High durability and stability of 2D nanofluidic devices for long-term single-molecule sensing

Nanopores in two-dimensional (2D) membranes hold immense potential in single-molecule sensing, osmotic power generation, and information storage. Recent advances in 2D nanopores, especially on single-layer MoS 2 , focus on the scalable growth and manufacturing of nanopore devices. However, there sti...

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Published inNPJ 2D materials and applications Vol. 7; no. 1; p. 11
Main Authors Thakur, Mukeshchand, Cai, Nianduo, Zhang, Miao, Teng, Yunfei, Chernev, Andrey, Tripathi, Mukesh, Zhao, Yanfei, Macha, Michal, Elharouni, Farida, Lihter, Martina, Wen, Liping, Kis, Andras, Radenovic, Aleksandra
Format Journal Article
LanguageEnglish
Published London Nature Publishing Group UK 01.01.2023
Nature Publishing Group
Nature Portfolio
Subjects
639/301/357/1018
639/925/927/1058
Aqueous solutions
Biosensors
Chemistry and Materials Science
Durability
Engineering schools
Fluidics
Graphene
Information storage
Materials Science
Membranes
Molybdenum disulfide
Monolayers
Nanofluids
Nanotechnology
Oxidation
Pore size
Sensors
Shelf life
Signal to noise ratio
Stability analysis
Substrates
Surface stability
Surfaces and Interfaces
Thin Films
Two-dimensional materials
Nanopores
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Abstract Nanopores in two-dimensional (2D) membranes hold immense potential in single-molecule sensing, osmotic power generation, and information storage. Recent advances in 2D nanopores, especially on single-layer MoS 2 , focus on the scalable growth and manufacturing of nanopore devices. However, there still remains a bottleneck in controlling the nanopore stability in atomically thin membranes. Here, we evaluate the major factors responsible for the instability of the monolayer MoS 2 nanopores. We identify chemical oxidation and delamination of monolayers from their underlying substrates as the major reasons for the instability of MoS 2 nanopores. Surface modification of the substrate and reducing the oxygen from the measurement solution improves nanopore stability and dramatically increases their shelf-life. Understanding nanopore growth and stability can provide insights into controlling the pore size, shape and can enable long-term measurements with a high signal-to-noise ratio and engineering durable nanopore devices.
AbstractList Nanopores in two-dimensional (2D) membranes hold immense potential in single-molecule sensing, osmotic power generation, and information storage. Recent advances in 2D nanopores, especially on single-layer MoS2, focus on the scalable growth and manufacturing of nanopore devices. However, there still remains a bottleneck in controlling the nanopore stability in atomically thin membranes. Here, we evaluate the major factors responsible for the instability of the monolayer MoS2 nanopores. We identify chemical oxidation and delamination of monolayers from their underlying substrates as the major reasons for the instability of MoS2 nanopores. Surface modification of the substrate and reducing the oxygen from the measurement solution improves nanopore stability and dramatically increases their shelf-life. Understanding nanopore growth and stability can provide insights into controlling the pore size, shape and can enable long-term measurements with a high signal-to-noise ratio and engineering durable nanopore devices.
Abstract Nanopores in two-dimensional (2D) membranes hold immense potential in single-molecule sensing, osmotic power generation, and information storage. Recent advances in 2D nanopores, especially on single-layer MoS 2 , focus on the scalable growth and manufacturing of nanopore devices. However, there still remains a bottleneck in controlling the nanopore stability in atomically thin membranes. Here, we evaluate the major factors responsible for the instability of the monolayer MoS 2 nanopores. We identify chemical oxidation and delamination of monolayers from their underlying substrates as the major reasons for the instability of MoS 2 nanopores. Surface modification of the substrate and reducing the oxygen from the measurement solution improves nanopore stability and dramatically increases their shelf-life. Understanding nanopore growth and stability can provide insights into controlling the pore size, shape and can enable long-term measurements with a high signal-to-noise ratio and engineering durable nanopore devices.
Nanopores in two-dimensional (2D) membranes hold immense potential in single-molecule sensing, osmotic power generation, and information storage. Recent advances in 2D nanopores, especially on single-layer MoS , focus on the scalable growth and manufacturing of nanopore devices. However, there still remains a bottleneck in controlling the nanopore stability in atomically thin membranes. Here, we evaluate the major factors responsible for the instability of the monolayer MoS nanopores. We identify chemical oxidation and delamination of monolayers from their underlying substrates as the major reasons for the instability of MoS nanopores. Surface modification of the substrate and reducing the oxygen from the measurement solution improves nanopore stability and dramatically increases their shelf-life. Understanding nanopore growth and stability can provide insights into controlling the pore size, shape and can enable long-term measurements with a high signal-to-noise ratio and engineering durable nanopore devices.
Nanopores in two-dimensional (2D) membranes hold immense potential in single-molecule sensing, osmotic power generation, and information storage. Recent advances in 2D nanopores, especially on single-layer MoS 2 , focus on the scalable growth and manufacturing of nanopore devices. However, there still remains a bottleneck in controlling the nanopore stability in atomically thin membranes. Here, we evaluate the major factors responsible for the instability of the monolayer MoS 2 nanopores. We identify chemical oxidation and delamination of monolayers from their underlying substrates as the major reasons for the instability of MoS 2 nanopores. Surface modification of the substrate and reducing the oxygen from the measurement solution improves nanopore stability and dramatically increases their shelf-life. Understanding nanopore growth and stability can provide insights into controlling the pore size, shape and can enable long-term measurements with a high signal-to-noise ratio and engineering durable nanopore devices.
Abstract Nanopores in two-dimensional (2D) membranes hold immense potential in single-molecule sensing, osmotic power generation, and information storage. Recent advances in 2D nanopores, especially on single-layer MoS2, focus on the scalable growth and manufacturing of nanopore devices. However, there still remains a bottleneck in controlling the nanopore stability in atomically thin membranes. Here, we evaluate the major factors responsible for the instability of the monolayer MoS2 nanopores. We identify chemical oxidation and delamination of monolayers from their underlying substrates as the major reasons for the instability of MoS2 nanopores. Surface modification of the substrate and reducing the oxygen from the measurement solution improves nanopore stability and dramatically increases their shelf-life. Understanding nanopore growth and stability can provide insights into controlling the pore size, shape and can enable long-term measurements with a high signal-to-noise ratio and engineering durable nanopore devices.
ArticleNumber 11
Author Zhang, Miao
Wen, Liping
Elharouni, Farida
Teng, Yunfei
Macha, Michal
Chernev, Andrey
Tripathi, Mukesh
Lihter, Martina
Thakur, Mukeshchand
Zhao, Yanfei
Kis, Andras
Radenovic, Aleksandra
Cai, Nianduo
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Keywords Two-dimensional materials
Nanopores
Language English
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PublicationTitle NPJ 2D materials and applications
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Snippet Nanopores in two-dimensional (2D) membranes hold immense potential in single-molecule sensing, osmotic power generation, and information storage. Recent...
Abstract Nanopores in two-dimensional (2D) membranes hold immense potential in single-molecule sensing, osmotic power generation, and information storage....
Abstract Nanopores in two-dimensional (2D) membranes hold immense potential in single-molecule sensing, osmotic power generation, and information storage....
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SubjectTerms 639/301/357/1018
639/925/927/1058
Aqueous solutions
Biosensors
Chemistry and Materials Science
Durability
Engineering schools
Fluidics
Graphene
Information storage
Materials Science
Membranes
Molybdenum disulfide
Monolayers
Nanofluids
Nanotechnology
Oxidation
Pore size
Sensors
Shelf life
Signal to noise ratio
Stability analysis
Substrates
Surface stability
Surfaces and Interfaces
Thin Films
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Title High durability and stability of 2D nanofluidic devices for long-term single-molecule sensing
URI https://link.springer.com/article/10.1038/s41699-023-00373-5
https://www.ncbi.nlm.nih.gov/pubmed/38665480
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https://doaj.org/article/7fbd7c75edea4429b05cb27c86640419
Volume 7
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