Fluoropolymer sorbent for efficient and selective capturing of per- and polyfluorinated compounds

Per- and poly-fluoroalkyl substances (PFAS) have gained widespread attention due to their adverse effects on health and environment. Developing efficient technology to capture PFAS from contaminated sources remains a great challenge. In this study, we introduce a type of reusable polymeric sorbent (...

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Published inNature communications Vol. 15; no. 1; pp. 8269 - 10
Main Authors Yang, Zhuojing, Zhu, Yutong, Tan, Xiao, Gunjal, Samruddhi Jayendra Jayendra, Dewapriya, Pradeep, Wang, Yiqing, Xin, Ruijing, Fu, Changkui, Liu, Kehan, Macintosh, Katie, Sprague, Lee G., Leung, Lam, Hopkins, Timothy E., Thomas, Kevin V., Guo, Jianhua, Whittaker, Andrew K., Zhang, Cheng
Format Journal Article
LanguageEnglish
Published London Nature Publishing Group UK 27.09.2024
Nature Publishing Group
Nature Portfolio
Subjects
639/301
639/638/455
Detection limits
Drinking water
Fluoropolymers
Humanities and Social Sciences
Impurities
Landfill
Landfills
Leachates
multidisciplinary
Perfluoroalkyl & polyfluoroalkyl substances
Perfluorochemicals
Polymers
Resins
Science
Science (multidisciplinary)
Sorbents
Waste disposal sites
Water pollution
Online AccessGet full text
ISSN2041-1723
2041-1723
DOI10.1038/s41467-024-52690-y

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Abstract Per- and poly-fluoroalkyl substances (PFAS) have gained widespread attention due to their adverse effects on health and environment. Developing efficient technology to capture PFAS from contaminated sources remains a great challenge. In this study, we introduce a type of reusable polymeric sorbent (PFPE-IEX + ) for rapid, efficient, and selective removal of multiple PFAS impurities from various contaminated water sources. The resin achieves >98% removal efficiency ([PFPE-IEX + ] = 0.5–5 mg mL −1 , [PFAS] 0  = 1–10 ppb in potable water and landfill leachate) and >500 mg g −1 sorption capacity for the 11 types of examined PFAS. We achieve efficient PFAS removal without breakthrough and subsequent resin regeneration and demonstrate good PFAS recovery in a proof-of-concept cartridge setup. The outcomes of this study offer valuable guidance to the design of platforms for efficient and selective PFAS capture from contaminated water, such as drinking water and landfill leachate. It is challenging to remove Per- and polyfluoroalkyl substances (PFAS) from water. Here, authors developed a polymer sorbent capable of selectively and efficiently removing PFAS from contaminated water sources to levels below detection limits.
AbstractList Per- and poly-fluoroalkyl substances (PFAS) have gained widespread attention due to their adverse effects on health and environment. Developing efficient technology to capture PFAS from contaminated sources remains a great challenge. In this study, we introduce a type of reusable polymeric sorbent (PFPE-IEX + ) for rapid, efficient, and selective removal of multiple PFAS impurities from various contaminated water sources. The resin achieves >98% removal efficiency ([PFPE-IEX + ] = 0.5-5 mg mL-1, [PFAS]0 = 1-10 ppb in potable water and landfill leachate) and >500 mg g-1 sorption capacity for the 11 types of examined PFAS. We achieve efficient PFAS removal without breakthrough and subsequent resin regeneration and demonstrate good PFAS recovery in a proof-of-concept cartridge setup. The outcomes of this study offer valuable guidance to the design of platforms for efficient and selective PFAS capture from contaminated water, such as drinking water and landfill leachate.Per- and poly-fluoroalkyl substances (PFAS) have gained widespread attention due to their adverse effects on health and environment. Developing efficient technology to capture PFAS from contaminated sources remains a great challenge. In this study, we introduce a type of reusable polymeric sorbent (PFPE-IEX + ) for rapid, efficient, and selective removal of multiple PFAS impurities from various contaminated water sources. The resin achieves >98% removal efficiency ([PFPE-IEX + ] = 0.5-5 mg mL-1, [PFAS]0 = 1-10 ppb in potable water and landfill leachate) and >500 mg g-1 sorption capacity for the 11 types of examined PFAS. We achieve efficient PFAS removal without breakthrough and subsequent resin regeneration and demonstrate good PFAS recovery in a proof-of-concept cartridge setup. The outcomes of this study offer valuable guidance to the design of platforms for efficient and selective PFAS capture from contaminated water, such as drinking water and landfill leachate.
Abstract Per- and poly-fluoroalkyl substances (PFAS) have gained widespread attention due to their adverse effects on health and environment. Developing efficient technology to capture PFAS from contaminated sources remains a great challenge. In this study, we introduce a type of reusable polymeric sorbent (PFPE-IEX + ) for rapid, efficient, and selective removal of multiple PFAS impurities from various contaminated water sources. The resin achieves >98% removal efficiency ([PFPE-IEX + ] = 0.5–5 mg mL−1, [PFAS]0 = 1–10 ppb in potable water and landfill leachate) and >500 mg g−1 sorption capacity for the 11 types of examined PFAS. We achieve efficient PFAS removal without breakthrough and subsequent resin regeneration and demonstrate good PFAS recovery in a proof-of-concept cartridge setup. The outcomes of this study offer valuable guidance to the design of platforms for efficient and selective PFAS capture from contaminated water, such as drinking water and landfill leachate.
Per- and poly-fluoroalkyl substances (PFAS) have gained widespread attention due to their adverse effects on health and environment. Developing efficient technology to capture PFAS from contaminated sources remains a great challenge. In this study, we introduce a type of reusable polymeric sorbent (PFPE-IEX + ) for rapid, efficient, and selective removal of multiple PFAS impurities from various contaminated water sources. The resin achieves >98% removal efficiency ([PFPE-IEX + ] = 0.5–5 mg mL −1 , [PFAS] 0  = 1–10 ppb in potable water and landfill leachate) and >500 mg g −1 sorption capacity for the 11 types of examined PFAS. We achieve efficient PFAS removal without breakthrough and subsequent resin regeneration and demonstrate good PFAS recovery in a proof-of-concept cartridge setup. The outcomes of this study offer valuable guidance to the design of platforms for efficient and selective PFAS capture from contaminated water, such as drinking water and landfill leachate. It is challenging to remove Per- and polyfluoroalkyl substances (PFAS) from water. Here, authors developed a polymer sorbent capable of selectively and efficiently removing PFAS from contaminated water sources to levels below detection limits.
Per- and poly-fluoroalkyl substances (PFAS) have gained widespread attention due to their adverse effects on health and environment. Developing efficient technology to capture PFAS from contaminated sources remains a great challenge. In this study, we introduce a type of reusable polymeric sorbent (PFPE-IEX + ) for rapid, efficient, and selective removal of multiple PFAS impurities from various contaminated water sources. The resin achieves >98% removal efficiency ([PFPE-IEX + ] = 0.5-5 mg mL , [PFAS]  = 1-10 ppb in potable water and landfill leachate) and >500 mg g sorption capacity for the 11 types of examined PFAS. We achieve efficient PFAS removal without breakthrough and subsequent resin regeneration and demonstrate good PFAS recovery in a proof-of-concept cartridge setup. The outcomes of this study offer valuable guidance to the design of platforms for efficient and selective PFAS capture from contaminated water, such as drinking water and landfill leachate.
Per- and poly-fluoroalkyl substances (PFAS) have gained widespread attention due to their adverse effects on health and environment. Developing efficient technology to capture PFAS from contaminated sources remains a great challenge. In this study, we introduce a type of reusable polymeric sorbent (PFPE-IEX + ) for rapid, efficient, and selective removal of multiple PFAS impurities from various contaminated water sources. The resin achieves >98% removal efficiency ([PFPE-IEX + ] = 0.5–5 mg mL−1, [PFAS]0 = 1–10 ppb in potable water and landfill leachate) and >500 mg g−1 sorption capacity for the 11 types of examined PFAS. We achieve efficient PFAS removal without breakthrough and subsequent resin regeneration and demonstrate good PFAS recovery in a proof-of-concept cartridge setup. The outcomes of this study offer valuable guidance to the design of platforms for efficient and selective PFAS capture from contaminated water, such as drinking water and landfill leachate.It is challenging to remove Per- and polyfluoroalkyl substances (PFAS) from water. Here, authors developed a polymer sorbent capable of selectively and efficiently removing PFAS from contaminated water sources to levels below detection limits.
ArticleNumber 8269
Author Tan, Xiao
Macintosh, Katie
Zhang, Cheng
Hopkins, Timothy E.
Liu, Kehan
Gunjal, Samruddhi Jayendra Jayendra
Sprague, Lee G.
Fu, Changkui
Leung, Lam
Wang, Yiqing
Zhu, Yutong
Whittaker, Andrew K.
Yang, Zhuojing
Xin, Ruijing
Dewapriya, Pradeep
Guo, Jianhua
Thomas, Kevin V.
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BackLink https://www.ncbi.nlm.nih.gov/pubmed/39333086$$D View this record in MEDLINE/PubMed
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Snippet Per- and poly-fluoroalkyl substances (PFAS) have gained widespread attention due to their adverse effects on health and environment. Developing efficient...
Abstract Per- and poly-fluoroalkyl substances (PFAS) have gained widespread attention due to their adverse effects on health and environment. Developing...
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SubjectTerms 639/301
639/638/455
Detection limits
Drinking water
Fluoropolymers
Humanities and Social Sciences
Impurities
Landfill
Landfills
Leachates
multidisciplinary
Perfluoroalkyl & polyfluoroalkyl substances
Perfluorochemicals
Polymers
Resins
Science
Science (multidisciplinary)
Sorbents
Waste disposal sites
Water pollution
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Title Fluoropolymer sorbent for efficient and selective capturing of per- and polyfluorinated compounds
URI https://link.springer.com/article/10.1038/s41467-024-52690-y
https://www.ncbi.nlm.nih.gov/pubmed/39333086
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https://pubmed.ncbi.nlm.nih.gov/PMC11436832
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Volume 15
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