Modulation of recombination zone position for quasi-two-dimensional blue perovskite light-emitting diodes with efficiency exceeding 5
In recent years, substantial progress has been made in developing perovskite light-emitting diodes with near-infrared, red and green emissions and over 20% external quantum efficiency. However, the development of perovskite light-emitting diodes with blue emission remains a great challenge, which re...
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| Published in | Nature communications Vol. 10; no. 1; pp. 1027 - 10 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
04.03.2019
Nature Publishing Group Nature Portfolio |
| Subjects | |
| Online Access | Get full text |
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| Abstract | In recent years, substantial progress has been made in developing perovskite light-emitting diodes with near-infrared, red and green emissions and over 20% external quantum efficiency. However, the development of perovskite light-emitting diodes with blue emission remains a great challenge, which retards further development of full-color displays and white-light illumination based on perovskite emissive materials. Here, firstly, through composition and dimensional engineering, we prepare quasi-two-dimensional perovskite thin films with improved blue emission, taking advantages of reduced trap density and enhanced photoluminescence quantum yield. Secondly, we find a vertically non-uniform distribution of perovskite crystals in the PEDOT:PSS/perovskite hybrid film. Through modulating the position of the recombination zone, we activate the majority of quasi-two-dimensional perovskite crystals, and thus demonstrate the most efficient blue perovskite light-emitting diode to date with emission peak at 480 nm, record luminance of 3780 cd m
−2
and record external quantum efficiency of 5.7%.
Halide perovskite based light-emitting diodes attracted intensive research interest recently but the efficiency of blue diodes is much lower than the green and red ones. Here Li et al. push up the efficiency of blue diodes through composition engineering and vertical morphology control. |
|---|---|
| AbstractList | Halide perovskite based light-emitting diodes attracted intensive research interest recently but the efficiency of blue diodes is much lower than the green and red ones. Here Li et al. push up the efficiency of blue diodes through composition engineering and vertical morphology control. In recent years, substantial progress has been made in developing perovskite light-emitting diodes with near-infrared, red and green emissions and over 20% external quantum efficiency. However, the development of perovskite light-emitting diodes with blue emission remains a great challenge, which retards further development of full-color displays and white-light illumination based on perovskite emissive materials. Here, firstly, through composition and dimensional engineering, we prepare quasi-two-dimensional perovskite thin films with improved blue emission, taking advantages of reduced trap density and enhanced photoluminescence quantum yield. Secondly, we find a vertically non-uniform distribution of perovskite crystals in the PEDOT:PSS/perovskite hybrid film. Through modulating the position of the recombination zone, we activate the majority of quasi-two-dimensional perovskite crystals, and thus demonstrate the most efficient blue perovskite light-emitting diode to date with emission peak at 480 nm, record luminance of 3780 cd m-2 and record external quantum efficiency of 5.7%.In recent years, substantial progress has been made in developing perovskite light-emitting diodes with near-infrared, red and green emissions and over 20% external quantum efficiency. However, the development of perovskite light-emitting diodes with blue emission remains a great challenge, which retards further development of full-color displays and white-light illumination based on perovskite emissive materials. Here, firstly, through composition and dimensional engineering, we prepare quasi-two-dimensional perovskite thin films with improved blue emission, taking advantages of reduced trap density and enhanced photoluminescence quantum yield. Secondly, we find a vertically non-uniform distribution of perovskite crystals in the PEDOT:PSS/perovskite hybrid film. Through modulating the position of the recombination zone, we activate the majority of quasi-two-dimensional perovskite crystals, and thus demonstrate the most efficient blue perovskite light-emitting diode to date with emission peak at 480 nm, record luminance of 3780 cd m-2 and record external quantum efficiency of 5.7%. In recent years, substantial progress has been made in developing perovskite light-emitting diodes with near-infrared, red and green emissions and over 20% external quantum efficiency. However, the development of perovskite light-emitting diodes with blue emission remains a great challenge, which retards further development of full-color displays and white-light illumination based on perovskite emissive materials. Here, firstly, through composition and dimensional engineering, we prepare quasi-two-dimensional perovskite thin films with improved blue emission, taking advantages of reduced trap density and enhanced photoluminescence quantum yield. Secondly, we find a vertically non-uniform distribution of perovskite crystals in the PEDOT:PSS/perovskite hybrid film. Through modulating the position of the recombination zone, we activate the majority of quasi-two-dimensional perovskite crystals, and thus demonstrate the most efficient blue perovskite light-emitting diode to date with emission peak at 480 nm, record luminance of 3780 cd m −2 and record external quantum efficiency of 5.7%. Halide perovskite based light-emitting diodes attracted intensive research interest recently but the efficiency of blue diodes is much lower than the green and red ones. Here Li et al. push up the efficiency of blue diodes through composition engineering and vertical morphology control. In recent years, substantial progress has been made in developing perovskite light-emitting diodes with near-infrared, red and green emissions and over 20% external quantum efficiency. However, the development of perovskite light-emitting diodes with blue emission remains a great challenge, which retards further development of full-color displays and white-light illumination based on perovskite emissive materials. Here, firstly, through composition and dimensional engineering, we prepare quasi-two-dimensional perovskite thin films with improved blue emission, taking advantages of reduced trap density and enhanced photoluminescence quantum yield. Secondly, we find a vertically non-uniform distribution of perovskite crystals in the PEDOT:PSS/perovskite hybrid film. Through modulating the position of the recombination zone, we activate the majority of quasi-two-dimensional perovskite crystals, and thus demonstrate the most efficient blue perovskite light-emitting diode to date with emission peak at 480 nm, record luminance of 3780 cd m−2 and record external quantum efficiency of 5.7%.Halide perovskite based light-emitting diodes attracted intensive research interest recently but the efficiency of blue diodes is much lower than the green and red ones. Here Li et al. push up the efficiency of blue diodes through composition engineering and vertical morphology control. In recent years, substantial progress has been made in developing perovskite light-emitting diodes with near-infrared, red and green emissions and over 20% external quantum efficiency. However, the development of perovskite light-emitting diodes with blue emission remains a great challenge, which retards further development of full-color displays and white-light illumination based on perovskite emissive materials. Here, firstly, through composition and dimensional engineering, we prepare quasi-two-dimensional perovskite thin films with improved blue emission, taking advantages of reduced trap density and enhanced photoluminescence quantum yield. Secondly, we find a vertically non-uniform distribution of perovskite crystals in the PEDOT:PSS/perovskite hybrid film. Through modulating the position of the recombination zone, we activate the majority of quasi-two-dimensional perovskite crystals, and thus demonstrate the most efficient blue perovskite light-emitting diode to date with emission peak at 480 nm, record luminance of 3780 cd m −2 and record external quantum efficiency of 5.7%. In recent years, substantial progress has been made in developing perovskite light-emitting diodes with near-infrared, red and green emissions and over 20% external quantum efficiency. However, the development of perovskite light-emitting diodes with blue emission remains a great challenge, which retards further development of full-color displays and white-light illumination based on perovskite emissive materials. Here, firstly, through composition and dimensional engineering, we prepare quasi-two-dimensional perovskite thin films with improved blue emission, taking advantages of reduced trap density and enhanced photoluminescence quantum yield. Secondly, we find a vertically non-uniform distribution of perovskite crystals in the PEDOT:PSS/perovskite hybrid film. Through modulating the position of the recombination zone, we activate the majority of quasi-two-dimensional perovskite crystals, and thus demonstrate the most efficient blue perovskite light-emitting diode to date with emission peak at 480 nm, record luminance of 3780 cd m and record external quantum efficiency of 5.7%. |
| ArticleNumber | 1027 |
| Author | Li, Zhenchao Chen, Ziming Yip, Hin-Lap Yang, Yongchao Cao, Yong Xue, Qifan |
| Author_xml | – sequence: 1 givenname: Zhenchao surname: Li fullname: Li, Zhenchao organization: State Key Laboratory of Luminescent Materials and Devices, Institute of Polymer Optoelectronic Materials and Devices, School of Materials Science and Engineering, South China University of Technology – sequence: 2 givenname: Ziming surname: Chen fullname: Chen, Ziming organization: State Key Laboratory of Luminescent Materials and Devices, Institute of Polymer Optoelectronic Materials and Devices, School of Materials Science and Engineering, South China University of Technology – sequence: 3 givenname: Yongchao surname: Yang fullname: Yang, Yongchao organization: State Key Laboratory of Luminescent Materials and Devices, Institute of Polymer Optoelectronic Materials and Devices, School of Materials Science and Engineering, South China University of Technology – sequence: 4 givenname: Qifan surname: Xue fullname: Xue, Qifan organization: State Key Laboratory of Luminescent Materials and Devices, Institute of Polymer Optoelectronic Materials and Devices, School of Materials Science and Engineering, South China University of Technology – sequence: 5 givenname: Hin-Lap surname: Yip fullname: Yip, Hin-Lap email: msangusyip@scut.edu.cn organization: State Key Laboratory of Luminescent Materials and Devices, Institute of Polymer Optoelectronic Materials and Devices, School of Materials Science and Engineering, South China University of Technology – sequence: 6 givenname: Yong surname: Cao fullname: Cao, Yong organization: State Key Laboratory of Luminescent Materials and Devices, Institute of Polymer Optoelectronic Materials and Devices, School of Materials Science and Engineering, South China University of Technology |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/30833581$$D View this record in MEDLINE/PubMed |
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| Snippet | In recent years, substantial progress has been made in developing perovskite light-emitting diodes with near-infrared, red and green emissions and over 20%... Halide perovskite based light-emitting diodes attracted intensive research interest recently but the efficiency of blue diodes is much lower than the green and... |
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| SubjectTerms | 639/301 639/301/1019/1020/1089 639/624 639/624/1020 639/624/1020/1089 Crystals Efficiency Emission spectra Emissions Emissions control Humanities and Social Sciences Light emitting diodes Luminance multidisciplinary Near infrared radiation Organic light emitting diodes Perovskites Photoluminescence Photons Quantum efficiency Recombination Science Science (multidisciplinary) Thin films White light |
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| Title | Modulation of recombination zone position for quasi-two-dimensional blue perovskite light-emitting diodes with efficiency exceeding 5 |
| URI | https://link.springer.com/article/10.1038/s41467-019-09011-5 https://www.ncbi.nlm.nih.gov/pubmed/30833581 https://www.proquest.com/docview/2187937932 https://www.proquest.com/docview/2188208143 https://pubmed.ncbi.nlm.nih.gov/PMC6399279 https://doaj.org/article/308f267c4a39431a8208bdca7617cd88 |
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