A Pyrazine‐Based Polymer for Fast‐Charge Batteries

The lack of high‐power and stable cathodes prohibits the development of rechargeable metal (Na, Mg, Al) batteries. Herein, poly(hexaazatrinaphthalene) (PHATN), an environmentally benign, abundant and sustainable polymer, is employed as a universal cathode material for these batteries. In Na‐ion batt...

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Published inAngewandte Chemie (International ed.) Vol. 58; no. 49; pp. 17820 - 17826
Main Authors Mao, Minglei, Luo, Chao, Pollard, Travis P., Hou, Singyuk, Gao, Tao, Fan, Xiulin, Cui, Chunyu, Yue, Jinming, Tong, Yuxin, Yang, Gaojing, Deng, Tao, Zhang, Ming, Ma, Jianmin, Suo, Liumin, Borodin, Oleg, Wang, Chunsheng
Format Journal Article
LanguageEnglish
Published Germany Wiley Subscription Services, Inc 02.12.2019
Wiley
EditionInternational ed. in English
Subjects
Aluminum
bio-inspired
Cathodes
charge transport
defects
Electrode materials
ENERGY STORAGE
energy storage (including batteries and capacitors)
fast charging
Flux density
Magnesium
Metal ions
Photoelectron spectroscopy
Photoelectrons
polymer cathodes
Polymers
Pyrazine
rechargeable AI batteries
rechargeable Al batteries
Rechargeable batteries
rechargeable Mg batteries
Sodium
sodium ion batteries
synthesis (novel materials)
synthesis (scalable processing)
synthesis (self-assembly)
rechargeable Al batteries
fast charging
polymer cathodes
rechargeable Mg batteries
sodium ion batteries
Online AccessGet full text
ISSN1433-7851
1521-3773
1521-3773
DOI10.1002/anie.201910916

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Abstract The lack of high‐power and stable cathodes prohibits the development of rechargeable metal (Na, Mg, Al) batteries. Herein, poly(hexaazatrinaphthalene) (PHATN), an environmentally benign, abundant and sustainable polymer, is employed as a universal cathode material for these batteries. In Na‐ion batteries (NIBs), PHATN delivers a reversible capacity of 220 mAh g−1 at 50 mA g−1, corresponding to the energy density of 440 Wh kg−1, and still retains 100 mAh g−1 at 10 Ag−1 after 50 000 cycles, which is among the best performances in NIBs. Such an exceptional performance is also observed in more challenging Mg and Al batteries. PHATN retains reversible capacities of 110 mAh g−1 after 200 cycles in Mg batteries and 92 mAh g−1 after 100 cycles in Al batteries. DFT calculations, X‐ray photoelectron spectroscopy, Raman, and FTIR show that the electron‐deficient pyrazine sites in PHATN are the redox centers to reversibly react with metal ions. Poly(hexaazatrinaphthalene) (PHATN), an environmentally benign, abundant and sustainable polymer, is employed as a universal cathode material for metal batteries. Exceptional performance is observed in Na and in more challenging Mg and Al batteries. The electron‐deficient pyrazine sites in PHATN are the redox centers to reversibly react with metal ions.
AbstractList The lack of high‐power and stable cathodes prohibits the development of rechargeable metal (Na, Mg, Al) batteries. Herein, poly(hexaazatrinaphthalene) (PHATN), an environmentally benign, abundant and sustainable polymer, is employed as a universal cathode material for these batteries. In Na‐ion batteries (NIBs), PHATN delivers a reversible capacity of 220 mAh g −1 at 50 mA g −1 , corresponding to the energy density of 440 Wh kg −1 , and still retains 100 mAh g −1 at 10 Ag −1 after 50 000 cycles, which is among the best performances in NIBs. Such an exceptional performance is also observed in more challenging Mg and Al batteries. PHATN retains reversible capacities of 110 mAh g −1 after 200 cycles in Mg batteries and 92 mAh g −1 after 100 cycles in Al batteries. DFT calculations, X‐ray photoelectron spectroscopy, Raman, and FTIR show that the electron‐deficient pyrazine sites in PHATN are the redox centers to reversibly react with metal ions.
The lack of high-power and stable cathodes prohibits the development of rechargeable metal (Na, Mg, Al) batteries. Here, poly(hexaazatrinaphthalene) (PHATN), an environmentally benign, abundant and sustainable polymer, is employed as a universal cathode material for these batteries. In Na-ion batteries (NIBs), PHATN delivers a reversible capacity of 220 mAh g-1 at 50 mA g-1, corresponding to the energy density of 440 Wh kg-1, and still retains 100 mAh g-1 at 10 Ag-1 after 50 000 cycles, which is among the best performances in NIBs. Such an exceptional performance is also observed in more challenging Mg and Al batteries. PHATN retains reversible capacities of 110 mAh g-1 after 200 cycles in Mg batteries and 92 mAh g-1 after 100 cycles in Al batteries. DFT calculations, X-ray photoelectron spectroscopy, Raman, and FTIR show that the electron-deficient pyrazine sites in PHATN are the redox centers to reversibly react with metal ions.
The lack of high-power and stable cathodes prohibits the development of rechargeable metal (Na, Mg, Al) batteries. Herein, poly(hexaazatrinaphthalene) (PHATN), an environmentally benign, abundant and sustainable polymer, is employed as a universal cathode material for these batteries. In Na-ion batteries (NIBs), PHATN delivers a reversible capacity of 220 mAh g at 50 mA g , corresponding to the energy density of 440 Wh kg , and still retains 100 mAh g at 10 Ag after 50 000 cycles, which is among the best performances in NIBs. Such an exceptional performance is also observed in more challenging Mg and Al batteries. PHATN retains reversible capacities of 110 mAh g after 200 cycles in Mg batteries and 92 mAh g after 100 cycles in Al batteries. DFT calculations, X-ray photoelectron spectroscopy, Raman, and FTIR show that the electron-deficient pyrazine sites in PHATN are the redox centers to reversibly react with metal ions.
The lack of high-power and stable cathodes prohibits the development of rechargeable metal (Na, Mg, Al) batteries. Herein, poly(hexaazatrinaphthalene) (PHATN), an environmentally benign, abundant and sustainable polymer, is employed as a universal cathode material for these batteries. In Na-ion batteries (NIBs), PHATN delivers a reversible capacity of 220 mAh g-1 at 50 mA g-1 , corresponding to the energy density of 440 Wh kg-1 , and still retains 100 mAh g-1 at 10 Ag-1 after 50 000 cycles, which is among the best performances in NIBs. Such an exceptional performance is also observed in more challenging Mg and Al batteries. PHATN retains reversible capacities of 110 mAh g-1 after 200 cycles in Mg batteries and 92 mAh g-1 after 100 cycles in Al batteries. DFT calculations, X-ray photoelectron spectroscopy, Raman, and FTIR show that the electron-deficient pyrazine sites in PHATN are the redox centers to reversibly react with metal ions.The lack of high-power and stable cathodes prohibits the development of rechargeable metal (Na, Mg, Al) batteries. Herein, poly(hexaazatrinaphthalene) (PHATN), an environmentally benign, abundant and sustainable polymer, is employed as a universal cathode material for these batteries. In Na-ion batteries (NIBs), PHATN delivers a reversible capacity of 220 mAh g-1 at 50 mA g-1 , corresponding to the energy density of 440 Wh kg-1 , and still retains 100 mAh g-1 at 10 Ag-1 after 50 000 cycles, which is among the best performances in NIBs. Such an exceptional performance is also observed in more challenging Mg and Al batteries. PHATN retains reversible capacities of 110 mAh g-1 after 200 cycles in Mg batteries and 92 mAh g-1 after 100 cycles in Al batteries. DFT calculations, X-ray photoelectron spectroscopy, Raman, and FTIR show that the electron-deficient pyrazine sites in PHATN are the redox centers to reversibly react with metal ions.
The lack of high‐power and stable cathodes prohibits the development of rechargeable metal (Na, Mg, Al) batteries. Herein, poly(hexaazatrinaphthalene) (PHATN), an environmentally benign, abundant and sustainable polymer, is employed as a universal cathode material for these batteries. In Na‐ion batteries (NIBs), PHATN delivers a reversible capacity of 220 mAh g−1 at 50 mA g−1, corresponding to the energy density of 440 Wh kg−1, and still retains 100 mAh g−1 at 10 Ag−1 after 50 000 cycles, which is among the best performances in NIBs. Such an exceptional performance is also observed in more challenging Mg and Al batteries. PHATN retains reversible capacities of 110 mAh g−1 after 200 cycles in Mg batteries and 92 mAh g−1 after 100 cycles in Al batteries. DFT calculations, X‐ray photoelectron spectroscopy, Raman, and FTIR show that the electron‐deficient pyrazine sites in PHATN are the redox centers to reversibly react with metal ions. Poly(hexaazatrinaphthalene) (PHATN), an environmentally benign, abundant and sustainable polymer, is employed as a universal cathode material for metal batteries. Exceptional performance is observed in Na and in more challenging Mg and Al batteries. The electron‐deficient pyrazine sites in PHATN are the redox centers to reversibly react with metal ions.
The lack of high‐power and stable cathodes prohibits the development of rechargeable metal (Na, Mg, Al) batteries. Herein, poly(hexaazatrinaphthalene) (PHATN), an environmentally benign, abundant and sustainable polymer, is employed as a universal cathode material for these batteries. In Na‐ion batteries (NIBs), PHATN delivers a reversible capacity of 220 mAh g−1 at 50 mA g−1, corresponding to the energy density of 440 Wh kg−1, and still retains 100 mAh g−1 at 10 Ag−1 after 50 000 cycles, which is among the best performances in NIBs. Such an exceptional performance is also observed in more challenging Mg and Al batteries. PHATN retains reversible capacities of 110 mAh g−1 after 200 cycles in Mg batteries and 92 mAh g−1 after 100 cycles in Al batteries. DFT calculations, X‐ray photoelectron spectroscopy, Raman, and FTIR show that the electron‐deficient pyrazine sites in PHATN are the redox centers to reversibly react with metal ions.
Author Wang, Chunsheng
Yue, Jinming
Deng, Tao
Luo, Chao
Gao, Tao
Borodin, Oleg
Mao, Minglei
Pollard, Travis P.
Hou, Singyuk
Tong, Yuxin
Ma, Jianmin
Suo, Liumin
Cui, Chunyu
Fan, Xiulin
Yang, Gaojing
Zhang, Ming
Author_xml – sequence: 1
  givenname: Minglei
  surname: Mao
  fullname: Mao, Minglei
  organization: Chinese Academy of Sciences
– sequence: 2
  givenname: Chao
  surname: Luo
  fullname: Luo, Chao
  email: cluo@gmu.edu
  organization: George Mason University
– sequence: 3
  givenname: Travis P.
  surname: Pollard
  fullname: Pollard, Travis P.
  organization: US Army Research Laboratory
– sequence: 4
  givenname: Singyuk
  surname: Hou
  fullname: Hou, Singyuk
  organization: University of Maryland
– sequence: 5
  givenname: Tao
  surname: Gao
  fullname: Gao, Tao
  organization: University of Maryland
– sequence: 6
  givenname: Xiulin
  surname: Fan
  fullname: Fan, Xiulin
  organization: University of Maryland
– sequence: 7
  givenname: Chunyu
  surname: Cui
  fullname: Cui, Chunyu
  organization: Hunan University
– sequence: 8
  givenname: Jinming
  surname: Yue
  fullname: Yue, Jinming
  organization: Chinese Academy of Sciences
– sequence: 9
  givenname: Yuxin
  surname: Tong
  fullname: Tong, Yuxin
  organization: Chinese Academy of Sciences
– sequence: 10
  givenname: Gaojing
  surname: Yang
  fullname: Yang, Gaojing
  organization: Chinese Academy of Sciences
– sequence: 11
  givenname: Tao
  surname: Deng
  fullname: Deng, Tao
  organization: University of Maryland
– sequence: 12
  givenname: Ming
  surname: Zhang
  fullname: Zhang, Ming
  organization: Hunan University
– sequence: 13
  givenname: Jianmin
  surname: Ma
  fullname: Ma, Jianmin
  organization: Hunan University
– sequence: 14
  givenname: Liumin
  surname: Suo
  fullname: Suo, Liumin
  organization: Chinese Academy of Sciences
– sequence: 15
  givenname: Oleg
  surname: Borodin
  fullname: Borodin, Oleg
  email: oleg.a.borodin.civ@mail.mil
  organization: US Army Research Laboratory
– sequence: 16
  givenname: Chunsheng
  orcidid: 0000-0002-8626-6381
  surname: Wang
  fullname: Wang, Chunsheng
  email: cswang@umd.edu
  organization: University of Maryland
BackLink https://www.ncbi.nlm.nih.gov/pubmed/31571354$$D View this record in MEDLINE/PubMed
https://www.osti.gov/servlets/purl/1767522$$D View this record in Osti.gov
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Snippet The lack of high‐power and stable cathodes prohibits the development of rechargeable metal (Na, Mg, Al) batteries. Herein, poly(hexaazatrinaphthalene) (PHATN),...
The lack of high-power and stable cathodes prohibits the development of rechargeable metal (Na, Mg, Al) batteries. Herein, poly(hexaazatrinaphthalene) (PHATN),...
The lack of high-power and stable cathodes prohibits the development of rechargeable metal (Na, Mg, Al) batteries. Here, poly(hexaazatrinaphthalene) (PHATN),...
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SubjectTerms Aluminum
bio-inspired
Cathodes
charge transport
defects
Electrode materials
ENERGY STORAGE
energy storage (including batteries and capacitors)
fast charging
Flux density
Magnesium
Metal ions
Photoelectron spectroscopy
Photoelectrons
polymer cathodes
Polymers
Pyrazine
rechargeable AI batteries
rechargeable Al batteries
Rechargeable batteries
rechargeable Mg batteries
Sodium
sodium ion batteries
synthesis (novel materials)
synthesis (scalable processing)
synthesis (self-assembly)
Title A Pyrazine‐Based Polymer for Fast‐Charge Batteries
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fanie.201910916
https://www.ncbi.nlm.nih.gov/pubmed/31571354
https://www.proquest.com/docview/2317519941
https://www.proquest.com/docview/2299773157
https://www.osti.gov/servlets/purl/1767522
Volume 58
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