Mass transport and charge transfer through an electrified interface between metallic lithium and solid-state electrolytes

• Published in: Communications chemistry Vol. 6; no. 1; pp. 124 - 8
• Main Authors: Katzenmeier, Leon, Gößwein, Manuel, Carstensen, Leif, Sterzinger, Johannes, Ederer, Michael, Müller-Buschbaum, Peter, Gagliardi, Alessio, Bandarenka, Aliaksandr S.
• Format: Journal Article
• Language: English
• Published: London Nature Publishing Group UK 15.06.2023; Nature Publishing Group; Nature Portfolio
• Subjects: 639/301/119/544; 639/638/161/891; Charge transfer; Chemistry; Chemistry and Materials Science; Chemistry/Food Science; Depletion; Electrodes; Electrolytes; Energy storage; Impedance; Interfaces; Lithium; Lithium-ion batteries; Mass transport; Molten salt electrolytes; Rechargeable batteries; Solid electrolytes; Solid state; Space charge; Spectroellipsometry

All-solid-state Li-ion batteries are one of the most promising energy storage devices for future automotive applications as high energy density metallic Li anodes can be safely used. However, introducing solid-state electrolytes needs a better understanding of the forming electrified electrode/elect...