Dynamic electrocatalyst with current-driven oxyhydroxide shell for rechargeable zinc-air battery
Recent fruitful studies on rechargeable zinc-air battery have led to emergence of various bifunctional oxygen electrocatalysts, especially metal-based materials. However, their electrocatalytic configuration and evolution pathway during battery operation are rarely spotlighted. Herein, to depict the...
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| Published in | Nature communications Vol. 11; no. 1; pp. 1952 - 10 |
|---|---|
| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
23.04.2020
Nature Publishing Group Nature Portfolio |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Recent fruitful studies on rechargeable zinc-air battery have led to emergence of various bifunctional oxygen electrocatalysts, especially metal-based materials. However, their electrocatalytic configuration and evolution pathway during battery operation are rarely spotlighted. Herein, to depict the underlying behaviors, a concept named dynamic electrocatalyst is proposed. By selecting a bimetal nitride as representation, a current-driven “shell-bulk” configuration is visualized via time-resolved X-ray and electron spectroscopy analyses. A dynamic picture sketching the generation and maturation of nanoscale oxyhydroxide shell is presented, and periodic valence swings of performance-dominant element are observed. Upon maturation, zinc-air battery experiences a near two-fold enlargement in power density to 234 mW cm
−2
, a gradual narrowing of voltage gap to 0.85 V at 30 mA cm
−2
, followed by stable cycling for hundreds of hours. The revealed configuration can serve as the basis to construct future blueprints for metal-based electrocatalysts, and push zinc-air battery toward practical application.
Interest in rechargeable Zn-air batteries has been renewed in recent years, however, their oxygen electrocatalysts remain not fully understood. Here the authors reveal the presence of a current-driven oxyhydroxide shell in a so-called dynamic eletrocatalyst that enables optimized battery performance. |
|---|---|
| AbstractList | Recent fruitful studies on rechargeable zinc-air battery have led to emergence of various bifunctional oxygen electrocatalysts, especially metal-based materials. However, their electrocatalytic configuration and evolution pathway during battery operation are rarely spotlighted. Herein, to depict the underlying behaviors, a concept named dynamic electrocatalyst is proposed. By selecting a bimetal nitride as representation, a current-driven "shell-bulk" configuration is visualized via time-resolved X-ray and electron spectroscopy analyses. A dynamic picture sketching the generation and maturation of nanoscale oxyhydroxide shell is presented, and periodic valence swings of performance-dominant element are observed. Upon maturation, zinc-air battery experiences a near two-fold enlargement in power density to 234 mW cm-2, a gradual narrowing of voltage gap to 0.85 V at 30 mA cm-2, followed by stable cycling for hundreds of hours. The revealed configuration can serve as the basis to construct future blueprints for metal-based electrocatalysts, and push zinc-air battery toward practical application.Recent fruitful studies on rechargeable zinc-air battery have led to emergence of various bifunctional oxygen electrocatalysts, especially metal-based materials. However, their electrocatalytic configuration and evolution pathway during battery operation are rarely spotlighted. Herein, to depict the underlying behaviors, a concept named dynamic electrocatalyst is proposed. By selecting a bimetal nitride as representation, a current-driven "shell-bulk" configuration is visualized via time-resolved X-ray and electron spectroscopy analyses. A dynamic picture sketching the generation and maturation of nanoscale oxyhydroxide shell is presented, and periodic valence swings of performance-dominant element are observed. Upon maturation, zinc-air battery experiences a near two-fold enlargement in power density to 234 mW cm-2, a gradual narrowing of voltage gap to 0.85 V at 30 mA cm-2, followed by stable cycling for hundreds of hours. The revealed configuration can serve as the basis to construct future blueprints for metal-based electrocatalysts, and push zinc-air battery toward practical application. Recent fruitful studies on rechargeable zinc-air battery have led to emergence of various bifunctional oxygen electrocatalysts, especially metal-based materials. However, their electrocatalytic configuration and evolution pathway during battery operation are rarely spotlighted. Herein, to depict the underlying behaviors, a concept named dynamic electrocatalyst is proposed. By selecting a bimetal nitride as representation, a current-driven “shell-bulk” configuration is visualized via time-resolved X-ray and electron spectroscopy analyses. A dynamic picture sketching the generation and maturation of nanoscale oxyhydroxide shell is presented, and periodic valence swings of performance-dominant element are observed. Upon maturation, zinc-air battery experiences a near two-fold enlargement in power density to 234 mW cm−2, a gradual narrowing of voltage gap to 0.85 V at 30 mA cm−2, followed by stable cycling for hundreds of hours. The revealed configuration can serve as the basis to construct future blueprints for metal-based electrocatalysts, and push zinc-air battery toward practical application.Interest in rechargeable Zn-air batteries has been renewed in recent years, however, their oxygen electrocatalysts remain not fully understood. Here the authors reveal the presence of a current-driven oxyhydroxide shell in a so-called dynamic eletrocatalyst that enables optimized battery performance. Recent fruitful studies on rechargeable zinc-air battery have led to emergence of various bifunctional oxygen electrocatalysts, especially metal-based materials. However, their electrocatalytic configuration and evolution pathway during battery operation are rarely spotlighted. Herein, to depict the underlying behaviors, a concept named dynamic electrocatalyst is proposed. By selecting a bimetal nitride as representation, a current-driven “shell-bulk” configuration is visualized via time-resolved X-ray and electron spectroscopy analyses. A dynamic picture sketching the generation and maturation of nanoscale oxyhydroxide shell is presented, and periodic valence swings of performance-dominant element are observed. Upon maturation, zinc-air battery experiences a near two-fold enlargement in power density to 234 mW cm −2 , a gradual narrowing of voltage gap to 0.85 V at 30 mA cm −2 , followed by stable cycling for hundreds of hours. The revealed configuration can serve as the basis to construct future blueprints for metal-based electrocatalysts, and push zinc-air battery toward practical application. Interest in rechargeable Zn-air batteries has been renewed in recent years, however, their oxygen electrocatalysts remain not fully understood. Here the authors reveal the presence of a current-driven oxyhydroxide shell in a so-called dynamic eletrocatalyst that enables optimized battery performance. Interest in rechargeable Zn-air batteries has been renewed in recent years, however, their oxygen electrocatalysts remain not fully understood. Here the authors reveal the presence of a current-driven oxyhydroxide shell in a so-called dynamic eletrocatalyst that enables optimized battery performance. Recent fruitful studies on rechargeable zinc-air battery have led to emergence of various bifunctional oxygen electrocatalysts, especially metal-based materials. However, their electrocatalytic configuration and evolution pathway during battery operation are rarely spotlighted. Herein, to depict the underlying behaviors, a concept named dynamic electrocatalyst is proposed. By selecting a bimetal nitride as representation, a current-driven “shell-bulk” configuration is visualized via time-resolved X-ray and electron spectroscopy analyses. A dynamic picture sketching the generation and maturation of nanoscale oxyhydroxide shell is presented, and periodic valence swings of performance-dominant element are observed. Upon maturation, zinc-air battery experiences a near two-fold enlargement in power density to 234 mW cm −2 , a gradual narrowing of voltage gap to 0.85 V at 30 mA cm −2 , followed by stable cycling for hundreds of hours. The revealed configuration can serve as the basis to construct future blueprints for metal-based electrocatalysts, and push zinc-air battery toward practical application. Recent fruitful studies on rechargeable zinc-air battery have led to emergence of various bifunctional oxygen electrocatalysts, especially metal-based materials. However, their electrocatalytic configuration and evolution pathway during battery operation are rarely spotlighted. Herein, to depict the underlying behaviors, a concept named dynamic electrocatalyst is proposed. By selecting a bimetal nitride as representation, a current-driven "shell-bulk" configuration is visualized via time-resolved X-ray and electron spectroscopy analyses. A dynamic picture sketching the generation and maturation of nanoscale oxyhydroxide shell is presented, and periodic valence swings of performance-dominant element are observed. Upon maturation, zinc-air battery experiences a near two-fold enlargement in power density to 234 mW cm , a gradual narrowing of voltage gap to 0.85 V at 30 mA cm , followed by stable cycling for hundreds of hours. The revealed configuration can serve as the basis to construct future blueprints for metal-based electrocatalysts, and push zinc-air battery toward practical application. |
| ArticleNumber | 1952 |
| Author | Liang, Ruilin Luo, Dan Li, Jun-Tao Zhang, Shao-Jian Wang, Xin Deng, Ya-Ping Chen, Zhongwei Jiang, Yi Yu, Aiping Hu, Yongfeng |
| Author_xml | – sequence: 1 givenname: Ya-Ping surname: Deng fullname: Deng, Ya-Ping organization: Department of Chemical Engineering, Waterloo Institute for Nanotechnology, Waterloo Institute for Sustainable Energy, University of Waterloo – sequence: 2 givenname: Yi surname: Jiang fullname: Jiang, Yi organization: Department of Chemical Engineering, Waterloo Institute for Nanotechnology, Waterloo Institute for Sustainable Energy, University of Waterloo – sequence: 3 givenname: Ruilin surname: Liang fullname: Liang, Ruilin organization: Department of Chemical Engineering, Waterloo Institute for Nanotechnology, Waterloo Institute for Sustainable Energy, University of Waterloo – sequence: 4 givenname: Shao-Jian surname: Zhang fullname: Zhang, Shao-Jian organization: College of Energy, Xiamen University – sequence: 5 givenname: Dan orcidid: 0000-0001-9289-888X surname: Luo fullname: Luo, Dan organization: Department of Chemical Engineering, Waterloo Institute for Nanotechnology, Waterloo Institute for Sustainable Energy, University of Waterloo – sequence: 6 givenname: Yongfeng surname: Hu fullname: Hu, Yongfeng organization: Canadian Light Source, University of Saskatchewan – sequence: 7 givenname: Xin orcidid: 0000-0002-4771-8453 surname: Wang fullname: Wang, Xin email: wangxin@scnu.edu.cn organization: South China Academy of Advanced Optoelectronics and International Academy of Optoelectronics at Zhaoqing, South China Normal University – sequence: 8 givenname: Jun-Tao surname: Li fullname: Li, Jun-Tao organization: College of Energy, Xiamen University – sequence: 9 givenname: Aiping surname: Yu fullname: Yu, Aiping organization: Department of Chemical Engineering, Waterloo Institute for Nanotechnology, Waterloo Institute for Sustainable Energy, University of Waterloo – sequence: 10 givenname: Zhongwei orcidid: 0000-0003-3463-5509 surname: Chen fullname: Chen, Zhongwei email: zhwchen@uwaterloo.ca organization: Department of Chemical Engineering, Waterloo Institute for Nanotechnology, Waterloo Institute for Sustainable Energy, University of Waterloo |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/32327651$$D View this record in MEDLINE/PubMed |
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| ContentType | Journal Article |
| Copyright | The Author(s) 2020 The Author(s) 2020. This work is published under http://creativecommons.org/licenses/by/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License. |
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| DOI | 10.1038/s41467-020-15853-1 |
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| Snippet | Recent fruitful studies on rechargeable zinc-air battery have led to emergence of various bifunctional oxygen electrocatalysts, especially metal-based... Interest in rechargeable Zn-air batteries has been renewed in recent years, however, their oxygen electrocatalysts remain not fully understood. Here the... |
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| SubjectTerms | 140/146 639/638/161/886 639/638/161/891 Batteries Bimetals Configurations Electrocatalysts Enlargement Humanities and Social Sciences Maturation Metal air batteries multidisciplinary Oxygen Rechargeable batteries Science Science (multidisciplinary) Spectroscopy Zinc Zinc-oxygen batteries |
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| Title | Dynamic electrocatalyst with current-driven oxyhydroxide shell for rechargeable zinc-air battery |
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