Fusion of the extended modified liquid drop model for nucleation and dynamical nucleation theory

We present a new phenomenological approach to nucleation, based on the combination of the "extended modified liquid drop" model and dynamical nucleation theory. The new model proposes a new cluster definition, which properly includes the effect of fluctuations, and it is consistent both th...

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Published inPhysical review letters Vol. 93; no. 16; p. 165701
Main Authors Reguera, D, Reiss, H
Format Journal Article
LanguageEnglish
Published United States 15.10.2004
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Abstract We present a new phenomenological approach to nucleation, based on the combination of the "extended modified liquid drop" model and dynamical nucleation theory. The new model proposes a new cluster definition, which properly includes the effect of fluctuations, and it is consistent both thermodynamically and kinetically. The model is able to predict successfully the free energy of formation of the critical nucleus, using only macroscopic thermodynamic properties. It also accounts for the spinodal and provides excellent agreement with the result of recent simulations.
AbstractList We present a new phenomenological approach to nucleation, based on the combination of the "extended modified liquid drop" model and dynamical nucleation theory. The new model proposes a new cluster definition, which properly includes the effect of fluctuations, and it is consistent both thermodynamically and kinetically. The model is able to predict successfully the free energy of formation of the critical nucleus, using only macroscopic thermodynamic properties. It also accounts for the spinodal and provides excellent agreement with the result of recent simulations.
Author Reguera, D
Reiss, H
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BackLink https://www.ncbi.nlm.nih.gov/pubmed/15525003$$D View this record in MEDLINE/PubMed
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