Conductive silicone elastomers electrodes processable by screen printing
Conductive inks consisting of graphene and carbon black conductive fillers into a polydimethylsiloxane (PDMS) matrix, which can be processed into thin films by screen printing are developed. The influence of filler composition and content on mechanical and electrical properties of the conductive com...
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Published in | Scientific reports Vol. 9; no. 1; pp. 13331 - 11 |
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Main Authors | , , , , , , |
Format | Journal Article |
Language | English |
Published |
London
Nature Publishing Group UK
16.09.2019
Nature Publishing Group |
Subjects | |
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Abstract | Conductive inks consisting of graphene and carbon black conductive fillers into a polydimethylsiloxane (PDMS) matrix, which can be processed into thin films by screen printing are developed. The influence of filler composition and content on mechanical and electrical properties of the conductive composites is investigated. The best composites were evaluated as electrode material for dielectric elastomer actuators and for piezoelectric sensors. With increasing filler content, the electrical properties of the resulting composites of graphite nanoplates (GNPs) or a binary mixture of GNPs and carbon black (CB) with PDMS (M
w
= 139 kg/mol) are enhanced. Hence, PDMS composites filled with GNPs (42 wt.%) or a binary mixture of GNPs/CB (300/150 ratio, 30 wt.% of total filler loading) exhibited constant contact resistance values of 0.5 and 5 Ω determined in life-cycle test, respectively, thus rendering them suitable as electrode materials for piezosensors. On the other hand, dielectric elastomer actuators require more flexible electrode materials, which could be tuned by varying the polymer molecular weight and by reducing the filler content. Therefore, a composite consisting of PDMS (M
w
= 692 kg/mol) and a binary filler mixture of GNPs/CB (150/75 ratio, 18 wt.% of total filler loading) was used for producing the electrodes of dielectric elastomer transducers (DETs). The produced DETs with different electrode thicknesses were characterized in terms of their performance. The negligible hysteresis of the electrode materials is favorable for sensor and actuator applications. |
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AbstractList | Abstract
Conductive inks consisting of graphene and carbon black conductive fillers into a polydimethylsiloxane (PDMS) matrix, which can be processed into thin films by screen printing are developed. The influence of filler composition and content on mechanical and electrical properties of the conductive composites is investigated. The best composites were evaluated as electrode material for dielectric elastomer actuators and for piezoelectric sensors. With increasing filler content, the electrical properties of the resulting composites of graphite nanoplates (GNPs) or a binary mixture of GNPs and carbon black (CB) with PDMS (M
w
= 139 kg/mol) are enhanced. Hence, PDMS composites filled with GNPs (42 wt.%) or a binary mixture of GNPs/CB (300/150 ratio, 30 wt.% of total filler loading) exhibited constant contact resistance values of 0.5 and 5 Ω determined in life-cycle test, respectively, thus rendering them suitable as electrode materials for piezosensors. On the other hand, dielectric elastomer actuators require more flexible electrode materials, which could be tuned by varying the polymer molecular weight and by reducing the filler content. Therefore, a composite consisting of PDMS (M
w
= 692 kg/mol) and a binary filler mixture of GNPs/CB (150/75 ratio, 18 wt.% of total filler loading) was used for producing the electrodes of dielectric elastomer transducers (DETs). The produced DETs with different electrode thicknesses were characterized in terms of their performance. The negligible hysteresis of the electrode materials is favorable for sensor and actuator applications. Conductive inks consisting of graphene and carbon black conductive fillers into a polydimethylsiloxane (PDMS) matrix, which can be processed into thin films by screen printing are developed. The influence of filler composition and content on mechanical and electrical properties of the conductive composites is investigated. The best composites were evaluated as electrode material for dielectric elastomer actuators and for piezoelectric sensors. With increasing filler content, the electrical properties of the resulting composites of graphite nanoplates (GNPs) or a binary mixture of GNPs and carbon black (CB) with PDMS (M = 139 kg/mol) are enhanced. Hence, PDMS composites filled with GNPs (42 wt.%) or a binary mixture of GNPs/CB (300/150 ratio, 30 wt.% of total filler loading) exhibited constant contact resistance values of 0.5 and 5 Ω determined in life-cycle test, respectively, thus rendering them suitable as electrode materials for piezosensors. On the other hand, dielectric elastomer actuators require more flexible electrode materials, which could be tuned by varying the polymer molecular weight and by reducing the filler content. Therefore, a composite consisting of PDMS (M = 692 kg/mol) and a binary filler mixture of GNPs/CB (150/75 ratio, 18 wt.% of total filler loading) was used for producing the electrodes of dielectric elastomer transducers (DETs). The produced DETs with different electrode thicknesses were characterized in terms of their performance. The negligible hysteresis of the electrode materials is favorable for sensor and actuator applications. Conductive inks consisting of graphene and carbon black conductive fillers into a polydimethylsiloxane (PDMS) matrix, which can be processed into thin films by screen printing are developed. The influence of filler composition and content on mechanical and electrical properties of the conductive composites is investigated. The best composites were evaluated as electrode material for dielectric elastomer actuators and for piezoelectric sensors. With increasing filler content, the electrical properties of the resulting composites of graphite nanoplates (GNPs) or a binary mixture of GNPs and carbon black (CB) with PDMS (Mw = 139 kg/mol) are enhanced. Hence, PDMS composites filled with GNPs (42 wt.%) or a binary mixture of GNPs/CB (300/150 ratio, 30 wt.% of total filler loading) exhibited constant contact resistance values of 0.5 and 5 Ω determined in life-cycle test, respectively, thus rendering them suitable as electrode materials for piezosensors. On the other hand, dielectric elastomer actuators require more flexible electrode materials, which could be tuned by varying the polymer molecular weight and by reducing the filler content. Therefore, a composite consisting of PDMS (Mw = 692 kg/mol) and a binary filler mixture of GNPs/CB (150/75 ratio, 18 wt.% of total filler loading) was used for producing the electrodes of dielectric elastomer transducers (DETs). The produced DETs with different electrode thicknesses were characterized in terms of their performance. The negligible hysteresis of the electrode materials is favorable for sensor and actuator applications. Conductive inks consisting of graphene and carbon black conductive fillers into a polydimethylsiloxane (PDMS) matrix, which can be processed into thin films by screen printing are developed. The influence of filler composition and content on mechanical and electrical properties of the conductive composites is investigated. The best composites were evaluated as electrode material for dielectric elastomer actuators and for piezoelectric sensors. With increasing filler content, the electrical properties of the resulting composites of graphite nanoplates (GNPs) or a binary mixture of GNPs and carbon black (CB) with PDMS (M w = 139 kg/mol) are enhanced. Hence, PDMS composites filled with GNPs (42 wt.%) or a binary mixture of GNPs/CB (300/150 ratio, 30 wt.% of total filler loading) exhibited constant contact resistance values of 0.5 and 5 Ω determined in life-cycle test, respectively, thus rendering them suitable as electrode materials for piezosensors. On the other hand, dielectric elastomer actuators require more flexible electrode materials, which could be tuned by varying the polymer molecular weight and by reducing the filler content. Therefore, a composite consisting of PDMS (M w = 692 kg/mol) and a binary filler mixture of GNPs/CB (150/75 ratio, 18 wt.% of total filler loading) was used for producing the electrodes of dielectric elastomer transducers (DETs). The produced DETs with different electrode thicknesses were characterized in terms of their performance. The negligible hysteresis of the electrode materials is favorable for sensor and actuator applications. |
ArticleNumber | 13331 |
Author | Nüesch, Frank A. Dascalu, Mihaela Krämer, Ronny Opris, Dorina M. Häfliger, Daniel Burda, Iurii Quinsaat, Jose Enrico Q. |
Author_xml | – sequence: 1 givenname: Jose Enrico Q. surname: Quinsaat fullname: Quinsaat, Jose Enrico Q. email: jose.quinsaat@gmx.ch organization: Swiss Federal Laboratories for Materials Science and Technology Empa, Laboratory for Functional Polymers – sequence: 2 givenname: Iurii surname: Burda fullname: Burda, Iurii organization: Swiss Federal Laboratories for Materials Science and Technology Empa, Laboratory for Mechanical Systems Engineering – sequence: 3 givenname: Ronny surname: Krämer fullname: Krämer, Ronny organization: Sateco AG – sequence: 4 givenname: Daniel surname: Häfliger fullname: Häfliger, Daniel organization: Sateco AG – sequence: 5 givenname: Frank A. surname: Nüesch fullname: Nüesch, Frank A. organization: Swiss Federal Laboratories for Materials Science and Technology Empa, Laboratory for Functional Polymers, Ecole Polytechnique Fédérale de Lausanne (EPFL), Institut des Matériaux – sequence: 6 givenname: Mihaela surname: Dascalu fullname: Dascalu, Mihaela organization: Swiss Federal Laboratories for Materials Science and Technology Empa, Laboratory for Functional Polymers – sequence: 7 givenname: Dorina M. surname: Opris fullname: Opris, Dorina M. email: dorina.opris@empa.ch organization: Swiss Federal Laboratories for Materials Science and Technology Empa, Laboratory for Functional Polymers |
BackLink | https://www.ncbi.nlm.nih.gov/pubmed/31527691$$D View this record in MEDLINE/PubMed |
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Snippet | Conductive inks consisting of graphene and carbon black conductive fillers into a polydimethylsiloxane (PDMS) matrix, which can be processed into thin films by... Abstract Conductive inks consisting of graphene and carbon black conductive fillers into a polydimethylsiloxane (PDMS) matrix, which can be processed into thin... |
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StartPage | 13331 |
SubjectTerms | 639/301/1005/1006 639/301/1005/1009 639/638/298 Black carbon Carbon black Elastomers Electrical properties Electrodes Humanities and Social Sciences Molecular weight multidisciplinary Polydimethylsiloxane Polymers Science Science (multidisciplinary) Screen printing Silicones Thin films Transducers |
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Title | Conductive silicone elastomers electrodes processable by screen printing |
URI | https://link.springer.com/article/10.1038/s41598-019-49939-8 https://www.ncbi.nlm.nih.gov/pubmed/31527691 https://www.proquest.com/docview/2291323948 https://search.proquest.com/docview/2292999923 https://pubmed.ncbi.nlm.nih.gov/PMC6746820 |
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