Macroscopically uniform interface layer with Li+ conductive channels for high-performance Li metal batteries

• Published in: Nature communications Vol. 15; no. 1; pp. 10045 - 12
• Main Authors: Chen, Qian, Gao, Binyin, Yang, Zhilin, Li, Yong, Zhai, QingWei, Jia, Yangyu, Zhang, Qiannan, Gu, Xiaokang, Zuo, Jinghan, Wang, Lei, Wang, Tianshuai, Zhai, Pengbo, Yang, Cheng, Gong, Yongji
• Format: Journal Article
• Language: English
• Published: London Nature Publishing Group UK 20.11.2024; Nature Publishing Group; Nature Portfolio
• Subjects: 140/146; 147/135; 147/143; 147/3; 639/301/299/891; 639/301/357/1018; 639/4077/4079/891; Basal plane; Battery cycles; Carbon; Carbon nitride; Channel pores; Channels; Deposition; Grain boundaries; Humanities and Social Sciences; Ion transport; Lithium; Lithium batteries; Lithium ions; Metals; multidisciplinary; Pollutant deposition; Science; Science (multidisciplinary); Solid electrolytes; Tortuosity

The numerous grainboundaries solid electrolyte interface, whether naturally occurring or artificially designed, leads to non-uniform Li metal deposition and consequently results in poor full-battery performance. Herein, a lithium-ion selective transport layer is reported to achieve a highly efficien...