A Universal Organic Cathode for Ultrafast Lithium and Multivalent Metal Batteries
Low‐cost multivalent battery chemistries (Mg2+, Al3+) have been extensively investigated for large‐scale energy storage applications. However, their commercialization is plagued by the poor power density and cycle life of cathodes. A universal polyimides@CNT (PI@CNT) cathode is now presented that ca...
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| Published in | Angewandte Chemie (International ed.) Vol. 57; no. 24; pp. 7146 - 7150 |
|---|---|
| Main Authors | , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
11.06.2018
Wiley Blackwell (John Wiley & Sons) |
| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Low‐cost multivalent battery chemistries (Mg2+, Al3+) have been extensively investigated for large‐scale energy storage applications. However, their commercialization is plagued by the poor power density and cycle life of cathodes. A universal polyimides@CNT (PI@CNT) cathode is now presented that can reversibly store various cations with different valences (Li+, Mg2+, Al3+) at an extremely fast rate. The ion‐coordination charge storage mechanism of PI@CNT is systemically investigated. Full cells using PI@CNT cathodes and corresponding metal anodes exhibit long cycle life (>10000 cycles), fast kinetics (>20 C), and wide operating temperature range (−40 to 50 °C), making the low‐cost industrial polyimides universal cathodes for different multivalent metal batteries. The stable ion‐coordinated mechanism opens a new foundation for the development of high‐energy and high‐power multivalent batteries.
A universal ultrafast organic cathode for multivalent batteries is reported. In contrast to slow solid‐state ion diffusion and phase transformation in inorganic materials with a stiff crystal structure, the soft structure of the PI@CNT composite with the ion‐coordination charge storage mechanism ensures ultrafast reaction kinetics, improving the traditional low power and poor cycle life of multivalent battery chemistries. |
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| AbstractList | Low‐cost multivalent battery chemistries (Mg2+, Al3+) have been extensively investigated for large‐scale energy storage applications. However, their commercialization is plagued by the poor power density and cycle life of cathodes. A universal polyimides@CNT (PI@CNT) cathode is now presented that can reversibly store various cations with different valences (Li+, Mg2+, Al3+) at an extremely fast rate. The ion‐coordination charge storage mechanism of PI@CNT is systemically investigated. Full cells using PI@CNT cathodes and corresponding metal anodes exhibit long cycle life (>10000 cycles), fast kinetics (>20 C), and wide operating temperature range (−40 to 50 °C), making the low‐cost industrial polyimides universal cathodes for different multivalent metal batteries. The stable ion‐coordinated mechanism opens a new foundation for the development of high‐energy and high‐power multivalent batteries. Low‐cost multivalent battery chemistries (Mg2+, Al3+) have been extensively investigated for large‐scale energy storage applications. However, their commercialization is plagued by the poor power density and cycle life of cathodes. A universal polyimides@CNT (PI@CNT) cathode is now presented that can reversibly store various cations with different valences (Li+, Mg2+, Al3+) at an extremely fast rate. The ion‐coordination charge storage mechanism of PI@CNT is systemically investigated. Full cells using PI@CNT cathodes and corresponding metal anodes exhibit long cycle life (>10000 cycles), fast kinetics (>20 C), and wide operating temperature range (−40 to 50 °C), making the low‐cost industrial polyimides universal cathodes for different multivalent metal batteries. The stable ion‐coordinated mechanism opens a new foundation for the development of high‐energy and high‐power multivalent batteries. A universal ultrafast organic cathode for multivalent batteries is reported. In contrast to slow solid‐state ion diffusion and phase transformation in inorganic materials with a stiff crystal structure, the soft structure of the PI@CNT composite with the ion‐coordination charge storage mechanism ensures ultrafast reaction kinetics, improving the traditional low power and poor cycle life of multivalent battery chemistries. Low-cost multivalent battery chemistries (Mg2+ , Al3+ ) have been extensively investigated for large-scale energy storage applications. However, their commercialization is plagued by the poor power density and cycle life of cathodes. A universal polyimides@CNT (PI@CNT) cathode is now presented that can reversibly store various cations with different valences (Li+ , Mg2+ , Al3+ ) at an extremely fast rate. The ion-coordination charge storage mechanism of PI@CNT is systemically investigated. Full cells using PI@CNT cathodes and corresponding metal anodes exhibit long cycle life (>10000 cycles), fast kinetics (>20 C), and wide operating temperature range (-40 to 50 °C), making the low-cost industrial polyimides universal cathodes for different multivalent metal batteries. The stable ion-coordinated mechanism opens a new foundation for the development of high-energy and high-power multivalent batteries.Low-cost multivalent battery chemistries (Mg2+ , Al3+ ) have been extensively investigated for large-scale energy storage applications. However, their commercialization is plagued by the poor power density and cycle life of cathodes. A universal polyimides@CNT (PI@CNT) cathode is now presented that can reversibly store various cations with different valences (Li+ , Mg2+ , Al3+ ) at an extremely fast rate. The ion-coordination charge storage mechanism of PI@CNT is systemically investigated. Full cells using PI@CNT cathodes and corresponding metal anodes exhibit long cycle life (>10000 cycles), fast kinetics (>20 C), and wide operating temperature range (-40 to 50 °C), making the low-cost industrial polyimides universal cathodes for different multivalent metal batteries. The stable ion-coordinated mechanism opens a new foundation for the development of high-energy and high-power multivalent batteries. Abstract Low‐cost multivalent battery chemistries (Mg 2+ , Al 3+ ) have been extensively investigated for large‐scale energy storage applications. However, their commercialization is plagued by the poor power density and cycle life of cathodes. A universal polyimides@CNT (PI@CNT) cathode is now presented that can reversibly store various cations with different valences (Li + , Mg 2+ , Al 3+ ) at an extremely fast rate. The ion‐coordination charge storage mechanism of PI@CNT is systemically investigated. Full cells using PI@CNT cathodes and corresponding metal anodes exhibit long cycle life (>10000 cycles), fast kinetics (>20 C), and wide operating temperature range (−40 to 50 °C), making the low‐cost industrial polyimides universal cathodes for different multivalent metal batteries. The stable ion‐coordinated mechanism opens a new foundation for the development of high‐energy and high‐power multivalent batteries. Low-cost multivalent battery chemistries (Mg , Al ) have been extensively investigated for large-scale energy storage applications. However, their commercialization is plagued by the poor power density and cycle life of cathodes. A universal polyimides@CNT (PI@CNT) cathode is now presented that can reversibly store various cations with different valences (Li , Mg , Al ) at an extremely fast rate. The ion-coordination charge storage mechanism of PI@CNT is systemically investigated. Full cells using PI@CNT cathodes and corresponding metal anodes exhibit long cycle life (>10000 cycles), fast kinetics (>20 C), and wide operating temperature range (-40 to 50 °C), making the low-cost industrial polyimides universal cathodes for different multivalent metal batteries. The stable ion-coordinated mechanism opens a new foundation for the development of high-energy and high-power multivalent batteries. Low‐cost multivalent battery chemistries (Mg 2+ , Al 3+ ) have been extensively investigated for large‐scale energy storage applications. However, their commercialization is plagued by the poor power density and cycle life of cathodes. A universal polyimides@CNT (PI@CNT) cathode is now presented that can reversibly store various cations with different valences (Li + , Mg 2+ , Al 3+ ) at an extremely fast rate. The ion‐coordination charge storage mechanism of PI@CNT is systemically investigated. Full cells using PI@CNT cathodes and corresponding metal anodes exhibit long cycle life (>10000 cycles), fast kinetics (>20 C), and wide operating temperature range (−40 to 50 °C), making the low‐cost industrial polyimides universal cathodes for different multivalent metal batteries. The stable ion‐coordinated mechanism opens a new foundation for the development of high‐energy and high‐power multivalent batteries. |
| Author | Wang, Chunsheng Li, Xiaogang Deng, Tao Luo, Chao Gao, Tao Wang, Ruixing Wang, Fei Chen, Ji Hou, Singyuk Ji, Xiao Chen, Long Wang, Luning Fan, Xiulin |
| Author_xml | – sequence: 1 givenname: Xiulin surname: Fan fullname: Fan, Xiulin organization: University of Maryland – sequence: 2 givenname: Fei surname: Wang fullname: Wang, Fei organization: Sensor and Electron Devices Directorate Power and Energy Division U.S. Army Research Laboratory – sequence: 3 givenname: Xiao surname: Ji fullname: Ji, Xiao organization: University of Maryland – sequence: 4 givenname: Ruixing surname: Wang fullname: Wang, Ruixing organization: University of Maryland – sequence: 5 givenname: Tao surname: Gao fullname: Gao, Tao organization: University of Maryland – sequence: 6 givenname: Singyuk surname: Hou fullname: Hou, Singyuk organization: University of Maryland – sequence: 7 givenname: Ji surname: Chen fullname: Chen, Ji organization: University of Maryland – sequence: 8 givenname: Tao surname: Deng fullname: Deng, Tao organization: University of Maryland – sequence: 9 givenname: Xiaogang surname: Li fullname: Li, Xiaogang organization: University of Maryland – sequence: 10 givenname: Long surname: Chen fullname: Chen, Long organization: University of Maryland – sequence: 11 givenname: Chao surname: Luo fullname: Luo, Chao organization: University of Maryland – sequence: 12 givenname: Luning surname: Wang fullname: Wang, Luning organization: University of Maryland – sequence: 13 givenname: Chunsheng orcidid: 0000-0002-8626-6381 surname: Wang fullname: Wang, Chunsheng email: cswang@umd.edu organization: University of Maryland |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/29704298$$D View this record in MEDLINE/PubMed https://www.osti.gov/biblio/1437068$$D View this record in Osti.gov |
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| Keywords | lithium ion batteries magnesium aluminum multivalent batteries organic cathodes |
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| Snippet | Low‐cost multivalent battery chemistries (Mg2+, Al3+) have been extensively investigated for large‐scale energy storage applications. However, their... Low‐cost multivalent battery chemistries (Mg 2+ , Al 3+ ) have been extensively investigated for large‐scale energy storage applications. However, their... Low-cost multivalent battery chemistries (Mg , Al ) have been extensively investigated for large-scale energy storage applications. However, their... Low-cost multivalent battery chemistries (Mg2+ , Al3+ ) have been extensively investigated for large-scale energy storage applications. However, their... Abstract Low‐cost multivalent battery chemistries (Mg 2+ , Al 3+ ) have been extensively investigated for large‐scale energy storage applications. However,... |
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| SubjectTerms | Aluminum Batteries Cathodes Cations Commercialization Energy storage Ion charge Lithium lithium ion batteries Magnesium multivalent batteries Operating temperature organic cathodes Organic chemistry Polyimide resins |
| Title | A Universal Organic Cathode for Ultrafast Lithium and Multivalent Metal Batteries |
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