Lamella-nanostructured eutectic zinc–aluminum alloys as reversible and dendrite-free anodes for aqueous rechargeable batteries
Metallic zinc is an attractive anode material for aqueous rechargeable batteries because of its high theoretical capacity and low cost. However, state-of-the-art zinc anodes suffer from low coulombic efficiency and severe dendrite growth during stripping/plating processes, hampering their practical...
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| Published in | Nature communications Vol. 11; no. 1; pp. 1634 - 9 |
|---|---|
| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
02.04.2020
Nature Publishing Group Nature Portfolio |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Metallic zinc is an attractive anode material for aqueous rechargeable batteries because of its high theoretical capacity and low cost. However, state-of-the-art zinc anodes suffer from low coulombic efficiency and severe dendrite growth during stripping/plating processes, hampering their practical applications. Here we show that eutectic-composition alloying of zinc and aluminum as an effective strategy substantially tackles these irreversibility issues by making use of their lamellar structure, composed of alternating zinc and aluminum nanolamellas. The lamellar nanostructure not only promotes zinc stripping from precursor eutectic Zn
88
Al
12
(at%) alloys, but produces core/shell aluminum/aluminum sesquioxide interlamellar nanopatterns in situ to in turn guide subsequent growth of zinc, enabling dendrite-free zinc stripping/plating for more than 2000 h in oxygen-absent aqueous electrolyte. These outstanding electrochemical properties enlist zinc-ion batteries constructed with Zn
88
Al
12
alloy anode and K
x
MnO
2
cathode to deliver high-density energy at high levels of electrical power and retain 100% capacity after 200 hours.
Aqueous rechargeable Zn-ion batteries are attractive energy storage devices, but their wide adoption is impeded by the irreversible metallic Zn anode. Here the authors report lamellar-nanostructured eutectic Zn/Al alloys as reversible and dendrite-free anodes for improved battery performance. |
|---|---|
| AbstractList | Metallic zinc is an attractive anode material for aqueous rechargeable batteries because of its high theoretical capacity and low cost. However, state-of-the-art zinc anodes suffer from low coulombic efficiency and severe dendrite growth during stripping/plating processes, hampering their practical applications. Here we show that eutectic-composition alloying of zinc and aluminum as an effective strategy substantially tackles these irreversibility issues by making use of their lamellar structure, composed of alternating zinc and aluminum nanolamellas. The lamellar nanostructure not only promotes zinc stripping from precursor eutectic Zn
88
Al
12
(at%) alloys, but produces core/shell aluminum/aluminum sesquioxide interlamellar nanopatterns in situ to in turn guide subsequent growth of zinc, enabling dendrite-free zinc stripping/plating for more than 2000 h in oxygen-absent aqueous electrolyte. These outstanding electrochemical properties enlist zinc-ion batteries constructed with Zn
88
Al
12
alloy anode and K
x
MnO
2
cathode to deliver high-density energy at high levels of electrical power and retain 100% capacity after 200 hours.
Aqueous rechargeable Zn-ion batteries are attractive energy storage devices, but their wide adoption is impeded by the irreversible metallic Zn anode. Here the authors report lamellar-nanostructured eutectic Zn/Al alloys as reversible and dendrite-free anodes for improved battery performance. Metallic zinc is an attractive anode material for aqueous rechargeable batteries because of its high theoretical capacity and low cost. However, state-of-the-art zinc anodes suffer from low coulombic efficiency and severe dendrite growth during stripping/plating processes, hampering their practical applications. Here we show that eutectic-composition alloying of zinc and aluminum as an effective strategy substantially tackles these irreversibility issues by making use of their lamellar structure, composed of alternating zinc and aluminum nanolamellas. The lamellar nanostructure not only promotes zinc stripping from precursor eutectic Zn88Al12 (at%) alloys, but produces core/shell aluminum/aluminum sesquioxide interlamellar nanopatterns in situ to in turn guide subsequent growth of zinc, enabling dendrite-free zinc stripping/plating for more than 2000 h in oxygen-absent aqueous electrolyte. These outstanding electrochemical properties enlist zinc-ion batteries constructed with Zn88Al12 alloy anode and KxMnO2 cathode to deliver high-density energy at high levels of electrical power and retain 100% capacity after 200 hours.Aqueous rechargeable Zn-ion batteries are attractive energy storage devices, but their wide adoption is impeded by the irreversible metallic Zn anode. Here the authors report lamellar-nanostructured eutectic Zn/Al alloys as reversible and dendrite-free anodes for improved battery performance. Metallic zinc is an attractive anode material for aqueous rechargeable batteries because of its high theoretical capacity and low cost. However, state-of-the-art zinc anodes suffer from low coulombic efficiency and severe dendrite growth during stripping/plating processes, hampering their practical applications. Here we show that eutectic-composition alloying of zinc and aluminum as an effective strategy substantially tackles these irreversibility issues by making use of their lamellar structure, composed of alternating zinc and aluminum nanolamellas. The lamellar nanostructure not only promotes zinc stripping from precursor eutectic Zn 88 Al 12 (at%) alloys, but produces core/shell aluminum/aluminum sesquioxide interlamellar nanopatterns in situ to in turn guide subsequent growth of zinc, enabling dendrite-free zinc stripping/plating for more than 2000 h in oxygen-absent aqueous electrolyte. These outstanding electrochemical properties enlist zinc-ion batteries constructed with Zn 88 Al 12 alloy anode and K x MnO 2 cathode to deliver high-density energy at high levels of electrical power and retain 100% capacity after 200 hours. Metallic zinc is an attractive anode material for aqueous rechargeable batteries because of its high theoretical capacity and low cost. However, state-of-the-art zinc anodes suffer from low coulombic efficiency and severe dendrite growth during stripping/plating processes, hampering their practical applications. Here we show that eutectic-composition alloying of zinc and aluminum as an effective strategy substantially tackles these irreversibility issues by making use of their lamellar structure, composed of alternating zinc and aluminum nanolamellas. The lamellar nanostructure not only promotes zinc stripping from precursor eutectic Zn88Al12 (at%) alloys, but produces core/shell aluminum/aluminum sesquioxide interlamellar nanopatterns in situ to in turn guide subsequent growth of zinc, enabling dendrite-free zinc stripping/plating for more than 2000 h in oxygen-absent aqueous electrolyte. These outstanding electrochemical properties enlist zinc-ion batteries constructed with Zn88Al12 alloy anode and KxMnO2 cathode to deliver high-density energy at high levels of electrical power and retain 100% capacity after 200 hours.Metallic zinc is an attractive anode material for aqueous rechargeable batteries because of its high theoretical capacity and low cost. However, state-of-the-art zinc anodes suffer from low coulombic efficiency and severe dendrite growth during stripping/plating processes, hampering their practical applications. Here we show that eutectic-composition alloying of zinc and aluminum as an effective strategy substantially tackles these irreversibility issues by making use of their lamellar structure, composed of alternating zinc and aluminum nanolamellas. The lamellar nanostructure not only promotes zinc stripping from precursor eutectic Zn88Al12 (at%) alloys, but produces core/shell aluminum/aluminum sesquioxide interlamellar nanopatterns in situ to in turn guide subsequent growth of zinc, enabling dendrite-free zinc stripping/plating for more than 2000 h in oxygen-absent aqueous electrolyte. These outstanding electrochemical properties enlist zinc-ion batteries constructed with Zn88Al12 alloy anode and KxMnO2 cathode to deliver high-density energy at high levels of electrical power and retain 100% capacity after 200 hours. Metallic zinc is an attractive anode material for aqueous rechargeable batteries because of its high theoretical capacity and low cost. However, state-of-the-art zinc anodes suffer from low coulombic efficiency and severe dendrite growth during stripping/plating processes, hampering their practical applications. Here we show that eutectic-composition alloying of zinc and aluminum as an effective strategy substantially tackles these irreversibility issues by making use of their lamellar structure, composed of alternating zinc and aluminum nanolamellas. The lamellar nanostructure not only promotes zinc stripping from precursor eutectic Zn Al (at%) alloys, but produces core/shell aluminum/aluminum sesquioxide interlamellar nanopatterns in situ to in turn guide subsequent growth of zinc, enabling dendrite-free zinc stripping/plating for more than 2000 h in oxygen-absent aqueous electrolyte. These outstanding electrochemical properties enlist zinc-ion batteries constructed with Zn Al alloy anode and K MnO cathode to deliver high-density energy at high levels of electrical power and retain 100% capacity after 200 hours. Aqueous rechargeable Zn-ion batteries are attractive energy storage devices, but their wide adoption is impeded by the irreversible metallic Zn anode. Here the authors report lamellar-nanostructured eutectic Zn/Al alloys as reversible and dendrite-free anodes for improved battery performance. |
| ArticleNumber | 1634 |
| Author | Yao, Rui-Qi Lang, Xing-You Wang, Sheng-Bo Zhao, Ming Shi, Hang Wen, Zi Jiang, Qing Ran, Qing |
| Author_xml | – sequence: 1 givenname: Sheng-Bo orcidid: 0000-0002-7114-9262 surname: Wang fullname: Wang, Sheng-Bo organization: Key Laboratory of Automobile Materials (Jilin University), Ministry of Education, and School of Materials Science and Engineering, Jilin University – sequence: 2 givenname: Qing orcidid: 0000-0001-8963-5894 surname: Ran fullname: Ran, Qing organization: Key Laboratory of Automobile Materials (Jilin University), Ministry of Education, and School of Materials Science and Engineering, Jilin University – sequence: 3 givenname: Rui-Qi orcidid: 0000-0002-9910-1463 surname: Yao fullname: Yao, Rui-Qi organization: Key Laboratory of Automobile Materials (Jilin University), Ministry of Education, and School of Materials Science and Engineering, Jilin University – sequence: 4 givenname: Hang orcidid: 0000-0002-7327-3582 surname: Shi fullname: Shi, Hang organization: Key Laboratory of Automobile Materials (Jilin University), Ministry of Education, and School of Materials Science and Engineering, Jilin University – sequence: 5 givenname: Zi orcidid: 0000-0002-6515-441X surname: Wen fullname: Wen, Zi organization: Key Laboratory of Automobile Materials (Jilin University), Ministry of Education, and School of Materials Science and Engineering, Jilin University – sequence: 6 givenname: Ming orcidid: 0000-0002-2096-0880 surname: Zhao fullname: Zhao, Ming organization: Key Laboratory of Automobile Materials (Jilin University), Ministry of Education, and School of Materials Science and Engineering, Jilin University – sequence: 7 givenname: Xing-You orcidid: 0000-0002-8227-9695 surname: Lang fullname: Lang, Xing-You email: xylang@jlu.edu.cn organization: Key Laboratory of Automobile Materials (Jilin University), Ministry of Education, and School of Materials Science and Engineering, Jilin University – sequence: 8 givenname: Qing orcidid: 0000-0003-0660-596X surname: Jiang fullname: Jiang, Qing email: jiangq@jlu.edu.cn organization: Key Laboratory of Automobile Materials (Jilin University), Ministry of Education, and School of Materials Science and Engineering, Jilin University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/32242024$$D View this record in MEDLINE/PubMed |
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| Snippet | Metallic zinc is an attractive anode material for aqueous rechargeable batteries because of its high theoretical capacity and low cost. However,... Aqueous rechargeable Zn-ion batteries are attractive energy storage devices, but their wide adoption is impeded by the irreversible metallic Zn anode. Here the... |
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| SubjectTerms | 639/301/299 639/4077/4079/891 Alloys Aluminum Anodes Aqueous electrolytes Batteries Dendrites Dendritic structure Electric power Electrochemical analysis Electrochemistry Electrode materials Energy storage Eutectic composition Humanities and Social Sciences Lamella Lamellar structure Lithium multidisciplinary Nanostructure Rechargeable batteries Science Science (multidisciplinary) Storage batteries Stripping Zinc Zinc base alloys Zinc plating |
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| Title | Lamella-nanostructured eutectic zinc–aluminum alloys as reversible and dendrite-free anodes for aqueous rechargeable batteries |
| URI | https://link.springer.com/article/10.1038/s41467-020-15478-4 https://www.ncbi.nlm.nih.gov/pubmed/32242024 https://www.proquest.com/docview/2386361802 https://www.proquest.com/docview/2386274275 https://pubmed.ncbi.nlm.nih.gov/PMC7118111 https://doaj.org/article/d03bf99dc3bc4707b830931b3198ce27 |
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