An exceptionally flexible hydrogen-bonded organic framework with large-scale void regulation and adaptive guest accommodation abilities
Flexible hydrogen-bonded organic frameworks (FHOFs) are quite rare but promising for applications in separation, sensing and host-guest chemistry. They are difficult to stabilize, making their constructions a major challenge. Here, a flexible HOF (named 8PN) with permanent porosity has been successf...
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| Published in | Nature communications Vol. 10; no. 1; pp. 3074 - 8 |
|---|---|
| Main Authors | , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
12.07.2019
Nature Publishing Group Nature Portfolio |
| Subjects | |
| Online Access | Get full text |
| ISSN | 2041-1723 2041-1723 |
| DOI | 10.1038/s41467-019-10575-5 |
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| Abstract | Flexible hydrogen-bonded organic frameworks (FHOFs) are quite rare but promising for applications in separation, sensing and host-guest chemistry. They are difficult to stabilize, making their constructions a major challenge. Here, a flexible HOF (named 8PN) with permanent porosity has been successfully constructed. Nine single crystals of 8PN with different pore structures are obtained, achieving a large-scale void regulation from 4.4% to 33.2% of total cell volume. In response to external stimuli, multimode reversible structural transformations of 8PN accompanied by changes in luminescence properties have been realized. Furthermore, a series of high-quality co-crystals containing guests of varying shapes, sizes, aggregation states and even amounts are obtained, showing that 8PN can adapt to different guests by regulating the molecular conformations and assembling forms of its building blocks. The unexpected flexibility of 8PN makes it a promising material for enriching the applications of existing porous materials.
Flexible hydrogen-bonded organic frameworks (FHOFs) are challenging in fabrication but promising materials for applications in separation and sensing. Here, the authors report a stimuli responsive and flexible HOF which can adapt to different guests by regulating the molecular conformation. |
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| AbstractList | Flexible hydrogen-bonded organic frameworks (FHOFs) are quite rare but promising for applications in separation, sensing and host-guest chemistry. They are difficult to stabilize, making their constructions a major challenge. Here, a flexible HOF (named 8PN) with permanent porosity has been successfully constructed. Nine single crystals of 8PN with different pore structures are obtained, achieving a large-scale void regulation from 4.4% to 33.2% of total cell volume. In response to external stimuli, multimode reversible structural transformations of 8PN accompanied by changes in luminescence properties have been realized. Furthermore, a series of high-quality co-crystals containing guests of varying shapes, sizes, aggregation states and even amounts are obtained, showing that 8PN can adapt to different guests by regulating the molecular conformations and assembling forms of its building blocks. The unexpected flexibility of 8PN makes it a promising material for enriching the applications of existing porous materials.
Flexible hydrogen-bonded organic frameworks (FHOFs) are challenging in fabrication but promising materials for applications in separation and sensing. Here, the authors report a stimuli responsive and flexible HOF which can adapt to different guests by regulating the molecular conformation. Flexible hydrogen-bonded organic frameworks (FHOFs) are quite rare but promising for applications in separation, sensing and host-guest chemistry. They are difficult to stabilize, making their constructions a major challenge. Here, a flexible HOF (named 8PN) with permanent porosity has been successfully constructed. Nine single crystals of 8PN with different pore structures are obtained, achieving a large-scale void regulation from 4.4% to 33.2% of total cell volume. In response to external stimuli, multimode reversible structural transformations of 8PN accompanied by changes in luminescence properties have been realized. Furthermore, a series of high-quality co-crystals containing guests of varying shapes, sizes, aggregation states and even amounts are obtained, showing that 8PN can adapt to different guests by regulating the molecular conformations and assembling forms of its building blocks. The unexpected flexibility of 8PN makes it a promising material for enriching the applications of existing porous materials. Flexible hydrogen-bonded organic frameworks (FHOFs) are quite rare but promising for applications in separation, sensing and host-guest chemistry. They are difficult to stabilize, making their constructions a major challenge. Here, a flexible HOF (named 8PN) with permanent porosity has been successfully constructed. Nine single crystals of 8PN with different pore structures are obtained, achieving a large-scale void regulation from 4.4% to 33.2% of total cell volume. In response to external stimuli, multimode reversible structural transformations of 8PN accompanied by changes in luminescence properties have been realized. Furthermore, a series of high-quality co-crystals containing guests of varying shapes, sizes, aggregation states and even amounts are obtained, showing that 8PN can adapt to different guests by regulating the molecular conformations and assembling forms of its building blocks. The unexpected flexibility of 8PN makes it a promising material for enriching the applications of existing porous materials.Flexible hydrogen-bonded organic frameworks (FHOFs) are quite rare but promising for applications in separation, sensing and host-guest chemistry. They are difficult to stabilize, making their constructions a major challenge. Here, a flexible HOF (named 8PN) with permanent porosity has been successfully constructed. Nine single crystals of 8PN with different pore structures are obtained, achieving a large-scale void regulation from 4.4% to 33.2% of total cell volume. In response to external stimuli, multimode reversible structural transformations of 8PN accompanied by changes in luminescence properties have been realized. Furthermore, a series of high-quality co-crystals containing guests of varying shapes, sizes, aggregation states and even amounts are obtained, showing that 8PN can adapt to different guests by regulating the molecular conformations and assembling forms of its building blocks. The unexpected flexibility of 8PN makes it a promising material for enriching the applications of existing porous materials. Flexible hydrogen-bonded organic frameworks (FHOFs) are challenging in fabrication but promising materials for applications in separation and sensing. Here, the authors report a stimuli responsive and flexible HOF which can adapt to different guests by regulating the molecular conformation. |
| ArticleNumber | 3074 |
| Author | Mao, Zhu Aldred, Matthew P. Qu, Lunjun Yang, Zhiyong Li, Wenlang Zhao, Juan Chi, Zhenguo Huang, Qiuyi Zhang, Yi Li, Yang Zhang, Hao Yu, Tao |
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| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/31300644$$D View this record in MEDLINE/PubMed |
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| Snippet | Flexible hydrogen-bonded organic frameworks (FHOFs) are quite rare but promising for applications in separation, sensing and host-guest chemistry. They are... Flexible hydrogen-bonded organic frameworks (FHOFs) are challenging in fabrication but promising materials for applications in separation and sensing. Here,... |
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| SubjectTerms | 639/301/923/1028 639/301/923/966 639/638/298/923/1028 Cell size Construction Crystal structure Crystals External stimuli Humanities and Social Sciences Hydrogen bonding Luminescence multidisciplinary Optical properties Organic chemistry Porosity Porous materials Science Science (multidisciplinary) Single crystals Supramolecular compounds |
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| Title | An exceptionally flexible hydrogen-bonded organic framework with large-scale void regulation and adaptive guest accommodation abilities |
| URI | https://link.springer.com/article/10.1038/s41467-019-10575-5 https://www.ncbi.nlm.nih.gov/pubmed/31300644 https://www.proquest.com/docview/2256641095 https://www.proquest.com/docview/2257700218 https://pubmed.ncbi.nlm.nih.gov/PMC6625987 https://doaj.org/article/bf193ad1646f4714b4a954fd81f85f70 |
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