Thermodynamic analysis of carbon dioxide reforming of methane in view of solid carbon formation
A thermodynamic equilibrium analysis on the multi-reaction system for carbon dioxide reforming of methane in view of carbon formation was performed with Aspen plus based on direct minimization of Gibbs free energy method. The effects of CO2/CH4 ratio (0.5–3), reaction temperature (573–1473K) and pre...
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| Published in | Fuel processing technology Vol. 92; no. 3; pp. 678 - 691 |
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| Main Authors | , |
| Format | Journal Article |
| Language | English |
| Published |
Amsterdam
Elsevier B.V
01.03.2011
Elsevier |
| Subjects | |
| Online Access | Get full text |
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| Abstract | A thermodynamic equilibrium analysis on the multi-reaction system for carbon dioxide reforming of methane in view of carbon formation was performed with Aspen plus based on direct minimization of Gibbs free energy method. The effects of CO2/CH4 ratio (0.5–3), reaction temperature (573–1473K) and pressure (1–25atm) on equilibrium conversions, product compositions and solid carbon were studied. Numerical analysis revealed that the optimal working conditions for syngas production in Fischer–Tropsch synthesis were at temperatures higher than 1173K for CO2/CH4 ratio being 1 at which about 4mol of syngas (H2/CO=1) could be produced from 2mol of reactants with negligible amount of carbon formation. Although temperatures above 973K had suppressed the carbon formation, the moles of water formed increased especially at higher CO2/CH4 ratios (being 2 and 3). The increment could be attributed to RWGS reaction attested by the enhanced number of CO moles, declined H2 moles and gradual increment of CO2 conversion. The simulated reactant conversions and product distribution were compared with experimental results in the literatures to study the differences between the real behavior and thermodynamic equilibrium profile of CO2 reforming of methane. The potential of producing decent yields of ethylene, ethane, methanol and dimethyl ether seemed to depend on active and selective catalysts. Higher pressures suppressed the effect of temperature on reactant conversion, augmented carbon deposition and decreased CO and H2 production due to methane decomposition and CO disproportionation reactions. Analysis of oxidative CO2 reforming of methane with equal amount of CH4 and CO2 revealed reactant conversions and syngas yields above 90% corresponded to the optimal operating temperature and feed ratio of 1073K and CO2:CH4:O2=1:1:0.1, respectively. The H2/CO ratio was maintained at unity while water formation was minimized and solid carbon eliminated. |
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| AbstractList | A thermodynamic equilibrium analysis on the multi-reaction system for carbon dioxide reforming of methane in view of carbon formation was performed with Aspen plus based on direct minimization of Gibbs free energy method. The effects of CO sub(2)/CH sub(4) ratio (0.5-3), reaction temperature (573-1473 K) and pressure (1-25 atm) on equilibrium conversions, product compositions and solid carbon were studied. Numerical analysis revealed that the optimal working conditions for syngas production in Fischer-Tropsch synthesis were at temperatures higher than 1173 K for CO sub(2)/CH sub(4) ratio being 1 at which about 4 mol of syngas (H sub(2)/CO = 1) could be produced from 2 mol of reactants with negligible amount of carbon formation. Although temperatures above 973 K had suppressed the carbon formation, the moles of water formed increased especially at higher CO sub(2)/CH sub(4) ratios (being 2 and 3). The increment could be attributed to RWGS reaction attested by the enhanced number of CO moles, declined H sub(2) moles and gradual increment of CO sub(2) conversion. The simulated reactant conversions and product distribution were compared with experimental results in the literatures to study the differences between the real behavior and thermodynamic equilibrium profile of CO sub(2) reforming of methane. The potential of producing decent yields of ethylene, ethane, methanol and dimethyl ether seemed to depend on active and selective catalysts. Higher pressures suppressed the effect of temperature on reactant conversion, augmented carbon deposition and decreased CO and H sub(2) production due to methane decomposition and CO disproportionation reactions. Analysis of oxidative CO sub(2) reforming of methane with equal amount of CH sub(4) and CO sub(2) revealed reactant conversions and syngas yields above 90% corresponded to the optimal operating temperature and feed ratio of 1073 K and CO sub(2):CH sub(4):O sub(2) = 1:1:0.1, respectively. The H sub(2)/CO ratio was maintained at unity while water formation was minimized and solid carbon eliminated. A thermodynamic equilibrium analysis on the multi-reaction system for carbon dioxide reforming of methane in view of carbon formation was performed with Aspen plus based on direct minimization of Gibbs free energy method. The effects of CO₂/CH₄ ratio (0.5–3), reaction temperature (573–1473K) and pressure (1–25atm) on equilibrium conversions, product compositions and solid carbon were studied. Numerical analysis revealed that the optimal working conditions for syngas production in Fischer–Tropsch synthesis were at temperatures higher than 1173K for CO₂/CH₄ ratio being 1 at which about 4mol of syngas (H₂/CO=1) could be produced from 2mol of reactants with negligible amount of carbon formation. Although temperatures above 973K had suppressed the carbon formation, the moles of water formed increased especially at higher CO₂/CH₄ ratios (being 2 and 3). The increment could be attributed to RWGS reaction attested by the enhanced number of CO moles, declined H₂ moles and gradual increment of CO₂ conversion. The simulated reactant conversions and product distribution were compared with experimental results in the literatures to study the differences between the real behavior and thermodynamic equilibrium profile of CO₂ reforming of methane. The potential of producing decent yields of ethylene, ethane, methanol and dimethyl ether seemed to depend on active and selective catalysts. Higher pressures suppressed the effect of temperature on reactant conversion, augmented carbon deposition and decreased CO and H₂ production due to methane decomposition and CO disproportionation reactions. Analysis of oxidative CO₂ reforming of methane with equal amount of CH₄ and CO₂ revealed reactant conversions and syngas yields above 90% corresponded to the optimal operating temperature and feed ratio of 1073K and CO₂:CH₄:O₂=1:1:0.1, respectively. The H₂/CO ratio was maintained at unity while water formation was minimized and solid carbon eliminated. A thermodynamic equilibrium analysis on the multi-reaction system for carbon dioxide reforming of methane in view of carbon formation was performed with Aspen plus based on direct minimization of Gibbs free energy method. The effects of CO2/CH4 ratio (0.5–3), reaction temperature (573–1473K) and pressure (1–25atm) on equilibrium conversions, product compositions and solid carbon were studied. Numerical analysis revealed that the optimal working conditions for syngas production in Fischer–Tropsch synthesis were at temperatures higher than 1173K for CO2/CH4 ratio being 1 at which about 4mol of syngas (H2/CO=1) could be produced from 2mol of reactants with negligible amount of carbon formation. Although temperatures above 973K had suppressed the carbon formation, the moles of water formed increased especially at higher CO2/CH4 ratios (being 2 and 3). The increment could be attributed to RWGS reaction attested by the enhanced number of CO moles, declined H2 moles and gradual increment of CO2 conversion. The simulated reactant conversions and product distribution were compared with experimental results in the literatures to study the differences between the real behavior and thermodynamic equilibrium profile of CO2 reforming of methane. The potential of producing decent yields of ethylene, ethane, methanol and dimethyl ether seemed to depend on active and selective catalysts. Higher pressures suppressed the effect of temperature on reactant conversion, augmented carbon deposition and decreased CO and H2 production due to methane decomposition and CO disproportionation reactions. Analysis of oxidative CO2 reforming of methane with equal amount of CH4 and CO2 revealed reactant conversions and syngas yields above 90% corresponded to the optimal operating temperature and feed ratio of 1073K and CO2:CH4:O2=1:1:0.1, respectively. The H2/CO ratio was maintained at unity while water formation was minimized and solid carbon eliminated. |
| Author | Amin, N.A.S. Nikoo, M. Khoshtinat |
| Author_xml | – sequence: 1 givenname: M. Khoshtinat surname: Nikoo fullname: Nikoo, M. Khoshtinat email: m_k_nikoo@yahoo.com organization: Chemical Reaction Engineering Group (CREG), Faculty of Chemical Engineering, Universiti Teknologi Malaysia, 81310 UTM, Skudai, Johor, Malaysia – sequence: 2 givenname: N.A.S. surname: Amin fullname: Amin, N.A.S. email: noraishah@fkkksa.utm.my organization: Chemical Reaction Engineering Group (CREG), Faculty of Chemical Engineering, Universiti Teknologi Malaysia, 81310 UTM, Skudai, Johor, Malaysia |
| BackLink | http://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=23822565$$DView record in Pascal Francis |
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| SubjectTerms | Applied sciences Carbon Carbon dioxide Carbon formation Carbon monoxide catalysts Conversion Energy Energy. Thermal use of fuels ethane ethylene Exact sciences and technology Fuels Gibbs free energy hydrogen hydrogen production Methane methanol Moles Optimization Reforming synthesis gas temperature Thermodynamic equilibrium working conditions yields |
| Title | Thermodynamic analysis of carbon dioxide reforming of methane in view of solid carbon formation |
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