Hysteresis-free perovskite solar cells made of potassium-doped organometal halide perovskite
Potassium-doped organometal halide perovskite solar cells (PSCs) of more than 20% power conversion efficiency (PCE) without I-V hysteresis were constructed. The crystal lattice of the organometal halide perovskite was expanded with increasing of the potassium ratio, where both absorption and photolu...
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| Published in | Scientific reports Vol. 7; no. 1; pp. 12183 - 7 |
|---|---|
| Main Authors | , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
22.09.2017
Nature Publishing Group |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Potassium-doped organometal halide perovskite solar cells (PSCs) of more than 20% power conversion efficiency (PCE) without
I-V
hysteresis were constructed. The crystal lattice of the organometal halide perovskite was expanded with increasing of the potassium ratio, where both absorption and photoluminescence spectra shifted to the longer wavelength, suggesting that the optical band gap decreased. In the case of the perovskite with the 5% K
+
, the conduction band minimum (CBM) became similar to the CBM level of the TiO
2
-Li. In this situation, the electron transfer barrier at the interface between TiO
2
-Li and the perovskite was minimised. In fact, the transient current rise at the maximum power voltages of PSCs with 5% K
+
was faster than that without K
+
. It is concluded that stagnation-less carrier transportation could minimise the
I-V
hysteresis of PSCs. |
|---|---|
| AbstractList | Potassium-doped organometal halide perovskite solar cells (PSCs) of more than 20% power conversion efficiency (PCE) without
I-V
hysteresis were constructed. The crystal lattice of the organometal halide perovskite was expanded with increasing of the potassium ratio, where both absorption and photoluminescence spectra shifted to the longer wavelength, suggesting that the optical band gap decreased. In the case of the perovskite with the 5% K
+
, the conduction band minimum (CBM) became similar to the CBM level of the TiO
2
-Li. In this situation, the electron transfer barrier at the interface between TiO
2
-Li and the perovskite was minimised. In fact, the transient current rise at the maximum power voltages of PSCs with 5% K
+
was faster than that without K
+
. It is concluded that stagnation-less carrier transportation could minimise the
I-V
hysteresis of PSCs. Potassium-doped organometal halide perovskite solar cells (PSCs) of more than 20% power conversion efficiency (PCE) without I-V hysteresis were constructed. The crystal lattice of the organometal halide perovskite was expanded with increasing of the potassium ratio, where both absorption and photoluminescence spectra shifted to the longer wavelength, suggesting that the optical band gap decreased. In the case of the perovskite with the 5% K , the conduction band minimum (CBM) became similar to the CBM level of the TiO -Li. In this situation, the electron transfer barrier at the interface between TiO -Li and the perovskite was minimised. In fact, the transient current rise at the maximum power voltages of PSCs with 5% K was faster than that without K . It is concluded that stagnation-less carrier transportation could minimise the I-V hysteresis of PSCs. Potassium-doped organometal halide perovskite solar cells (PSCs) of more than 20% power conversion efficiency (PCE) without I-V hysteresis were constructed. The crystal lattice of the organometal halide perovskite was expanded with increasing of the potassium ratio, where both absorption and photoluminescence spectra shifted to the longer wavelength, suggesting that the optical band gap decreased. In the case of the perovskite with the 5% K+, the conduction band minimum (CBM) became similar to the CBM level of the TiO2-Li. In this situation, the electron transfer barrier at the interface between TiO2-Li and the perovskite was minimised. In fact, the transient current rise at the maximum power voltages of PSCs with 5% K+ was faster than that without K+. It is concluded that stagnation-less carrier transportation could minimise the I-V hysteresis of PSCs.Potassium-doped organometal halide perovskite solar cells (PSCs) of more than 20% power conversion efficiency (PCE) without I-V hysteresis were constructed. The crystal lattice of the organometal halide perovskite was expanded with increasing of the potassium ratio, where both absorption and photoluminescence spectra shifted to the longer wavelength, suggesting that the optical band gap decreased. In the case of the perovskite with the 5% K+, the conduction band minimum (CBM) became similar to the CBM level of the TiO2-Li. In this situation, the electron transfer barrier at the interface between TiO2-Li and the perovskite was minimised. In fact, the transient current rise at the maximum power voltages of PSCs with 5% K+ was faster than that without K+. It is concluded that stagnation-less carrier transportation could minimise the I-V hysteresis of PSCs. Potassium-doped organometal halide perovskite solar cells (PSCs) of more than 20% power conversion efficiency (PCE) without I-V hysteresis were constructed. The crystal lattice of the organometal halide perovskite was expanded with increasing of the potassium ratio, where both absorption and photoluminescence spectra shifted to the longer wavelength, suggesting that the optical band gap decreased. In the case of the perovskite with the 5% K+, the conduction band minimum (CBM) became similar to the CBM level of the TiO2-Li. In this situation, the electron transfer barrier at the interface between TiO2-Li and the perovskite was minimised. In fact, the transient current rise at the maximum power voltages of PSCs with 5% K+ was faster than that without K+. It is concluded that stagnation-less carrier transportation could minimise the I-V hysteresis of PSCs. |
| ArticleNumber | 12183 |
| Author | Wang, Haibin Uchida, Satoshi Murakami, Takurou N. Kubo, Takaya Segawa, Hiroshi Kinoshita, Takumi Awai, Fumiyasu Tang, Zeguo Jono, Ryota Bessho, Takeru Maitani, Masato M. |
| Author_xml | – sequence: 1 givenname: Zeguo surname: Tang fullname: Tang, Zeguo organization: Research Center for Advanced Science and Technology (RCAST), The University of Tokyo, 4-6-1, Komaba, Meguro-ku – sequence: 2 givenname: Takeru surname: Bessho fullname: Bessho, Takeru organization: Research Center for Advanced Science and Technology (RCAST), The University of Tokyo, 4-6-1, Komaba, Meguro-ku – sequence: 3 givenname: Fumiyasu surname: Awai fullname: Awai, Fumiyasu organization: Graduate School of Arts and Sciences, The University of Tokyo, Komaba 3-8-1, Meguro-ku – sequence: 4 givenname: Takumi surname: Kinoshita fullname: Kinoshita, Takumi organization: Research Center for Advanced Science and Technology (RCAST), The University of Tokyo, 4-6-1, Komaba, Meguro-ku – sequence: 5 givenname: Masato M. surname: Maitani fullname: Maitani, Masato M. organization: Research Center for Advanced Science and Technology (RCAST), The University of Tokyo, 4-6-1, Komaba, Meguro-ku – sequence: 6 givenname: Ryota orcidid: 0000-0001-9098-854X surname: Jono fullname: Jono, Ryota organization: Research Center for Advanced Science and Technology (RCAST), The University of Tokyo, 4-6-1, Komaba, Meguro-ku – sequence: 7 givenname: Takurou N. surname: Murakami fullname: Murakami, Takurou N. organization: Research Center for Photovoltaics, National Institute of Advanced Industrial Science and Technology (AIST), 1-1-1 Higashi, Tsukuba – sequence: 8 givenname: Haibin surname: Wang fullname: Wang, Haibin organization: Research Center for Advanced Science and Technology (RCAST), The University of Tokyo, 4-6-1, Komaba, Meguro-ku – sequence: 9 givenname: Takaya surname: Kubo fullname: Kubo, Takaya organization: Research Center for Advanced Science and Technology (RCAST), The University of Tokyo, 4-6-1, Komaba, Meguro-ku – sequence: 10 givenname: Satoshi orcidid: 0000-0002-4971-574X surname: Uchida fullname: Uchida, Satoshi organization: Research Center for Advanced Science and Technology (RCAST), The University of Tokyo, 4-6-1, Komaba, Meguro-ku – sequence: 11 givenname: Hiroshi surname: Segawa fullname: Segawa, Hiroshi email: csegawa@mail.ecc.u-tokyo.ac.jp organization: Research Center for Advanced Science and Technology (RCAST), The University of Tokyo, 4-6-1, Komaba, Meguro-ku, Graduate School of Arts and Sciences, The University of Tokyo, Komaba 3-8-1, Meguro-ku |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/28939887$$D View this record in MEDLINE/PubMed |
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| ContentType | Journal Article |
| Copyright | The Author(s) 2017 2017. This work is published under http://creativecommons.org/licenses/by/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License. |
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| Snippet | Potassium-doped organometal halide perovskite solar cells (PSCs) of more than 20% power conversion efficiency (PCE) without
I-V
hysteresis were constructed.... Potassium-doped organometal halide perovskite solar cells (PSCs) of more than 20% power conversion efficiency (PCE) without I-V hysteresis were constructed.... |
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| SubjectTerms | 140/125 639/4077/909/4101/4096/946 639/638/439/946 Conduction Electron transfer Humanities and Social Sciences Hysteresis multidisciplinary Photons Photovoltaic cells Potassium Science Science (multidisciplinary) Solar cells Titanium dioxide |
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| Title | Hysteresis-free perovskite solar cells made of potassium-doped organometal halide perovskite |
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