is reported. An electrolyte‐dependent reaction mechanism in δ‐MnO2 is identified. Nondiffusion controlled Zn2+ intercalation in bulky δ‐MnO2 and control of H+ conversion reaction pathways over a wide C‐rate charge–discharge range facilitate high rate performance of the δ‐MnO2 cathode without sacrificing the energy density in optimal electrolytes. The Zn‐δ‐MnO2 system delivers a discharge capacity of 136.9 mAh g−1 at 20 C and capacity retention of 93% over 4000 cycles with this joint charge storage mechanism. This study opens a new gateway for the design of high‐rate electrode materials by manipulating the effective redox reactions in electrode materials for rechargeable batteries.
Rational manipulation of the charge‐storage mechanism of aqueous rechargeable Zn–MnO2 batteries is demonstrated through the use of a layered δ‐MnO2 cathode. Nondiffusion control of pseudocapacitance‐like Zn2+ intercalation in bulky δ‐MnO2, followed by control of the H+ conversion reaction pathway over a wide C‐rate charge–discharge range facilitates high rate and a long lifetime of δ‐MnO2 cathodes. |
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| AbstractList | Aqueous rechargeable zinc–manganese dioxide batteries show great promise for large‐scale energy storage due to their use of environmentally friendly, abundant, and rechargeable Zn metal anodes and MnO2 cathodes. In the literature various intercalation and conversion reaction mechanisms in MnO2 have been reported, but it is not clear how these mechanisms can be simultaneously manipulated to improve the charge storage and transport properties. A systematical study to understand the charge storage mechanisms in a layered δ‐MnO2 cathode is reported. An electrolyte‐dependent reaction mechanism in δ‐MnO2 is identified. Nondiffusion controlled Zn2+ intercalation in bulky δ‐MnO2 and control of H+ conversion reaction pathways over a wide C‐rate charge–discharge range facilitate high rate performance of the δ‐MnO2 cathode without sacrificing the energy density in optimal electrolytes. The Zn‐δ‐MnO2 system delivers a discharge capacity of 136.9 mAh g−1 at 20 C and capacity retention of 93% over 4000 cycles with this joint charge storage mechanism. This study opens a new gateway for the design of high‐rate electrode materials by manipulating the effective redox reactions in electrode materials for rechargeable batteries. Aqueous rechargeable zinc-manganese dioxide batteries show great promise for large-scale energy storage due to their use of environmentally friendly, abundant, and rechargeable Zn metal anodes and MnO2 cathodes. In the literature various intercalation and conversion reaction mechanisms in MnO2 have been reported, but it is not clear how these mechanisms can be simultaneously manipulated to improve the charge storage and transport properties. A systematical study to understand the charge storage mechanisms in a layered δ-MnO2 cathode is reported. An electrolyte-dependent reaction mechanism in δ-MnO2 is identified. Nondiffusion controlled Zn2+ intercalation in bulky δ-MnO2 and control of H+ conversion reaction pathways over a wide C-rate charge-discharge range facilitate high rate performance of the δ-MnO2 cathode without sacrificing the energy density in optimal electrolytes. The Zn-δ-MnO2 system delivers a discharge capacity of 136.9 mAh g-1 at 20 C and capacity retention of 93% over 4000 cycles with this joint charge storage mechanism. This study opens a new gateway for the design of high-rate electrode materials by manipulating the effective redox reactions in electrode materials for rechargeable batteries.Aqueous rechargeable zinc-manganese dioxide batteries show great promise for large-scale energy storage due to their use of environmentally friendly, abundant, and rechargeable Zn metal anodes and MnO2 cathodes. In the literature various intercalation and conversion reaction mechanisms in MnO2 have been reported, but it is not clear how these mechanisms can be simultaneously manipulated to improve the charge storage and transport properties. A systematical study to understand the charge storage mechanisms in a layered δ-MnO2 cathode is reported. An electrolyte-dependent reaction mechanism in δ-MnO2 is identified. Nondiffusion controlled Zn2+ intercalation in bulky δ-MnO2 and control of H+ conversion reaction pathways over a wide C-rate charge-discharge range facilitate high rate performance of the δ-MnO2 cathode without sacrificing the energy density in optimal electrolytes. The Zn-δ-MnO2 system delivers a discharge capacity of 136.9 mAh g-1 at 20 C and capacity retention of 93% over 4000 cycles with this joint charge storage mechanism. This study opens a new gateway for the design of high-rate electrode materials by manipulating the effective redox reactions in electrode materials for rechargeable batteries. Aqueous rechargeable zinc–manganese dioxide batteries show great promise for large‐scale energy storage due to their use of environmentally friendly, abundant, and rechargeable Zn metal anodes and MnO2 cathodes. In the literature various intercalation and conversion reaction mechanisms in MnO2 have been reported, but it is not clear how these mechanisms can be simultaneously manipulated to improve the charge storage and transport properties. A systematical study to understand the charge storage mechanisms in a layered δ‐MnO2 cathode is reported. An electrolyte‐dependent reaction mechanism in δ‐MnO2 is identified. Nondiffusion controlled Zn2+ intercalation in bulky δ‐MnO2 and control of H+ conversion reaction pathways over a wide C‐rate charge–discharge range facilitate high rate performance of the δ‐MnO2 cathode without sacrificing the energy density in optimal electrolytes. The Zn‐δ‐MnO2 system delivers a discharge capacity of 136.9 mAh g−1 at 20 C and capacity retention of 93% over 4000 cycles with this joint charge storage mechanism. This study opens a new gateway for the design of high‐rate electrode materials by manipulating the effective redox reactions in electrode materials for rechargeable batteries. Rational manipulation of the charge‐storage mechanism of aqueous rechargeable Zn–MnO2 batteries is demonstrated through the use of a layered δ‐MnO2 cathode. Nondiffusion control of pseudocapacitance‐like Zn2+ intercalation in bulky δ‐MnO2, followed by control of the H+ conversion reaction pathway over a wide C‐rate charge–discharge range facilitates high rate and a long lifetime of δ‐MnO2 cathodes. Aqueous rechargeable zinc-manganese dioxide batteries show great promise for large-scale energy storage due to their use of environmentally friendly, abundant, and rechargeable Zn metal anodes and MnO cathodes. In the literature various intercalation and conversion reaction mechanisms in MnO have been reported, but it is not clear how these mechanisms can be simultaneously manipulated to improve the charge storage and transport properties. A systematical study to understand the charge storage mechanisms in a layered δ-MnO cathode is reported. An electrolyte-dependent reaction mechanism in δ-MnO is identified. Nondiffusion controlled Zn intercalation in bulky δ-MnO and control of H conversion reaction pathways over a wide C-rate charge-discharge range facilitate high rate performance of the δ-MnO cathode without sacrificing the energy density in optimal electrolytes. The Zn-δ-MnO system delivers a discharge capacity of 136.9 mAh g at 20 C and capacity retention of 93% over 4000 cycles with this joint charge storage mechanism. This study opens a new gateway for the design of high-rate electrode materials by manipulating the effective redox reactions in electrode materials for rechargeable batteries. Aqueous rechargeable zinc–manganese dioxide batteries show great promise for large‐scale energy storage due to their use of environmentally friendly, abundant, and rechargeable Zn metal anodes and MnO 2 cathodes. In the literature various intercalation and conversion reaction mechanisms in MnO 2 have been reported, but it is not clear how these mechanisms can be simultaneously manipulated to improve the charge storage and transport properties. A systematical study to understand the charge storage mechanisms in a layered δ‐MnO 2 cathode is reported. An electrolyte‐dependent reaction mechanism in δ‐MnO 2 is identified. Nondiffusion controlled Zn 2+ intercalation in bulky δ‐MnO 2 and control of H + conversion reaction pathways over a wide C‐rate charge–discharge range facilitate high rate performance of the δ‐MnO 2 cathode without sacrificing the energy density in optimal electrolytes. The Zn‐δ‐MnO 2 system delivers a discharge capacity of 136.9 mAh g −1 at 20 C and capacity retention of 93% over 4000 cycles with this joint charge storage mechanism. This study opens a new gateway for the design of high‐rate electrode materials by manipulating the effective redox reactions in electrode materials for rechargeable batteries. Abstract Aqueous rechargeable zinc–manganese dioxide batteries show great promise for large‐scale energy storage due to their use of environmentally friendly, abundant, and rechargeable Zn metal anodes and MnO 2 cathodes. In the literature various intercalation and conversion reaction mechanisms in MnO 2 have been reported, but it is not clear how these mechanisms can be simultaneously manipulated to improve the charge storage and transport properties. A systematical study to understand the charge storage mechanisms in a layered δ‐MnO 2 cathode is reported. An electrolyte‐dependent reaction mechanism in δ‐MnO 2 is identified. Nondiffusion controlled Zn 2+ intercalation in bulky δ‐MnO 2 and control of H + conversion reaction pathways over a wide C‐rate charge–discharge range facilitate high rate performance of the δ‐MnO 2 cathode without sacrificing the energy density in optimal electrolytes. The Zn‐δ‐MnO 2 system delivers a discharge capacity of 136.9 mAh g −1 at 20 C and capacity retention of 93% over 4000 cycles with this joint charge storage mechanism. This study opens a new gateway for the design of high‐rate electrode materials by manipulating the effective redox reactions in electrode materials for rechargeable batteries. |
| Author | Zou, Lianfeng Zhu, Jia Han, Kee Sung Jin, Yan Shao, Yuyan Liu, Lili Patel, Rajankumar L. Pan, Huilin Engelhard, Mark H. Wang, Chongmin Liu, Jun Nie, Zimin |
| Author_xml | – sequence: 1 givenname: Yan surname: Jin fullname: Jin, Yan organization: Nanjing University – sequence: 2 givenname: Lianfeng surname: Zou fullname: Zou, Lianfeng organization: Pacific Northwest National Laboratory – sequence: 3 givenname: Lili surname: Liu fullname: Liu, Lili organization: Pacific Northwest National Laboratory – sequence: 4 givenname: Mark H. surname: Engelhard fullname: Engelhard, Mark H. organization: Pacific Northwest National Laboratory – sequence: 5 givenname: Rajankumar L. surname: Patel fullname: Patel, Rajankumar L. organization: Pacific Northwest National Laboratory – sequence: 6 givenname: Zimin surname: Nie fullname: Nie, Zimin organization: Pacific Northwest National Laboratory – sequence: 7 givenname: Kee Sung surname: Han fullname: Han, Kee Sung organization: Pacific Northwest National Laboratory – sequence: 8 givenname: Yuyan surname: Shao fullname: Shao, Yuyan organization: Pacific Northwest National Laboratory – sequence: 9 givenname: Chongmin surname: Wang fullname: Wang, Chongmin organization: Pacific Northwest National Laboratory – sequence: 10 givenname: Jia surname: Zhu fullname: Zhu, Jia organization: Nanjing University – sequence: 11 givenname: Huilin surname: Pan fullname: Pan, Huilin email: huilin.pan@pnnl.gov organization: Pacific Northwest National Laboratory – sequence: 12 givenname: Jun orcidid: 0000-0001-7991-1015 surname: Liu fullname: Liu, Jun email: jun.liu@pnnl.gov organization: Pacific Northwest National Laboratory |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/31157468$$D View this record in MEDLINE/PubMed https://www.osti.gov/biblio/1545406$$D View this record in Osti.gov |
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| Snippet | Aqueous rechargeable zinc–manganese dioxide batteries show great promise for large‐scale energy storage due to their use of environmentally friendly, abundant,... Aqueous rechargeable zinc-manganese dioxide batteries show great promise for large-scale energy storage due to their use of environmentally friendly, abundant,... Abstract Aqueous rechargeable zinc–manganese dioxide batteries show great promise for large‐scale energy storage due to their use of environmentally friendly,... |
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| SubjectTerms | Aqueous Zn‐MnO2 batteries Batteries battery reaction mechanisms Cathodes Charge transport Conversion Discharge Electrode materials Electrodes Electrolytes Energy storage Flux density high‐rate batteries Intercalation joint charge storage Lithium Manganese dioxide Materials science Reaction mechanisms Rechargeable batteries Redox reactions Storage batteries Transport properties Zinc |
| Title | Joint Charge Storage for High‐Rate Aqueous Zinc–Manganese Dioxide Batteries |
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