Enhanced carbon dioxide electrolysis at redox manipulated interfaces
Utilization of carbon dioxide from industrial waste streams offers significant reductions in global carbon dioxide emissions. Solid oxide electrolysis is a highly efficient, high temperature approach that reduces polarization losses and best utilizes process heat; however, the technology is relative...
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| Published in | Nature communications Vol. 10; no. 1; pp. 1550 - 10 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
04.04.2019
Nature Publishing Group Nature Portfolio |
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| Online Access | Get full text |
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| Abstract | Utilization of carbon dioxide from industrial waste streams offers significant reductions in global carbon dioxide emissions. Solid oxide electrolysis is a highly efficient, high temperature approach that reduces polarization losses and best utilizes process heat; however, the technology is relatively unrefined for currently carbon dioxide electrolysis. In most electrochemical systems, the interface between active components are usually of great importance in determining the performance and lifetime of any energy materials application. Here we report a generic approach of interface engineering to achieve active interfaces at nanoscale by a synergistic control of materials functions and interface architectures. We show that the redox-manipulated interfaces facilitate the atomic oxygen transfer from adsorbed carbon dioxide molecules to the cathode lattice that determines carbon dioxide electrolysis at elevated temperatures. The composite cathodes with in situ grown interfaces demonstrate significantly enhanced carbon dioxide electrolysis and improved durability.
While solid oxide electrolysis presents an approach to remove CO
2
from high-temperature emission streams, it is challenging to engineer stable yet active interfaces. Here, authors show in situ exsolution of nanoscale metal-metal oxide interfaces that improve cathode activities and durabilities. |
|---|---|
| AbstractList | Utilization of carbon dioxide from industrial waste streams offers significant reductions in global carbon dioxide emissions. Solid oxide electrolysis is a highly efficient, high temperature approach that reduces polarization losses and best utilizes process heat; however, the technology is relatively unrefined for currently carbon dioxide electrolysis. In most electrochemical systems, the interface between active components are usually of great importance in determining the performance and lifetime of any energy materials application. Here we report a generic approach of interface engineering to achieve active interfaces at nanoscale by a synergistic control of materials functions and interface architectures. We show that the redox-manipulated interfaces facilitate the atomic oxygen transfer from adsorbed carbon dioxide molecules to the cathode lattice that determines carbon dioxide electrolysis at elevated temperatures. The composite cathodes with in situ grown interfaces demonstrate significantly enhanced carbon dioxide electrolysis and improved durability.
While solid oxide electrolysis presents an approach to remove CO
2
from high-temperature emission streams, it is challenging to engineer stable yet active interfaces. Here, authors show in situ exsolution of nanoscale metal-metal oxide interfaces that improve cathode activities and durabilities. While solid oxide electrolysis presents an approach to remove CO2 from high-temperature emission streams, it is challenging to engineer stable yet active interfaces. Here, authors show in situ exsolution of nanoscale metal-metal oxide interfaces that improve cathode activities and durabilities. Utilization of carbon dioxide from industrial waste streams offers significant reductions in global carbon dioxide emissions. Solid oxide electrolysis is a highly efficient, high temperature approach that reduces polarization losses and best utilizes process heat; however, the technology is relatively unrefined for currently carbon dioxide electrolysis. In most electrochemical systems, the interface between active components are usually of great importance in determining the performance and lifetime of any energy materials application. Here we report a generic approach of interface engineering to achieve active interfaces at nanoscale by a synergistic control of materials functions and interface architectures. We show that the redox-manipulated interfaces facilitate the atomic oxygen transfer from adsorbed carbon dioxide molecules to the cathode lattice that determines carbon dioxide electrolysis at elevated temperatures. The composite cathodes with in situ grown interfaces demonstrate significantly enhanced carbon dioxide electrolysis and improved durability. Abstract Utilization of carbon dioxide from industrial waste streams offers significant reductions in global carbon dioxide emissions. Solid oxide electrolysis is a highly efficient, high temperature approach that reduces polarization losses and best utilizes process heat; however, the technology is relatively unrefined for currently carbon dioxide electrolysis. In most electrochemical systems, the interface between active components are usually of great importance in determining the performance and lifetime of any energy materials application. Here we report a generic approach of interface engineering to achieve active interfaces at nanoscale by a synergistic control of materials functions and interface architectures. We show that the redox-manipulated interfaces facilitate the atomic oxygen transfer from adsorbed carbon dioxide molecules to the cathode lattice that determines carbon dioxide electrolysis at elevated temperatures. The composite cathodes with in situ grown interfaces demonstrate significantly enhanced carbon dioxide electrolysis and improved durability. Utilization of carbon dioxide from industrial waste streams offers significant reductions in global carbon dioxide emissions. Solid oxide electrolysis is a highly efficient, high temperature approach that reduces polarization losses and best utilizes process heat; however, the technology is relatively unrefined for currently carbon dioxide electrolysis. In most electrochemical systems, the interface between active components are usually of great importance in determining the performance and lifetime of any energy materials application. Here we report a generic approach of interface engineering to achieve active interfaces at nanoscale by a synergistic control of materials functions and interface architectures. We show that the redox-manipulated interfaces facilitate the atomic oxygen transfer from adsorbed carbon dioxide molecules to the cathode lattice that determines carbon dioxide electrolysis at elevated temperatures. The composite cathodes with in situ grown interfaces demonstrate significantly enhanced carbon dioxide electrolysis and improved durability.While solid oxide electrolysis presents an approach to remove CO2 from high-temperature emission streams, it is challenging to engineer stable yet active interfaces. Here, authors show in situ exsolution of nanoscale metal-metal oxide interfaces that improve cathode activities and durabilities. |
| ArticleNumber | 1550 |
| Author | Gan, Lizhen Lemmon, John P. Chen, Fanglin Wang, Wenyuan Xie, Kui Irvine, John T. S. |
| Author_xml | – sequence: 1 givenname: Wenyuan surname: Wang fullname: Wang, Wenyuan organization: Key Laboratory of Design and Assembly of Functional Nanostructures, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences – sequence: 2 givenname: Lizhen surname: Gan fullname: Gan, Lizhen organization: Key Laboratory of Design and Assembly of Functional Nanostructures, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, School of Transportation and Civil Engineering, Fujian Agriculture and Forestry University – sequence: 3 givenname: John P. surname: Lemmon fullname: Lemmon, John P. organization: National Institute of Clean and-Low-Carbon Energy (NICE) – sequence: 4 givenname: Fanglin orcidid: 0000-0001-9942-8872 surname: Chen fullname: Chen, Fanglin organization: Department of Mechanical Engineering, University of South Carolina – sequence: 5 givenname: John T. S. surname: Irvine fullname: Irvine, John T. S. email: jtsi@st-andrews.ac.uk organization: Key Laboratory of Design and Assembly of Functional Nanostructures, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, School of Chemistry, University of St Andrews – sequence: 6 givenname: Kui orcidid: 0000-0002-1215-0271 surname: Xie fullname: Xie, Kui email: kxie@fjirsm.ac.cn organization: Key Laboratory of Design and Assembly of Functional Nanostructures, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/30948715$$D View this record in MEDLINE/PubMed |
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| Snippet | Utilization of carbon dioxide from industrial waste streams offers significant reductions in global carbon dioxide emissions. Solid oxide electrolysis is a... Abstract Utilization of carbon dioxide from industrial waste streams offers significant reductions in global carbon dioxide emissions. Solid oxide electrolysis... While solid oxide electrolysis presents an approach to remove CO2 from high-temperature emission streams, it is challenging to engineer stable yet active... |
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| SubjectTerms | 639/301/299/886 639/4077/4079 639/638/263/915 639/925/357 Atomic oxygen Carbon dioxide Carbon dioxide emissions Cathodes Durability Electrochemistry Electrode polarization Electrolysis High temperature Humanities and Social Sciences Industrial wastes Interfaces multidisciplinary Oxygen transfer Process heat Science Science (multidisciplinary) Waste management Waste streams |
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| Title | Enhanced carbon dioxide electrolysis at redox manipulated interfaces |
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