Controlling the fluorescence and room-temperature phosphorescence behaviour of carbon nanodots with inorganic crystalline nanocomposites
There is a significant drive to identify alternative materials that exhibit room temperature phosphorescence for technologies including bio-imaging, photodynamic therapy and organic light-emitting diodes. Ideally, these materials should be non-toxic and cheap, and it will be possible to control thei...
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| Published in | Nature communications Vol. 10; no. 1; pp. 206 - 13 |
|---|---|
| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
14.01.2019
Nature Publishing Group Nature Portfolio |
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| Abstract | There is a significant drive to identify alternative materials that exhibit room temperature phosphorescence for technologies including bio-imaging, photodynamic therapy and organic light-emitting diodes. Ideally, these materials should be non-toxic and cheap, and it will be possible to control their photoluminescent properties. This was achieved here by embedding carbon nanodots within crystalline particles of alkaline earth carbonates, sulphates and oxalates. The resultant nanocomposites are luminescent and exhibit a bright, sub-second lifetime afterglow. Importantly, the excited state lifetimes, and steady-state and afterglow colours can all be systematically controlled by varying the cations and anions in the host inorganic phase, due to the influence of the cation size and material density on emissive and non-emissive electronic transitions. This simple strategy provides a flexible route for generating materials with specific, phosphorescent properties and is an exciting alternative to approaches relying on the synthesis of custom-made luminescent organic molecules.
Materials exhibiting room temperature phosphorescence (RTP) with short afterglow are desirable for bio-medical applications. Here the authors synthesise a library of compounds with tunable RTP properties, embedding carbon nanodots in non-toxic alkaline-earth carbonate, sulphate and oxalate hosts. |
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| AbstractList | There is a significant drive to identify alternative materials that exhibit room temperature phosphorescence for technologies including bio-imaging, photodynamic therapy and organic light-emitting diodes. Ideally, these materials should be non-toxic and cheap, and it will be possible to control their photoluminescent properties. This was achieved here by embedding carbon nanodots within crystalline particles of alkaline earth carbonates, sulphates and oxalates. The resultant nanocomposites are luminescent and exhibit a bright, sub-second lifetime afterglow. Importantly, the excited state lifetimes, and steady-state and afterglow colours can all be systematically controlled by varying the cations and anions in the host inorganic phase, due to the influence of the cation size and material density on emissive and non-emissive electronic transitions. This simple strategy provides a flexible route for generating materials with specific, phosphorescent properties and is an exciting alternative to approaches relying on the synthesis of custom-made luminescent organic molecules.
Materials exhibiting room temperature phosphorescence (RTP) with short afterglow are desirable for bio-medical applications. Here the authors synthesise a library of compounds with tunable RTP properties, embedding carbon nanodots in non-toxic alkaline-earth carbonate, sulphate and oxalate hosts. There is a significant drive to identify alternative materials that exhibit room temperature phosphorescence for technologies including bio-imaging, photodynamic therapy and organic light-emitting diodes. Ideally, these materials should be non-toxic and cheap, and it will be possible to control their photoluminescent properties. This was achieved here by embedding carbon nanodots within crystalline particles of alkaline earth carbonates, sulphates and oxalates. The resultant nanocomposites are luminescent and exhibit a bright, sub-second lifetime afterglow. Importantly, the excited state lifetimes, and steady-state and afterglow colours can all be systematically controlled by varying the cations and anions in the host inorganic phase, due to the influence of the cation size and material density on emissive and non-emissive electronic transitions. This simple strategy provides a flexible route for generating materials with specific, phosphorescent properties and is an exciting alternative to approaches relying on the synthesis of custom-made luminescent organic molecules. Materials exhibiting room temperature phosphorescence (RTP) with short afterglow are desirable for bio-medical applications. Here the authors synthesise a library of compounds with tunable RTP properties, embedding carbon nanodots in non-toxic alkaline-earth carbonate, sulphate and oxalate hosts. There is a significant drive to identify alternative materials that exhibit room temperature phosphorescence for technologies including bio-imaging, photodynamic therapy and organic light-emitting diodes. Ideally, these materials should be non-toxic and cheap, and it will be possible to control their photoluminescent properties. This was achieved here by embedding carbon nanodots within crystalline particles of alkaline earth carbonates, sulphates and oxalates. The resultant nanocomposites are luminescent and exhibit a bright, sub-second lifetime afterglow. Importantly, the excited state lifetimes, and steady-state and afterglow colours can all be systematically controlled by varying the cations and anions in the host inorganic phase, due to the influence of the cation size and material density on emissive and non-emissive electronic transitions. This simple strategy provides a flexible route for generating materials with specific, phosphorescent properties and is an exciting alternative to approaches relying on the synthesis of custom-made luminescent organic molecules.Materials exhibiting room temperature phosphorescence (RTP) with short afterglow are desirable for bio-medical applications. Here the authors synthesise a library of compounds with tunable RTP properties, embedding carbon nanodots in non-toxic alkaline-earth carbonate, sulphate and oxalate hosts. |
| ArticleNumber | 206 |
| Author | Gala de Pablo, Julia Botchway, Stanley W. Johnson, Benjamin R. G. Levenstein, Mark A. Ward, Andrew Green, David C. Meldrum, Fiona C. Zhang, Shuheng Holden, Mark A. |
| Author_xml | – sequence: 1 givenname: David C. surname: Green fullname: Green, David C. email: D.C.Green@leeds.ac.uk organization: School of Chemistry, University of Leeds – sequence: 2 givenname: Mark A. orcidid: 0000-0003-3060-7615 surname: Holden fullname: Holden, Mark A. organization: School of Chemistry, University of Leeds, School of Physics and Astronomy, University of Leeds – sequence: 3 givenname: Mark A. orcidid: 0000-0002-2309-3743 surname: Levenstein fullname: Levenstein, Mark A. organization: School of Chemistry, University of Leeds, School of Mechanical Engineering, University of Leeds – sequence: 4 givenname: Shuheng surname: Zhang fullname: Zhang, Shuheng organization: School of Chemistry, University of Leeds – sequence: 5 givenname: Benjamin R. G. surname: Johnson fullname: Johnson, Benjamin R. G. organization: School of Physics and Astronomy, University of Leeds – sequence: 6 givenname: Julia surname: Gala de Pablo fullname: Gala de Pablo, Julia organization: School of Physics and Astronomy, University of Leeds – sequence: 7 givenname: Andrew surname: Ward fullname: Ward, Andrew organization: Central Laser Facility, Science and Technology Facilities Council, Research Complex at Harwell, Rutherford Appleton Laboratory – sequence: 8 givenname: Stanley W. surname: Botchway fullname: Botchway, Stanley W. organization: Central Laser Facility, Science and Technology Facilities Council, Research Complex at Harwell, Rutherford Appleton Laboratory – sequence: 9 givenname: Fiona C. surname: Meldrum fullname: Meldrum, Fiona C. email: F.Meldrum@leeds.ac.uk organization: School of Chemistry, University of Leeds |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/30643136$$D View this record in MEDLINE/PubMed |
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| Snippet | There is a significant drive to identify alternative materials that exhibit room temperature phosphorescence for technologies including bio-imaging,... Materials exhibiting room temperature phosphorescence (RTP) with short afterglow are desirable for bio-medical applications. Here the authors synthesise a... |
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| SubjectTerms | 140/133 140/146 147/28 639/301/119/995 639/301/54 639/638/440/527 639/925/357 Anions Carbon Carbonates Cations Chemical synthesis Crystal structure Crystallinity Diodes Electron transitions Embedding Fluorescence Humanities and Social Sciences multidisciplinary Nanocomposites Organic chemistry Organic light emitting diodes Oxalates Phosphorescence Photodynamic therapy Photoluminescence Room temperature Science Science (multidisciplinary) Sulfates |
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| Title | Controlling the fluorescence and room-temperature phosphorescence behaviour of carbon nanodots with inorganic crystalline nanocomposites |
| URI | https://link.springer.com/article/10.1038/s41467-018-08214-6 https://www.ncbi.nlm.nih.gov/pubmed/30643136 https://www.proquest.com/docview/2167021209 https://pubmed.ncbi.nlm.nih.gov/PMC6331607 https://doaj.org/article/023d7185c8d84cf6847cb9afb95cdb0b |
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