Strength can be controlled by edge dislocations in refractory high-entropy alloys

Energy efficiency is motivating the search for new high-temperature (high-T) metals. Some new body-centered-cubic (BCC) random multicomponent “high-entropy alloys (HEAs)” based on refractory elements (Cr-Mo-Nb-Ta-V-W-Hf-Ti-Zr) possess exceptional strengths at high temperatures but the physical origi...

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Published inNature communications Vol. 12; no. 1; p. 5474
Main Authors Lee, Chanho, Maresca, Francesco, Feng, Rui, Chou, Yi, Ungar, T., Widom, Michael, An, Ke, Poplawsky, Jonathan D., Chou, Yi-Chia, Liaw, Peter K., Curtin, W. A.
Format Journal Article
LanguageEnglish
Published London Nature Publishing Group UK 16.09.2021
Nature Publishing Group
Nature Portfolio
Subjects
147/135
147/143
639/166/988
639/301/1023/303
639/301/1034/1037
Alloys
BCC metals
Body temperature
Chromium
Computational methods
Dislocation mobility
Edge dislocations
Electron microscopes
Energy efficiency
Entropy
High entropy alloys
High resolution electron microscopy
High strength alloys
High temperature
Humanities and Social Sciences
MATERIALS SCIENCE
Mechanical engineering
Mechanical properties
Metals
Molybdenum
multidisciplinary
Niobium
Plastic flow
Science
Science (multidisciplinary)
Screw dislocations
Titanium
Transmission electron microscopy
Tungsten
Zirconium
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Abstract Energy efficiency is motivating the search for new high-temperature (high-T) metals. Some new body-centered-cubic (BCC) random multicomponent “high-entropy alloys (HEAs)” based on refractory elements (Cr-Mo-Nb-Ta-V-W-Hf-Ti-Zr) possess exceptional strengths at high temperatures but the physical origins of this outstanding behavior are not known. Here we show, using integrated in-situ neutron-diffraction (ND), high-resolution transmission electron microscopy (HRTEM), and recent theory, that the high strength and strength retention of a NbTaTiV alloy and a high-strength/low-density CrMoNbV alloy are attributable to edge dislocations. This finding is surprising because plastic flows in BCC elemental metals and dilute alloys are generally controlled by screw dislocations. We use the insight and theory to perform a computationally-guided search over 10 7 BCC HEAs and identify over 10 6 possible ultra-strong high-T alloy compositions for future exploration. The strength in BCC high-entropy alloys is associated with the type of mobile dislocations. Here the authors demonstrate by means of an ample array of experimental techniques that edge dislocations can control the strength of BCC high-entropy alloys.
AbstractList Energy efficiency is motivating the search for new high-temperature (high-T) metals. Some new body-centered-cubic (BCC) random multicomponent “high-entropy alloys (HEAs)” based on refractory elements (Cr-Mo-Nb-Ta-V-W-Hf-Ti-Zr) possess exceptional strengths at high temperatures but the physical origins of this outstanding behavior are not known. Here we show, using integrated in-situ neutron-diffraction (ND), high-resolution transmission electron microscopy (HRTEM), and recent theory, that the high strength and strength retention of a NbTaTiV alloy and a high-strength/low-density CrMoNbV alloy are attributable to edge dislocations. This finding is surprising because plastic flows in BCC elemental metals and dilute alloys are generally controlled by screw dislocations. We use the insight and theory to perform a computationally-guided search over 10 7 BCC HEAs and identify over 10 6 possible ultra-strong high-T alloy compositions for future exploration. The strength in BCC high-entropy alloys is associated with the type of mobile dislocations. Here the authors demonstrate by means of an ample array of experimental techniques that edge dislocations can control the strength of BCC high-entropy alloys.
Energy efficiency is motivating the search for new high-temperature (high-T) metals. Some new body-centered-cubic (BCC) random multicomponent “high-entropy alloys (HEAs)” based on refractory elements (Cr-Mo-Nb-Ta-V-W-Hf-Ti-Zr) possess exceptional strengths at high temperatures but the physical origins of this outstanding behavior are not known. Here we show, using integrated in-situ neutron-diffraction (ND), high-resolution transmission electron microscopy (HRTEM), and recent theory, that the high strength and strength retention of a NbTaTiV alloy and a high-strength/low-density CrMoNbV alloy are attributable to edge dislocations. This finding is surprising because plastic flows in BCC elemental metals and dilute alloys are generally controlled by screw dislocations. We use the insight and theory to perform a computationally-guided search over 107 BCC HEAs and identify over 106 possible ultra-strong high-T alloy compositions for future exploration.
Abstract Energy efficiency is motivating the search for new high-temperature (high-T) metals. Some new body-centered-cubic (BCC) random multicomponent “high-entropy alloys (HEAs)” based on refractory elements (Cr-Mo-Nb-Ta-V-W-Hf-Ti-Zr) possess exceptional strengths at high temperatures but the physical origins of this outstanding behavior are not known. Here we show, using integrated in-situ neutron-diffraction (ND), high-resolution transmission electron microscopy (HRTEM), and recent theory, that the high strength and strength retention of a NbTaTiV alloy and a high-strength/low-density CrMoNbV alloy are attributable to edge dislocations. This finding is surprising because plastic flows in BCC elemental metals and dilute alloys are generally controlled by screw dislocations. We use the insight and theory to perform a computationally-guided search over 10 7 BCC HEAs and identify over 10 6 possible ultra-strong high-T alloy compositions for future exploration.
The strength in BCC high-entropy alloys is associated with the type of mobile dislocations. Here the authors demonstrate by means of an ample array of experimental techniques that edge dislocations can control the strength of BCC high-entropy alloys.
Energy efficiency is motivating the search for new high-temperature (high-T) metals. Some new body-centered-cubic (BCC) random multicomponent “high-entropy alloys (HEAs)” based on refractory elements (Cr-Mo-Nb-Ta-V-W-Hf-Ti-Zr) possess exceptional strengths at high temperatures but the physical origins of this outstanding behavior are not known. Here we show, using integrated in-situ neutron-diffraction (ND), high-resolution transmission electron microscopy (HRTEM), and recent theory, that the high strength and strength retention of a NbTaTiV alloy and a high-strength/low-density CrMoNbV alloy are attributable to edge dislocations. This finding is surprising because plastic flows in BCC elemental metals and dilute alloys are generally controlled by screw dislocations. We use the insight and theory to perform a computationally-guided search over 107 BCC HEAs and identify over 106 possible ultra-strong high-T alloy compositions for future exploration.The strength in BCC high-entropy alloys is associated with the type of mobile dislocations. Here the authors demonstrate by means of an ample array of experimental techniques that edge dislocations can control the strength of BCC high-entropy alloys.
ArticleNumber 5474
Author Ungar, T.
Curtin, W. A.
Chou, Yi-Chia
Feng, Rui
Liaw, Peter K.
An, Ke
Maresca, Francesco
Poplawsky, Jonathan D.
Chou, Yi
Widom, Michael
Lee, Chanho
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PublicationDate 2021-09-16
PublicationDateYYYYMMDD 2021-09-16
PublicationDate_xml – month: 09
  year: 2021
  text: 2021-09-16
  day: 16
PublicationDecade 2020
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PublicationTitle Nature communications
PublicationTitleAbbrev Nat Commun
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Publisher Nature Publishing Group UK
Nature Publishing Group
Nature Portfolio
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    fullname: Y Ikeda
SSID ssj0000391844
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Snippet Energy efficiency is motivating the search for new high-temperature (high-T) metals. Some new body-centered-cubic (BCC) random multicomponent “high-entropy...
Abstract Energy efficiency is motivating the search for new high-temperature (high-T) metals. Some new body-centered-cubic (BCC) random multicomponent...
The strength in BCC high-entropy alloys is associated with the type of mobile dislocations. Here the authors demonstrate by means of an ample array of...
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SubjectTerms 147/135
147/143
639/166/988
639/301/1023/303
639/301/1034/1037
Alloys
BCC metals
Body temperature
Chromium
Computational methods
Dislocation mobility
Edge dislocations
Electron microscopes
Energy efficiency
Entropy
High entropy alloys
High resolution electron microscopy
High strength alloys
High temperature
Humanities and Social Sciences
MATERIALS SCIENCE
Mechanical engineering
Mechanical properties
Metals
Molybdenum
multidisciplinary
Niobium
Plastic flow
Science
Science (multidisciplinary)
Screw dislocations
Titanium
Transmission electron microscopy
Tungsten
Zirconium
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Title Strength can be controlled by edge dislocations in refractory high-entropy alloys
URI https://link.springer.com/article/10.1038/s41467-021-25807-w
https://www.proquest.com/docview/2573124354
https://search.proquest.com/docview/2574406707
https://www.osti.gov/servlets/purl/1822756
https://pubmed.ncbi.nlm.nih.gov/PMC8446014
https://doaj.org/article/cff8e583f09e465f99650f8fee5275c9
Volume 12
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