A core–shell fiber moisture-driven electric generator enabled by synergetic complex coacervation and built-in potential

Moisture-driven electricity generators (MEGs) have been extensively researched; however, high-performance flexible variants have seldom been demonstrated. Here we present a novel complex coacervation with built-in potential strategy for developing a high-performance uniaxial MEG, featuring a core of...

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Published inNature communications Vol. 15; no. 1; pp. 10056 - 13
Main Authors Zan, Guangtao, Jiang, Wei, Kim, HoYeon, Zhao, Kaiying, Li, Shengyou, Lee, Kyuho, Jang, Jihye, Kim, Gwanho, Shin, EunAe, Kim, Woojoong, Oh, Jin Woo, Kim, Yeonji, Park, Jong Woong, Kim, Taebin, Lee, Seonju, Oh, Ji Hye, Shin, Jowon, Kim, Hyeong Jun, Park, Cheolmin
Format Journal Article
LanguageEnglish
Published London Nature Publishing Group UK 20.11.2024
Nature Publishing Group
Nature Portfolio
Subjects
639/301/299
639/4077/4072
Alginic acid
Coacervation
Current carriers
Electric generators
Electric potential
Generators
Humanities and Social Sciences
Moisture
multidisciplinary
Nanoribbons
Performance degradation
Polyelectrolytes
Relative humidity
Science
Science (multidisciplinary)
Sodium alginate
Sodium channels (voltage-gated)
Surface charge
Synapses
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Abstract Moisture-driven electricity generators (MEGs) have been extensively researched; however, high-performance flexible variants have seldom been demonstrated. Here we present a novel complex coacervation with built-in potential strategy for developing a high-performance uniaxial MEG, featuring a core of poly(3,4-ethylenedioxythiophene) (PEDOT) with a built-in charge potential and a gel shell composed of poly(diallyldimethylammonium chloride) (PDDA) and sodium alginate (NaAlg) coacervate. The complex coacervation of two oppositely charged polyelectrolytes produces extra mobile carriers and free volume in the device; meanwhile, the PEDOT core’s surface charge significantly accelerates carrier diffusion. Consequently, the uniaxial fiber-based MEG demonstrates breakthrough performance, achieving an output voltage of up to 0.8 V, a maximum current density of 1.05 mA/cm 2 , and a power density of 184 μW/cm 2 at 20% relative humidity. Moreover, the mechanical robustness is ensured for the PEDOT nanoribbon substrate without performance degradation even after 100,000 folding cycles, making it suitable for self-powered human interactive sensor and synapse. Notably, we have constructed the inaugural MEG-synapse self-powered device, with a fiber-based MEG successfully operating a synaptic memristor, thereby emulating autonomous human synapses linked with fibrous neurons. Overall, this work pioneers innovative design strategies and application scenarios for high-performance MEGs. The authors present a core–shell fiber moisture-driven electric generator by a synergetic complex coacervation and built-in potential strategy, enabling self-powered human interactive sensors and synaptic devices.
AbstractList Abstract Moisture-driven electricity generators (MEGs) have been extensively researched; however, high-performance flexible variants have seldom been demonstrated. Here we present a novel complex coacervation with built-in potential strategy for developing a high-performance uniaxial MEG, featuring a core of poly(3,4-ethylenedioxythiophene) (PEDOT) with a built-in charge potential and a gel shell composed of poly(diallyldimethylammonium chloride) (PDDA) and sodium alginate (NaAlg) coacervate. The complex coacervation of two oppositely charged polyelectrolytes produces extra mobile carriers and free volume in the device; meanwhile, the PEDOT core’s surface charge significantly accelerates carrier diffusion. Consequently, the uniaxial fiber-based MEG demonstrates breakthrough performance, achieving an output voltage of up to 0.8 V, a maximum current density of 1.05 mA/cm2, and a power density of 184 μW/cm2 at 20% relative humidity. Moreover, the mechanical robustness is ensured for the PEDOT nanoribbon substrate without performance degradation even after 100,000 folding cycles, making it suitable for self-powered human interactive sensor and synapse. Notably, we have constructed the inaugural MEG-synapse self-powered device, with a fiber-based MEG successfully operating a synaptic memristor, thereby emulating autonomous human synapses linked with fibrous neurons. Overall, this work pioneers innovative design strategies and application scenarios for high-performance MEGs.
Moisture-driven electricity generators (MEGs) have been extensively researched; however, high-performance flexible variants have seldom been demonstrated. Here we present a novel complex coacervation with built-in potential strategy for developing a high-performance uniaxial MEG, featuring a core of poly(3,4-ethylenedioxythiophene) (PEDOT) with a built-in charge potential and a gel shell composed of poly(diallyldimethylammonium chloride) (PDDA) and sodium alginate (NaAlg) coacervate. The complex coacervation of two oppositely charged polyelectrolytes produces extra mobile carriers and free volume in the device; meanwhile, the PEDOT core’s surface charge significantly accelerates carrier diffusion. Consequently, the uniaxial fiber-based MEG demonstrates breakthrough performance, achieving an output voltage of up to 0.8 V, a maximum current density of 1.05 mA/cm2, and a power density of 184 μW/cm2 at 20% relative humidity. Moreover, the mechanical robustness is ensured for the PEDOT nanoribbon substrate without performance degradation even after 100,000 folding cycles, making it suitable for self-powered human interactive sensor and synapse. Notably, we have constructed the inaugural MEG-synapse self-powered device, with a fiber-based MEG successfully operating a synaptic memristor, thereby emulating autonomous human synapses linked with fibrous neurons. Overall, this work pioneers innovative design strategies and application scenarios for high-performance MEGs.The authors present a core–shell fiber moisture-driven electric generator by a synergetic complex coacervation and built-in potential strategy, enabling self-powered human interactive sensors and synaptic devices.
Moisture-driven electricity generators (MEGs) have been extensively researched; however, high-performance flexible variants have seldom been demonstrated. Here we present a novel complex coacervation with built-in potential strategy for developing a high-performance uniaxial MEG, featuring a core of poly(3,4-ethylenedioxythiophene) (PEDOT) with a built-in charge potential and a gel shell composed of poly(diallyldimethylammonium chloride) (PDDA) and sodium alginate (NaAlg) coacervate. The complex coacervation of two oppositely charged polyelectrolytes produces extra mobile carriers and free volume in the device; meanwhile, the PEDOT core’s surface charge significantly accelerates carrier diffusion. Consequently, the uniaxial fiber-based MEG demonstrates breakthrough performance, achieving an output voltage of up to 0.8 V, a maximum current density of 1.05 mA/cm 2 , and a power density of 184 μW/cm 2 at 20% relative humidity. Moreover, the mechanical robustness is ensured for the PEDOT nanoribbon substrate without performance degradation even after 100,000 folding cycles, making it suitable for self-powered human interactive sensor and synapse. Notably, we have constructed the inaugural MEG-synapse self-powered device, with a fiber-based MEG successfully operating a synaptic memristor, thereby emulating autonomous human synapses linked with fibrous neurons. Overall, this work pioneers innovative design strategies and application scenarios for high-performance MEGs. The authors present a core–shell fiber moisture-driven electric generator by a synergetic complex coacervation and built-in potential strategy, enabling self-powered human interactive sensors and synaptic devices.
Moisture-driven electricity generators (MEGs) have been extensively researched; however, high-performance flexible variants have seldom been demonstrated. Here we present a novel complex coacervation with built-in potential strategy for developing a high-performance uniaxial MEG, featuring a core of poly(3,4-ethylenedioxythiophene) (PEDOT) with a built-in charge potential and a gel shell composed of poly(diallyldimethylammonium chloride) (PDDA) and sodium alginate (NaAlg) coacervate. The complex coacervation of two oppositely charged polyelectrolytes produces extra mobile carriers and free volume in the device; meanwhile, the PEDOT core's surface charge significantly accelerates carrier diffusion. Consequently, the uniaxial fiber-based MEG demonstrates breakthrough performance, achieving an output voltage of up to 0.8 V, a maximum current density of 1.05 mA/cm , and a power density of 184 μW/cm at 20% relative humidity. Moreover, the mechanical robustness is ensured for the PEDOT nanoribbon substrate without performance degradation even after 100,000 folding cycles, making it suitable for self-powered human interactive sensor and synapse. Notably, we have constructed the inaugural MEG-synapse self-powered device, with a fiber-based MEG successfully operating a synaptic memristor, thereby emulating autonomous human synapses linked with fibrous neurons. Overall, this work pioneers innovative design strategies and application scenarios for high-performance MEGs.
Moisture-driven electricity generators (MEGs) have been extensively researched; however, high-performance flexible variants have seldom been demonstrated. Here we present a novel complex coacervation with built-in potential strategy for developing a high-performance uniaxial MEG, featuring a core of poly(3,4-ethylenedioxythiophene) (PEDOT) with a built-in charge potential and a gel shell composed of poly(diallyldimethylammonium chloride) (PDDA) and sodium alginate (NaAlg) coacervate. The complex coacervation of two oppositely charged polyelectrolytes produces extra mobile carriers and free volume in the device; meanwhile, the PEDOT core's surface charge significantly accelerates carrier diffusion. Consequently, the uniaxial fiber-based MEG demonstrates breakthrough performance, achieving an output voltage of up to 0.8 V, a maximum current density of 1.05 mA/cm2, and a power density of 184 μW/cm2 at 20% relative humidity. Moreover, the mechanical robustness is ensured for the PEDOT nanoribbon substrate without performance degradation even after 100,000 folding cycles, making it suitable for self-powered human interactive sensor and synapse. Notably, we have constructed the inaugural MEG-synapse self-powered device, with a fiber-based MEG successfully operating a synaptic memristor, thereby emulating autonomous human synapses linked with fibrous neurons. Overall, this work pioneers innovative design strategies and application scenarios for high-performance MEGs.Moisture-driven electricity generators (MEGs) have been extensively researched; however, high-performance flexible variants have seldom been demonstrated. Here we present a novel complex coacervation with built-in potential strategy for developing a high-performance uniaxial MEG, featuring a core of poly(3,4-ethylenedioxythiophene) (PEDOT) with a built-in charge potential and a gel shell composed of poly(diallyldimethylammonium chloride) (PDDA) and sodium alginate (NaAlg) coacervate. The complex coacervation of two oppositely charged polyelectrolytes produces extra mobile carriers and free volume in the device; meanwhile, the PEDOT core's surface charge significantly accelerates carrier diffusion. Consequently, the uniaxial fiber-based MEG demonstrates breakthrough performance, achieving an output voltage of up to 0.8 V, a maximum current density of 1.05 mA/cm2, and a power density of 184 μW/cm2 at 20% relative humidity. Moreover, the mechanical robustness is ensured for the PEDOT nanoribbon substrate without performance degradation even after 100,000 folding cycles, making it suitable for self-powered human interactive sensor and synapse. Notably, we have constructed the inaugural MEG-synapse self-powered device, with a fiber-based MEG successfully operating a synaptic memristor, thereby emulating autonomous human synapses linked with fibrous neurons. Overall, this work pioneers innovative design strategies and application scenarios for high-performance MEGs.
ArticleNumber 10056
Author Shin, Jowon
Park, Cheolmin
Lee, Seonju
Lee, Kyuho
Jiang, Wei
Kim, Gwanho
Kim, Taebin
Shin, EunAe
Kim, Yeonji
Park, Jong Woong
Jang, Jihye
Oh, Jin Woo
Oh, Ji Hye
Zhao, Kaiying
Zan, Guangtao
Kim, HoYeon
Kim, Woojoong
Kim, Hyeong Jun
Li, Shengyou
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BackLink https://www.ncbi.nlm.nih.gov/pubmed/39567507$$D View this record in MEDLINE/PubMed
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Snippet Moisture-driven electricity generators (MEGs) have been extensively researched; however, high-performance flexible variants have seldom been demonstrated. Here...
Abstract Moisture-driven electricity generators (MEGs) have been extensively researched; however, high-performance flexible variants have seldom been...
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SubjectTerms 639/301/299
639/4077/4072
Alginic acid
Coacervation
Current carriers
Electric generators
Electric potential
Generators
Humanities and Social Sciences
Moisture
multidisciplinary
Nanoribbons
Performance degradation
Polyelectrolytes
Relative humidity
Science
Science (multidisciplinary)
Sodium alginate
Sodium channels (voltage-gated)
Surface charge
Synapses
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Title A core–shell fiber moisture-driven electric generator enabled by synergetic complex coacervation and built-in potential
URI https://link.springer.com/article/10.1038/s41467-024-54442-4
https://www.ncbi.nlm.nih.gov/pubmed/39567507
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https://pubmed.ncbi.nlm.nih.gov/PMC11579398
https://doaj.org/article/92ba17b0c3d04ad39d12fbef82e308be
Volume 15
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